搜索

x
中国物理学会期刊

Zn掺杂p型Ba8Ga16ZnxGe30-x笼合物的合成及热电性能

CSTR: 32037.14.aps.56.4983

Synthesis and thermoelectric properties of p-type Ba8Ga16ZnxGe30-x clathrates

CSTR: 32037.14.aps.56.4983
PDF
导出引用
  • 用熔融法结合放电等离子烧结方法合成了Zn掺杂单相p型Ge基Ⅰ型笼合物Ba8Ga16ZnxGe30-x(x=3, 4, 5, 6),探索Zn取代Ge对其热电性能的影响规律,结果表明:所制备的Ba8Ga16ZnxGe30-x化合物为p型传导,随Zn取代量x 

    Ba8Ga16ZnxGe30-x(x=3, 4, 5, 6) clathrates with different Zn contente were synthesized by melt method reaction and spark plasma sintering. The effect of Zn composition on the thermoelectric properties were investigated. The results show that all samples behave p-type conductor. The electric conductivity and room-temperature carrier mobility decrease with increasing Zn content, and the room-temperature carrier density Np increases with increasing Zn content. Of all p-type Ba8Ga16ZnxGe30-x compounds, Ba8Ga16Zn3Ge27 has the highest Seebeck coefficient, the value of which is 234 μV·K-1 at 300 K, and reaches as high as 295 μV·K-1 around 700 K. The thermal conductivity of Ba8Ga16ZnxGe30-x decrease with increasing x. The maximum ZT value of 0.38 is obtained at 806 K for Ba8Ga16Zn3Ge27.

     

    目录

    /

    返回文章
    返回