Abstract： Systematic experimental results for atomic magnetic moment and Curie temperature for amorphous alloys FeTmB(Tm=Ti, V, Cr, Mn, Zr, Nb, Mo, Ta, W) prepared by the drum spinning techniqul are reported. The average magnetic moment for each Ye atom is about 2.0 μB in all amorphous FeTmB alloys. The localized characteristics for Tm atom in the amorphous state is much outstanding than in the crystalline state. The average magnetic moment for each IVB(Ti), VB(V), VIB(Cr), VIIB(Mn) atom related with the number of outer electrons per atom is about 4, 5, 4, 3 μB, respectively, and is antiferromagnetic coupling with the Fe magnetic moment. The experimental data of the magnetic moment change rate dμ/dx is in good agreement with the calculated value using a mixed model. According to Friedel's VBS model the delectron states of IVB(Ti), VB(V) elements are completely above the Fermi level EF, but for the VIB(Cr), VIIB(Mn) elements they cross the Fermi level EF.