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Effect of casting process of polymer active layer on performances of polymer solar cells

Xu Miao Peng Jun-Biao

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Effect of casting process of polymer active layer on performances of polymer solar cells

Xu Miao, Peng Jun-Biao
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  • Hole mobility of poly[2-methoxy-5-(2′-ethylhexyloxy)-1,4- phenylenevinylene] (MEH-PPV) film fabricated by spin-casting and drop-casting has been measured by time-of-flight (TOF) technique. The non-dispersive hole transport current waveform is obtained. The results exhibit that the hole mobility of MEH-PPV prepared by drop-casting is higher than that of the film prepared by spin-casting. The solar cells based on MEH-PPV and fullerene derivative blend films prepared by spin-casting and drop-casting,respectively,were fabricated. The power-conversion efficiency (PCE) of the drop-casting device has a great improvement of over 35%,compared with that of spin-casting one. The improvement is attributed to the stronger absorption and better balance of electron and hole transport in MEH-PPV polymer films.
    [1]

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    [3]Sirringhaus H,Kawase T,Friend R H,Shimoda T,Inbasekaran M,Wu W,Woo E P 2000 Science 290 2123

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    [4]Campbell I H,Smith D L,Neef C J,Ferraris J P 1999 Appl. Phys. Lett. 74 2809

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    [5]Blom P W M,de Jong M J M,van Munster M G 1997 Phys. Rev. B 55 R656

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    [6]Sirringhaus H,Brown P J,Friend R H,Nielsen M M,Bechgaard K,Langeveld-Voss B M W,Spiering A J H,Janssen R A J,Meijer E W,Herwig P,de Leeuw D M 1999 Nature 401 685

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    [7]Hertel D,Bassler H 2008 Chemphyschem. 9 666

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    [8]Tian W J,Wen S P,Wu W C,Xia H J,Yang Z F,Zhou Y H 2007 Chin. Phys. 16 2136

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    [9]Peet J,Kim J Y,Coates N E,Ma W L,Moses D,Heeger A J,Bazan G C 2007 Nature Mater. 6 497

    [10]

    ]Li G,Shortriya V,Yao Y,Yang Y 2005 Nature Mater. 4 864

    [11]

    ]Yu H Z,Peng J B 2008 Chin. Phys. B 17 3143

    [12]

    ]Burroughes J H,Bradley D D C,Brown A R,Morks R N,Mackay K,Friend R H,Burn P L,Holmes A B 1990 Nature 347 539

    [13]

    ]Braun D,Heeger A J 1991 Appl. Phys. Lett. 58 1982

    [14]

    ]Gailberger M,Bassler H 1991 Phys. Rev. B 44 8643

    [15]

    ]Yu H Z,Peng J B,Zhou X M,2008 Acta Phys. Sin. 57 3898 (in Chinese)[於黄忠、彭俊彪、周晓明 2008 物理学报 57 3898]

    [16]

    ]Mo Y Q,Huang J,Jiang J X,Deng X Y,Niu Y H Cao Y 2002 Chin. J. Polym. Sci. 20 461

    [17]

    ]Mayer H,Haarer D,Naarmann H,Horhold H H 1995 Phys. Rev. B 52 2587

    [18]

    ]Inigo A R,Tan C H,Fann W S,Huang Y S,Perng G Y,Chen S A 2001 Adv. Mater. 13 504

    [19]

    ]Huang Y F,Inigo A R,Chang C C,Li K C,Liang C F,Chang C W,Lim T S,Chen S H,White J D,Jeng U S,Su A C,Huang Y S,Peng K Y,Chen S A,Pai W W,Lin C H,Tameev A R,Novikov S V,Vannikov A V,Fann W S 2007 Adv. Funct. Mater. 17 2902

    [20]

    ]Frenkel. J 1938 Phys. Rev. 54 647

    [21]

    ]Mihailetchi V D,Xie H,de Boer B,L. Koster J A,Blom P W M 2006 Adv. Funct. Mater. 19 699

    [22]

    ]Mihailetchi V D,Wildeman J,Blom P W M 2005 Phys. Rev. Lett. 94 126602

    [23]

