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利用532 nm脉冲激光进行水的受激拉曼散射研究，通过改变激光焦点与水-空气界面的距离，获得截然不同的OH伸缩振动受激斯托克斯和反斯托克斯谱线. 焦点距水-空气界面大于20 mm时，只存在 ±3400 cm-1的斯托克斯和反斯托克斯谱线；焦点距离水-空气界面小于20 mm时，存在±3000和± 3400 cm-1的斯托克斯和反斯托克斯谱线；继续缩小焦点与水-空气界面的距离，3000 cm-1谱线被增强，而3400 cm-1谱线被削弱. 研究结果表明，激光诱导水产生的等离子体增强了局部水分子的氢键，导致OH伸缩振动红移，同时过剩电子增强了水的OH伸缩振动受激拉曼散射.
[1] Lee S, Kim J, Lee S, Kim K S 1997 Phys. Rev. Lett. 79 2038
[2] Salzmann C G, Hallbrucker A, Fommey J K, Mayer E 2006 Chem. Phys. Lett. 429 469
[3] Chang H C, Huang K H, Yeh Y L, Lim S H 2000 Chem. Phys. Lett. 326 93
[4] Li F F, Cui Q L, He Z, Cui T, Zhang J, Zhou Q, Zou G T 2005 J. Chem. Phys. 123 174511
[5] Liu C S, Liang Y F, Zhu Z G, Li G X 2005 Chin. Phys. B 14 785
[6] Wei J F, Sun L Q, Zhang K, Hu X Y 2014 Chin. Phys. B 23 074209
[7] Fang W H, Li Z W, Sun C L, Li Z L, Song W, Men Z W, He L Q 2012 Chin. Phys. B 21 034211
[8] Sceats M, Rice S A, Butler J E 1975 J. Chem. Phys. 63 5390
[9] Mikenda W, Steinböck S 1996 J. Mol. Struct. 384 159
[10] Yui H, Yoneda Y, Kitamori T, Sawada T 1999 Phys. Rev. Lett. 82 4110
[11] Yui H, Sawada T 2000 Phys. Rev. Lett. 85 3512
[12] Zhang L, Dong Q L, Zhao J, Wang S J, Sheng Z M, He M Q, Zhang J 2009 Acta Phys. Sin. 58 1837 (in Chinese) [张蕾, 董全力, 赵静, 王首钧, 盛政明, 何民卿, 张杰 2009 物理学报 58 1837]
[13] Braun A, Korn G, Liu X, Du D, Squier J, Mourou G 1995 Opt. Lett. 20 73
[14] Grant K J, Paul G L 1990 Appl. Spectrosc. 44 1349
[15] Telle H R, Laubereau A 1980 Opt. Commun. 34 287
[16] Yui H, Fujiwara H, Sawada T 2002 Chem. Phys. Lett. 360 53
[17] Yui H, Sawada T 2003 Rev. Sci. Instrum. 74 456
[18] Yui H, Nakajima T, Hirao K, Sawada T J 2003 Phys. Chem. A 107 968
[19] Li Z L, Wang Y D, Zhou M, Men Z W, Sun C L, Li Z W 2012 Acta Phys. Sin. 61 064217 (in Chinese) [李占龙, 王一丁, 周密, 门志伟, 孙成林, 里佐威 2012 物理学报 61 064217]
[20] Graener H, Seifert G, Laubereau A 1991 Phys. Rev. Lett. 66 2092
[21] Yui H, Kato H, Someya Y 2008 J. Raman Spectrosc. 39 1688
[22] Walrafen G E 1967 J. Chem. Phys. 47 114
[23] Yui H 2010 Anal. Bioanal. Chem. 397 1181
[24] Zhu Z Q, Wang X L 2011 Acta Phys. Sin. 60 085205 (in Chinese) [朱竹青, 王晓雷 2011 物理学报 60 085205]
[25] Liu X L, Sun S H, Cao Y, Sun M Z, Liu Q C, Hu B T 2013 Acta Phys. Sin. 62 045201 (in Chinese) [刘小亮, 孙少华, 曹瑜, 孙铭泽, 刘情操, 胡碧涛 2013 物理学报 62 045201]
