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二维材料中的氢隧穿研究进展

辛延波 胡琪 牛栋华 郑晓虎 时洪亮 王玫 肖志松 黄安平 Zhang Zhi-Bin

二维材料中的氢隧穿研究进展

辛延波, 胡琪, 牛栋华, 郑晓虎, 时洪亮, 王玫, 肖志松, 黄安平, Zhang Zhi-Bin
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  • 石墨烯、石墨烯衍生物以及类石墨烯材料通常具有致密的网状晶格结构,研究表明这类材料对分子、原子和离子具有很强的阻挡性.然而对于不同形态的氢粒子(原子、离子、氢气分子)是否能够隧穿二维材料仍然存在很多科学争议,并已成为目前科学研究的一个热点.本文综述了氢隧穿二维材料的研究进展,介绍了不同结构氢粒子隧穿二维材料体系的特点,阐述了氢粒子隧穿不同质量石墨烯和类石墨烯材料时所需要逾越的势垒高度,并对比了其跃迁的难度.讨论了从二维材料本身出发,降低氢隧穿势垒大小和改变环境对氢隧穿过程的影响,实现氢粒子隧穿二维材料.最后展望了氢隧穿二维材料在实际应用中可能存在的问题及未来的研究方向.
      通信作者: 黄安平, aphuang@buaa.edu.cn
    • 基金项目: 国家自然科学基金(批准号:51372008,11574017,11574021,11604007)和北京市科学技术委员会专项计划(批准号:Z161100000216149)资助的课题.
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    [2]

    Bayer T, Bishop S R, Nishihara M, Sasaki K, Lyth S M 2014J.Power Sources 272 239

    [3]

    Forero A B, Ponciano J A C, Bott I S 2014Mater.Corros. 65 531

    [4]

    Wang B, Feng Y H, Wang Q S, Zhang W, Zhang L N, Ma J W, Zhang H R, Yu G H, Wang G Q 2016Acta Phys.Sin. 65 098101(in Chinese)[王彬, 冯雅辉, 王秋实, 张伟, 张丽娜, 马晋文, 张浩然, 于广辉, 王桂强2016物理学报65 098101]

    [5]

    Li X S, Colombo L, Ruoff R S 2016Adv.Mater. 28 6247

    [6]

    Dong Y F, He D W, Wang Y S, Xu H T, Gong Z 2016Acta Phys.Sin. 65 128101(in Chinese)[董艳芳, 何大伟, 王永生, 许海腾, 巩哲2016物理学报65 128101]

    [7]

    Achtyl J L, Unocic R R, Xu L, Cai Y, Raju M, Zhang W, Sacci R L, Vlassiouk I V, Fulvio P F, Ganesh P, Wesolowski D J, Dai S, Van D A C, Neurock M, Geiger F M 2015Nat.Commun. 6 6539

    [8]

    Bunch J S, Verbridge S S, Alden J S, van der Zande A M, Parpia J M, Craighead H G, McEuen P L 2008Nano Lett. 8 2458

    [9]

    Leenaerts O, Partoens B, Peeters F M 2008Appl.Phys.Lett. 93 193107

    [10]

    Wang W L, Kaxiras E 2010New J.Phys. 12 125012

    [11]

    Koenig S P, Wang L, Pellegrino J, Bunch J S 2012Nature Nanotechnol. 7 728

    [12]

    Paul D R 2012Science 335 413

    [13]

    Joshi R K, Carbone P, Wang F C, Kravets V G, Su Y, Grigorieva I V, Wu H A, Geim A K, Nair R R 2014Science 343 752

    [14]

    Miao M, Nardelli M B, Wang Q, Liu Y H 2013PCCP 15 16132

    [15]

    Hu S, Lozada-Hidalgo M, Wang F C, Mishchenko A, Schedin F, Nair R R, Hill E W, Boukhvalov D W, Katsnelson M I, Dryfe R A W, Grigorieva I V, Wu H A, Geim A K 2014Nature 516 227

