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金属玻璃的键态特征与塑性起源

袁晨晨

金属玻璃的键态特征与塑性起源

袁晨晨
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  • 由于缺乏位错、晶界等典型的晶格缺陷,金属玻璃体系中承载力的形变单元为短程序或中程序原子团簇,键的强度及成键方向是影响原子间协调变形能力主要因素.本文通过与晶态合金对比,指出金属玻璃中原子键合方式与宏观力学性能的潜在关系,综述了金属材料电子结构与力学性能内在关系的最新研究进展,并系统介绍了金属玻璃电子结构特征、表征参量和主要测试手段,使读者对金属玻璃体系中原子间的键态特征有较清晰的认识,对进一步探索本征塑性较好的金属玻璃体系具有一定指导意义.
      通信作者: 袁晨晨, yuanchenchenneu@163.com
    • 基金项目: 国家自然科学基金(批准号:51601038,51631003)、江苏省自然科学基金(批准号:BK20171354)、国家重点基础研究发展计划(批准号:2016YFB0300502)和中央高校基本科研业务费(批准号:2242017K40189)资助的课题.
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    Yang W M, Liu H S, Zhao Y C, Inoue A, Jiang K M, Huo J T, Ling H B, Li Q, Shen B L 2014 Sci. Rep. 4 6233

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    Eberhart M E, Clougherty D P 2004 Nat. Mater. 3 659

    [2]

    Eberhart M E, Giamei A F 1998 Mater. Sci. Eng. A: Struct. Mater. Prop. Microstruct. Process. 248 287

    [3]

    Jones T E, Eberhart M E, Clougherty D P, Woodward C 2008 Phys. Rev. Lett. 101 085505.

    [4]

    Liu Y, Chen K Y, Lu G, Zhang J H, Hu Z Q 1997 Acta Mater. 45 1837

    [5]

    Krasko G L, Olson G B 1990 Solid State Commun. 76 247

    [6]

    Lejcek P 2010 Grain Boundary Segregation in Metals (Vol. 136) (Berlin, Heidelberg: Springer-Verlag Press) p1

    [7]

    Sloman H A 1932 J. I. Met. 49 365

    [8]

    Lee H T, Brick R M 1952 J. I. Met. 4 147

    [9]

    Rosi F D, Dube C A, Alexander B H 1953 Trans. Am. I. Min. Metall. Eng. 197 257

    [10]

    Pugh S F 1954 Philos. Mag. 45 823

    [11]

    Bader R F W 1998 J. Phys. Chem. A 102 7314

    [12]

    Gschneidner K A, Ji M, Wang C Z, Ho K M, Russell A M, Mudryk Y, Becker A T, Larson J L 2009 Acta Mater. 57 5876

    [13]

    Maclaren J M, Crampin S, Vvedensky D D, Eberhart M E 1989 Phys. Rev. Lett. 63 2586

    [14]

    Maclaren J M, Gonis A, Schadler G 1992 Phys. Rev. B 45 14392.

    [15]

    Eberhart M E, Vvedensky D D 1987 Phys. Rev. Lett. 58 61

    [16]

    Eberhart M E 1999 Sci. Am. 281 66

    [17]

    Eberhart M E 1996 Acta Mater. 44 2495

    [18]

    Nakashima P N H, Smith A E, Etheridge J, Muddle B C 2011 Science 331 1583

    [19]

    Eberhart M E, Clougherty D P, Maclaren J M 1993 Philos. Mag. B: Phys. Condens. Matter Stat. Mech. Electron. Opt. Magn. Prop. 68 455

    [20]

    Eberhart M E, Jones T E, Sauer M A 2008 JOM 60 67

    [21]

    Eberhart M E 1996 Philos. Mag. A: Phys. Condens. Matter Struct. Defect Mech. Prop. 73 47

    [22]

    Beltz G E, Selinger R L B, Kim K S, Marder M P 1999 Fracture and Ductile Vs. Brittle Behavior-Theory, Modelling and Experiment (Vol. 539) (Cambridge: Cambridge University Press) p13

    [23]

    Eberhart M E, Donovan, M M, Maclaren, J M, Clougherty, D P 1991 Prog. Surf. Sci. 36 1

    [24]

    Niu H Y, Chen X Q, Liu P T, Xing W W, ChengX Y, Li D Z, Li Y Y 2012 Sci. Rep. 2 718

    [25]

    Ogata S, Li J, Yip S 2002 Science 298 807

    [26]

    Morinaga M, Saito J, Yukawa N, Adachi H 1990 Acta Metall. Mater. 38 25

    [27]

    Heredia F E, Pope D P 1991 Acta Metall. Mater. 39 2017

    [28]

    Lejcek P, Hofmann S 1995 Crit. Rev. Solid State Mater. Sci. 20 1

    [29]

    Datta A, Waghmare U V, Ramamurty U 2008 Acta Mater. 56 2531

    [30]

