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摘要: 用角分辨紫外光电子谱详细研究了V(001)表面上,S和O偏析引起的(4×1)-O,(2×2)-S两超结构,确定了S,O各自引起的吸附态的峰位和对称性;得到了O占据V(001)表面上空位的实验证据。所得实验结果与理论计算相等。
Abstract: Two surface superstructures (4×1)-O and (2×2)-S, induced respectively by oxygen and sulphur segregation on the V(001) surface, are studied in detail by ARVPS. The energy levels and symmetry of the adsorbate surface states derived from S- and O-ordered adsorbate over-layers are determined. Experimental evidence shows that the adsorption sites of oxygen on V(001) surface are four-fold hollow sites. All the experimental results consist with theoretical calculations, and are similar to that for oxygen on Ni(001) and Cr(001) surfaces.