    [16]

    Lozada-Hidalgo M, Hu S, Marshall O, Mishchenko A, Grigorenko A N, Dryfe R A W, Radha B, Grigorieva I V, Geim A K 2016Science 351 68

    [17]

    Hu S 2014Ph.D.Dissertation(City of Manchester:The University of Manchester)

    [18]

    Du H L, Li J Y, Zhang J, Su G, Li X Y, Zhao Y L 2011J.Phys.Chem.C 115 23261

    [19]

    Novoselov K S, Geim A K, Morozov S V, Jiang D, Zhang Y, Dubonos S V, Grigorieva I V, Firsov A A 2004Science 306 666

    [20]

    Mauritz K A, Moore R B 2004Chem.Rev. 104 4535

    [21]

    Xie D G, Wang Z J, Sun J, Li J, Ma E, Shan Z W 2015Nature Mater. 14 899

    [22]

    Poltavsky I, Zheng L M, Mortazavi M, Tkatchenko A https://arxiv.org/abs/1605.06341[2016-10-28]

    [23]

    Gao W, Wu G, Janicke M T, Cullen D A, Mukundan R, Baldwin J K, Brosha E L, Galande C, Ajayan P M, More K L, Dattelbaum A M, Zelenay P 2014Angew.Chem.Int.Ed. 53 3588

    [24]

    Huang X Q, Lin C F, Yin X L, Zhao R G, Wang E G, Hu Z H 2014Acta Phys.Sin. 63 197301(in Chinese)[黄向前, 林陈昉, 尹秀丽, 赵汝光, 王恩哥, 胡宗海2014物理学报63 197301]

    [25]

    Miura Y, Kasai H, Dio W A, Nakanishi H, Sugimoto T 2003J.Phys.Soc.Jpn. 72 995

    [26]

    Seel M, Pandey R 20162D Materials 3 025004

    [27]

    Poltavsky I, Tkatchenko A 2016Chem.Sci. 7 1368

    [28]

    Nair R R, Wu H A, Jayaram P N, Grigorieva I V, Geim A K 2012Science 335 442

    [29]

    Celebi K, Buchheim J, Wyss R M, Droudian A, Gasser P, Shorubalko I, Kye J I, Lee C, Park H G 2014Science 344 289

    [30]

    Su Y, Kravets V G, Wong S L, Waters J, Geim A K, Nair R R 2014Nat.Commun. 5 4843

    [31]

    O'Hern S C, Jang D, Bose S, Idrobo J C, Song Y, Laoui T, Kong J, Karnik R 2015Nano Lett. 15 3254

    [32]

    Hatakeyama K, Karim M R, Ogata C, Tateishi H, Funatsu A, Taniguchi T, Koinuma M, Hayami S, Matsumoto Y 2014Angew.Chem.Int.Ed. 126 7117

    [33]

    Hatakeyama K, Tateishi H, Taniguchi T, Koinuma M, Kida T, Hayami S, Yokoi H, Matsumoto Y 2014Chem.Mater. 26 5598

    [34]

    He G W, Chang C Y, Xu M Z, Hu S, Li L Q, Zhao J, Li Z, Li Z Y, Yin Y H, Gang M Y, Wu H, Yang X L, Griver M D, Jiang Z Y 2015Adv.Funct.Mater. 25 7502

    [35]

    Ravikumar, Scott K 2012Chem.Commun. 48 5584

    [36]

    Shao J J, Raidongia K, Koltonow A R, Huang J X 2015Nat.Commun. 6 7602

    [37]

    Hatakeyama K, Karim M R, Ogata C, Tateishi H, Taniguchi T, Koinuma M, Hayami S, Matsumoto Y 2014Chem.Commun. 50 14527

    [38]

    Tahat A, MartJ 2014Phys.Rev.E 89 052130

    [39]

    Kenneth B, Wiberg 1955Chem.Rev. 55 713

    [40]