    ]Li G,Yao Y,Yao H,Shortriya V,Yang G,Yang Y 2007 Adv.Funct. Mater. 17 1636

  • [1]

    [1]Friend R H,Gymer R W,Holmes A B,Burroughes J H,Marks R N,Taliani C,Bradley D D C,Dos Santos D A,Brédas J L,Lgdlund M,Salaneck W R 1999 Nature 397 121

    [2]

    [2]Yu G,Gao J,Hummelen J,Wudl F,Heeger A J 1995 Science 270 1789

    [3]

    [3]Sirringhaus H,Kawase T,Friend R H,Shimoda T,Inbasekaran M,Wu W,Woo E P 2000 Science 290 2123

    [4]

    [4]Campbell I H,Smith D L,Neef C J,Ferraris J P 1999 Appl. Phys. Lett. 74 2809

    [5]

    [5]Blom P W M,de Jong M J M,van Munster M G 1997 Phys. Rev. B 55 R656

    [6]

    [6]Sirringhaus H,Brown P J,Friend R H,Nielsen M M,Bechgaard K,Langeveld-Voss B M W,Spiering A J H,Janssen R A J,Meijer E W,Herwig P,de Leeuw D M 1999 Nature 401 685

    [7]

    [7]Hertel D,Bassler H 2008 Chemphyschem. 9 666

    [8]

    [8]Tian W J,Wen S P,Wu W C,Xia H J,Yang Z F,Zhou Y H 2007 Chin. Phys. 16 2136

    [9]

    [9]Peet J,Kim J Y,Coates N E,Ma W L,Moses D,Heeger A J,Bazan G C 2007 Nature Mater. 6 497

    [10]

    ]Li G,Shortriya V,Yao Y,Yang Y 2005 Nature Mater. 4 864

    [11]

    ]Yu H Z,Peng J B 2008 Chin. Phys. B 17 3143

    [12]

    ]Burroughes J H,Bradley D D C,Brown A R,Morks R N,Mackay K,Friend R H,Burn P L,Holmes A B 1990 Nature 347 539

    [13]

    ]Braun D,Heeger A J 1991 Appl. Phys. Lett. 58 1982

    [14]

    ]Gailberger M,Bassler H 1991 Phys. Rev. B 44 8643

    [15]

    ]Yu H Z,Peng J B,Zhou X M,2008 Acta Phys. Sin. 57 3898 (in Chinese)[於黄忠、彭俊彪、周晓明 2008 物理学报 57 3898]

    [16]

    ]Mo Y Q,Huang J,Jiang J X,Deng X Y,Niu Y H Cao Y 2002 Chin. J. Polym. Sci. 20 461

    [17]

    ]Mayer H,Haarer D,Naarmann H,Horhold H H 1995 Phys. Rev. B 52 2587

    [18]

    ]Inigo A R,Tan C H,Fann W S,Huang Y S,Perng G Y,Chen S A 2001 Adv. Mater. 13 504

    [19]

    ]Huang Y F,Inigo A R,Chang C C,Li K C,Liang C F,Chang C W,Lim T S,Chen S H,White J D,Jeng U S,Su A C,Huang Y S,Peng K Y,Chen S A,Pai W W,Lin C H,Tameev A R,Novikov S V,Vannikov A V,Fann W S 2007 Adv. Funct. Mater. 17 2902

    [20]

    ]Frenkel. J 1938 Phys. Rev. 54 647

    [21]

    ]Mihailetchi V D,Xie H,de Boer B,L. Koster J A,Blom P W M 2006 Adv. Funct. Mater. 19 699

    [22]

    ]Mihailetchi V D,Wildeman J,Blom P W M 2005 Phys. Rev. Lett. 94 126602

    [23]

    ]Li G,Yao Y,Yao H,Shortriya V,Yang G,Yang Y 2007 Adv.Funct. Mater. 17 1636

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Publishing process
  • Received Date:  07 May 2009
  • Accepted Date:  15 June 2009
  • Published Online:  15 March 2010

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