[26] Xu Z J 2013 Ph. D. Dissertation (Tianjin: Nankai University) (in Chinese) [徐智君 2013 博士学位论文 (天津: 南开大学)]
-
[1] Lee S, Kim J, Lee S, Kim K S 1997 Phys. Rev. Lett. 79 2038
[2] Salzmann C G, Hallbrucker A, Fommey J K, Mayer E 2006 Chem. Phys. Lett. 429 469
[3] Chang H C, Huang K H, Yeh Y L, Lim S H 2000 Chem. Phys. Lett. 326 93
[4] Li F F, Cui Q L, He Z, Cui T, Zhang J, Zhou Q, Zou G T 2005 J. Chem. Phys. 123 174511
[5] Liu C S, Liang Y F, Zhu Z G, Li G X 2005 Chin. Phys. B 14 785
[6] Wei J F, Sun L Q, Zhang K, Hu X Y 2014 Chin. Phys. B 23 074209
[7] Fang W H, Li Z W, Sun C L, Li Z L, Song W, Men Z W, He L Q 2012 Chin. Phys. B 21 034211
[8] Sceats M, Rice S A, Butler J E 1975 J. Chem. Phys. 63 5390
[9] Mikenda W, Steinböck S 1996 J. Mol. Struct. 384 159
[10] Yui H, Yoneda Y, Kitamori T, Sawada T 1999 Phys. Rev. Lett. 82 4110
[11] Yui H, Sawada T 2000 Phys. Rev. Lett. 85 3512
[12] Zhang L, Dong Q L, Zhao J, Wang S J, Sheng Z M, He M Q, Zhang J 2009 Acta Phys. Sin. 58 1837 (in Chinese) [张蕾, 董全力, 赵静, 王首钧, 盛政明, 何民卿, 张杰 2009 物理学报 58 1837]
[13] Braun A, Korn G, Liu X, Du D, Squier J, Mourou G 1995 Opt. Lett. 20 73
[14] Grant K J, Paul G L 1990 Appl. Spectrosc. 44 1349
[15] Telle H R, Laubereau A 1980 Opt. Commun. 34 287
[16] Yui H, Fujiwara H, Sawada T 2002 Chem. Phys. Lett. 360 53
[17] Yui H, Sawada T 2003 Rev. Sci. Instrum. 74 456
[18] Yui H, Nakajima T, Hirao K, Sawada T J 2003 Phys. Chem. A 107 968
[19] Li Z L, Wang Y D, Zhou M, Men Z W, Sun C L, Li Z W 2012 Acta Phys. Sin. 61 064217 (in Chinese) [李占龙, 王一丁, 周密, 门志伟, 孙成林, 里佐威 2012 物理学报 61 064217]
[20] Graener H, Seifert G, Laubereau A 1991 Phys. Rev. Lett. 66 2092
[21] Yui H, Kato H, Someya Y 2008 J. Raman Spectrosc. 39 1688
[22] Walrafen G E 1967 J. Chem. Phys. 47 114
[23] Yui H 2010 Anal. Bioanal. Chem. 397 1181
[24] Zhu Z Q, Wang X L 2011 Acta Phys. Sin. 60 085205 (in Chinese) [朱竹青, 王晓雷 2011 物理学报 60 085205]
[25] Liu X L, Sun S H, Cao Y, Sun M Z, Liu Q C, Hu B T 2013 Acta Phys. Sin. 62 045201 (in Chinese) [刘小亮, 孙少华, 曹瑜, 孙铭泽, 刘情操, 胡碧涛 2013 物理学报 62 045201]
[26] Xu Z J 2013 Ph. D. Dissertation (Tianjin: Nankai University) (in Chinese) [徐智君 2013 博士学位论文 (天津: 南开大学)]
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