    Jiang D E, Cooper V R, Dai S 2009Nano Lett. 9 4019

    [41]

    Radha B, Esfandiar A, Wang F C, Rooney A P, Gopinadhan K, Keerthi A, Mishchenko A, Janardanan A, Blake P, Fumagalli L, Lozada-hidalgo M, Gara S, Haigh S J, Grigorieva I V, Geim A K 2016Nature 538 222

    [42]

    Pan R, Fan X L, Luo Z F, An Y R 2016Comput.Mater.Sci. 124 106

    [43]

    Zhao Y C, Dai Z H, Sui P F, Zhang X L 2013Acta Phys.Sin. 62 137301(in Chinese)[赵银昌, 戴振宏, 隋鹏飞, 张晓玲2013物理学报62 137301]

    [44]

    Banerjee P, Pathak B, Ahuja R, Das G P 2016Int.J.Hydrogen Energy 41 14437

    [45]

    Tanabe T 2013J.Nucl.Mater. 438 S19

    [46]

    Krauss W, Konys J, Holstein N, Zimmermann H 2011J.Nucl.Mater. 417 1233

    [47]

    Wang Z, Chen T, Chen W, Chang K, Ma L, Huang G, Chen D, Lee J 2013J.Mater.Chem.A 1 2202

    [48]

    Chen Y N, Fu K, Zhu S, Luo W, Wang Y B, Li Y J, Hitz E M, Yao Y G, Dai J Q, Wan J D, Danner V A, Li T, Hu L 2016Nano Lett. 16 3616

    [49]

    Zheng X H, Gao L, Yao Q Z, Li Q Y, Zhang M, Xie X M, Qiao S, Wang G, Ma T B, Di Z F, Luo J B, Wang X 2016Nat.Commun. 7 13204

  • [1]

    Li H, Song Z N, Zhang X J, Huang Y, Li S G, Mao Y T, Ploehn H J, Bao Y, Yu M 2013Science 342 95

    [2]

    Bayer T, Bishop S R, Nishihara M, Sasaki K, Lyth S M 2014J.Power Sources 272 239

    [3]

    Forero A B, Ponciano J A C, Bott I S 2014Mater.Corros. 65 531

    [4]

    Wang B, Feng Y H, Wang Q S, Zhang W, Zhang L N, Ma J W, Zhang H R, Yu G H, Wang G Q 2016Acta Phys.Sin. 65 098101(in Chinese)[王彬, 冯雅辉, 王秋实, 张伟, 张丽娜, 马晋文, 张浩然, 于广辉, 王桂强2016物理学报65 098101]

    [5]

    Li X S, Colombo L, Ruoff R S 2016Adv.Mater. 28 6247

    [6]

    Dong Y F, He D W, Wang Y S, Xu H T, Gong Z 2016Acta Phys.Sin. 65 128101(in Chinese)[董艳芳, 何大伟, 王永生, 许海腾, 巩哲2016物理学报65 128101]

    [7]

    Achtyl J L, Unocic R R, Xu L, Cai Y, Raju M, Zhang W, Sacci R L, Vlassiouk I V, Fulvio P F, Ganesh P, Wesolowski D J, Dai S, Van D A C, Neurock M, Geiger F M 2015Nat.Commun. 6 6539

    [8]

    Bunch J S, Verbridge S S, Alden J S, van der Zande A M, Parpia J M, Craighead H G, McEuen P L 2008Nano Lett. 8 2458

    [9]

    Leenaerts O, Partoens B, Peeters F M 2008Appl.Phys.Lett. 93 193107

    [10]

    Wang W L, Kaxiras E 2010New J.Phys. 12 125012

    [11]

    Koenig S P, Wang L, Pellegrino J, Bunch J S 2012Nature Nanotechnol. 7 728

    [12]

    Paul D R 2012Science 335 413

    [13]

