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中国物理学会期刊

超强飞秒激光脉冲作用下氢分子的高次谐波行为——基于含时密度泛函理论的模拟

CSTR: 32037.14.aps.55.2972

High-order harmonic generation of hydrogen molecule irradiated by ultra-strong femto-second laser pulse——a simulation via TDDFT

CSTR: 32037.14.aps.55.2972
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  • 在含时密度泛函理论框架下,采用经典和量子相结合的模型,模拟了氢分子在超强飞秒激光脉冲作用下的高次谐波行为. 结果表明氢分子的高次谐波谱具有“下降—平台—截止”的结构和偶次谐波被禁闭仅出现奇次谐波的选择性特征;不同的激光偏振方向会导致高次谐波的截止频率和谱线强度的变化.

     

    The high order harmonic generation (HHG) of hydrogen molecule irradiated by ultra-strong femto-second laser pulse is simulated by the TTDFT method with the classical and quantum combination technique. The results indicate that the HHG spectra of H2 have a “decrease-plateau-cutoff” structure. A kind of “odd allowed, even forbidden” selective phenomenon of the order number of HHG is observed. Change in polarization direction of laser beam may change the cut-off order and spectrum intensity of HHG simultaneously.

     

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