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The pseudo quaternary system phase diagram of Y2O3-Fe2O3-Bi2O3-PbO·0.2B2O3 is obtained and used. Single crystals of the ferrimagnetic garnet Y3-xBixFe5O12(O≤x≤ 1.2) are grown by using Bi2O3-PbO-B2O3 flux systems. The dependences of the content Bi (x) in the single crystals of Bi-YIG on the compositions of the solutions arediscussed.
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