    Joshi R K, Carbone P, Wang F C, Kravets V G, Su Y, Grigorieva I V, Wu H A, Geim A K, Nair R R 2014Science 343 752

    [14]

    Miao M, Nardelli M B, Wang Q, Liu Y H 2013PCCP 15 16132

    [15]

    Hu S, Lozada-Hidalgo M, Wang F C, Mishchenko A, Schedin F, Nair R R, Hill E W, Boukhvalov D W, Katsnelson M I, Dryfe R A W, Grigorieva I V, Wu H A, Geim A K 2014Nature 516 227

    [16]

    Lozada-Hidalgo M, Hu S, Marshall O, Mishchenko A, Grigorenko A N, Dryfe R A W, Radha B, Grigorieva I V, Geim A K 2016Science 351 68

    [17]

    Hu S 2014Ph.D.Dissertation(City of Manchester:The University of Manchester)

    [18]

    Du H L, Li J Y, Zhang J, Su G, Li X Y, Zhao Y L 2011J.Phys.Chem.C 115 23261

    [19]

    Novoselov K S, Geim A K, Morozov S V, Jiang D, Zhang Y, Dubonos S V, Grigorieva I V, Firsov A A 2004Science 306 666

    [20]

    Mauritz K A, Moore R B 2004Chem.Rev. 104 4535

    [21]

    Xie D G, Wang Z J, Sun J, Li J, Ma E, Shan Z W 2015Nature Mater. 14 899

    [22]

    Poltavsky I, Zheng L M, Mortazavi M, Tkatchenko A https://arxiv.org/abs/1605.06341[2016-10-28]

    [23]

    Gao W, Wu G, Janicke M T, Cullen D A, Mukundan R, Baldwin J K, Brosha E L, Galande C, Ajayan P M, More K L, Dattelbaum A M, Zelenay P 2014Angew.Chem.Int.Ed. 53 3588

    [24]

    Huang X Q, Lin C F, Yin X L, Zhao R G, Wang E G, Hu Z H 2014Acta Phys.Sin. 63 197301(in Chinese)[黄向前, 林陈昉, 尹秀丽, 赵汝光, 王恩哥, 胡宗海2014物理学报63 197301]

    [25]

    Miura Y, Kasai H, Dio W A, Nakanishi H, Sugimoto T 2003J.Phys.Soc.Jpn. 72 995

    [26]

    Seel M, Pandey R 20162D Materials 3 025004

    [27]

    Poltavsky I, Tkatchenko A 2016Chem.Sci. 7 1368

    [28]

    Nair R R, Wu H A, Jayaram P N, Grigorieva I V, Geim A K 2012Science 335 442

    [29]

    Celebi K, Buchheim J, Wyss R M, Droudian A, Gasser P, Shorubalko I, Kye J I, Lee C, Park H G 2014Science 344 289

    [30]

    Su Y, Kravets V G, Wong S L, Waters J, Geim A K, Nair R R 2014Nat.Commun. 5 4843

    [31]

    O'Hern S C, Jang D, Bose S, Idrobo J C, Song Y, Laoui T, Kong J, Karnik R 2015Nano Lett. 15 3254

    [32]

    Hatakeyama K, Karim M R, Ogata C, Tateishi H, Funatsu A, Taniguchi T, Koinuma M, Hayami S, Matsumoto Y 2014Angew.Chem.Int.Ed. 126 7117

    [33]

    Hatakeyama K, Tateishi H, Taniguchi T, Koinuma M, Kida T, Hayami S, Yokoi H, Matsumoto Y 2014Chem.Mater. 26 5598

    [34]

    He G W, Chang C Y, Xu M Z, Hu S, Li L Q, Zhao J, Li Z, Li Z Y, Yin Y H, Gang M Y, Wu H, Yang X L, Griver M D, Jiang Z Y 2015Adv.Funct.Mater. 25 7502

    [35]

    Ravikumar, Scott K 2012Chem.Commun. 48 5584

    [36]

    Shao J J, Raidongia K, Koltonow A R, Huang J X 2015Nat.Commun. 6 7602

    [37]

    Hatakeyama K, Karim M R, Ogata C, Tateishi H, Taniguchi T, Koinuma M, Hayami S, Matsumoto Y 2014Chem.Commun. 50 14527

    [38]

    Tahat A, MartJ 2014Phys.Rev.E 89 052130

    [39]

    Kenneth B, Wiberg 1955Chem.Rev. 55 713

    [40]

    Jiang D E, Cooper V R, Dai S 2009Nano Lett. 9 4019

    [41]

    Radha B, Esfandiar A, Wang F C, Rooney A P, Gopinadhan K, Keerthi A, Mishchenko A, Janardanan A, Blake P, Fumagalli L, Lozada-hidalgo M, Gara S, Haigh S J, Grigorieva I V, Geim A K 2016Nature 538 222

    [42]

    Pan R, Fan X L, Luo Z F, An Y R 2016Comput.Mater.Sci. 124 106

    [43]

    Zhao Y C, Dai Z H, Sui P F, Zhang X L 2013Acta Phys.Sin. 62 137301(in Chinese)[赵银昌, 戴振宏, 隋鹏飞, 张晓玲2013物理学报62 137301]

    [44]

    Banerjee P, Pathak B, Ahuja R, Das G P 2016Int.J.Hydrogen Energy 41 14437

    [45]

    Tanabe T 2013J.Nucl.Mater. 438 S19

    [46]

    Krauss W, Konys J, Holstein N, Zimmermann H 2011J.Nucl.Mater. 417 1233

    [47]

    Wang Z, Chen T, Chen W, Chang K, Ma L, Huang G, Chen D, Lee J 2013J.Mater.Chem.A 1 2202

    [48]

    Chen Y N, Fu K, Zhu S, Luo W, Wang Y B, Li Y J, Hitz E M, Yao Y G, Dai J Q, Wan J D, Danner V A, Li T, Hu L 2016Nano Lett. 16 3616

    [49]

    Zheng X H, Gao L, Yao Q Z, Li Q Y, Zhang M, Xie X M, Qiao S, Wang G, Ma T B, Di Z F, Luo J B, Wang X 2016Nat.Commun. 7 13204

  • 引用本文:
    Citation:
计量
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  • 被引次数: 0
出版历程
  • 收稿日期:  2016-10-29
  • 修回日期:  2016-12-07
  • 刊出日期:  2017-03-05

二维材料中的氢隧穿研究进展

  • 1. 北京航空航天大学 物理科学与核能工程学院, 北京 100191;
  • 2. 北京大学物理学院, 量子材料科学中心, 北京 100871;
  • 3. Department of Engineering Sciences, Uppsala University, SE-75121, Uppsala, Sweden
  • 通信作者: 黄安平, aphuang@buaa.edu.cn
    基金项目: 

    国家自然科学基金(批准号:51372008,11574017,11574021,11604007)和北京市科学技术委员会专项计划(批准号:Z161100000216149)资助的课题.

摘要: 石墨烯、石墨烯衍生物以及类石墨烯材料通常具有致密的网状晶格结构,研究表明这类材料对分子、原子和离子具有很强的阻挡性.然而对于不同形态的氢粒子(原子、离子、氢气分子)是否能够隧穿二维材料仍然存在很多科学争议,并已成为目前科学研究的一个热点.本文综述了氢隧穿二维材料的研究进展,介绍了不同结构氢粒子隧穿二维材料体系的特点,阐述了氢粒子隧穿不同质量石墨烯和类石墨烯材料时所需要逾越的势垒高度,并对比了其跃迁的难度.讨论了从二维材料本身出发,降低氢隧穿势垒大小和改变环境对氢隧穿过程的影响,实现氢粒子隧穿二维材料.最后展望了氢隧穿二维材料在实际应用中可能存在的问题及未来的研究方向.

English Abstract

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