    Cheng Y Q, Cao A J, Ma E 2009 Acta Mater. 57 3253

    [31]

    Weaire D, Ashby M F, Logan J, Weins M J 1971 Acta Metall. 19 779

    [32]

    Cheng Y Q, Ma E 2011 Acta Mater. 59 1800

    [33]

    Wang W H 2007 Prog. Mater. Sci. 52 540

    [34]

    Spaepen F 1977 Acta Metall. 25 407

    [35]

    Argon A S 1979 Acta Metall. 27 47

    [36]

    Spaepen F 2006 Scr. Mater. 54 363

    [37]

    Johnson W L, Samwer K 2005 Phys. Rev. Lett. 95 195501

    [38]

    Wang W H 2005 J. Non-Cryst. Solids 351 1481

    [39]

    Wang W H 2006 J. Appl. Phys. 99 093506

    [40]

    Rouxel T 2007 J. Am. Ceram. Soc. 90 3019

    [41]

    Fukuhara M, Takahashi M, Kawazoe Y, Inoue A 2007 Appl. Phys. Lett. 90 073114

    [42]

    Mayou D, Nguyenmanh D, Pasturel A, Cyrotlackmann F 1986 Phys. Rev. B 33 3384

    [43]

    Tamura R, Takeuchi T, Aoki C, Takeuchi S, Kiss T, Yokoya T, Shin S 2004 Phys. Rev. Lett. 92 146402

    [44]

    Huang L, Wang C Z, Hao S G, Kramer M J, Ho K M 2010 Phys. Rev. B 81 014108

    [45]

    Yuan C C, Yang F, Kargl F, Holland-Moritz D, Simeoni G G, Meyer A 2015 Phys. Rev. B 91 214203

    [46]

    Amamou A, Krill G 1979 Solid State Commun. 31 971

    [47]

    Amamou A 1979 Phys. Status Solidi A: Appl. Res. 54 565

    [48]

    He Q A, Cheng Y Q, Ma E, Xu J A 2011 Acta Mater. 59 202

    [49]

    Cheng Y Q, Ma E, Sheng H W 2009 Phys. Rev. Lett. 102 245501

    [50]

    Weinert M, Watson R E 1998 Phys. Rev. B 58 9732

    [51]

    Sandor M T, Kecskes L J, He Q, Xu J, Wu Y 2011 Chin. Sci. Bull. 56 3937

    [52]

    Wang X F, Jones T E, Wu Y, Lu Z P, Halas S, DurakiewiczT, Eberhart M E 2014 J. Chem. Phys. 141 024503

    [53]

    Gu X J, Poon S J, Shiflet G J, Widom M 2008 Acta Mater. 56 88

    [54]

    Mitra A, Jiles D C 1997 J. Magn. Magn. Mater. 168 169

    [55]

    Duwez P, Lin S C H 1967 J. Appl. Phys. 38 4096

    [56]

    Nishiyama N, Inoue A 1996 Mater. T. JIM 37 1531

    [57]

    Xu D H, Duan G, Johnson W L 2004 Phys. Rev. Lett. 92 245504

    [58]

    Shen J, Liang W Z, Sun J F 2006 Appl. Phys. Lett. 89 121908

    [59]

    Inoue A, Shen B L, Yavari A R, Greer A L 2003 J. Mater. Res. 18 1487

    [60]

    Mott N F, Davis E A 1979 Electronic Processes in Non-Crystalline Materials (Oxford: Clarendon Press) Chaps. 5

    [61]

    Miracle D B 2004 Nat. Mater. 3 697

    [62]

    Sheng H W, Luo W K, Alamgir F M, Bai J M, Ma E 2006 Nature 439 419

    [63]

    Zeng Q, Sheng H, Ding Y, Wang L, Yang W, Jiang J Z, Mao W L, Mao H K 2011 Science 332 1404

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    Xi X K, Sandor M T, Wang H J, Wang J Q, Hwang W, Wu Y 2011 J. Phys.-Condes. Matter 23 115501

    [65]

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    [67]

    Oelhafen P, Hauser E, Guntherodt H J, Bennemann K H 1979 Phys. Rev. Lett. 43 1134

    [68]

    Amamou A 1980 Solid State Commun. 33 1029

    [69]

    Park R L 1975 Phys. Today 28 52

    [70]

    Onn D G, Johnson W D, Gleeson P F, Donnelly T A, Egami T, Liebermann H H 1977 J. Phys. C: Solid State Phys. 10 639

    [71]

    Butler N H 1977 Phys. Rev. B: Solid State 15 5267

    [72]

    Yang D P, Hines W A, Tsai C L, Giessen B C, Lu F C 1991 J. Appl. Phys. 69 6225

    [73]

    Hines W A, Glover K, Clark W G, Kabacoff L T, Modzelewski C U, Hasegawa R, Duwez P 1980 Phys. Rev. B 21 3771

    [74]

    Narath A 1969 Phys. Rev. 179 359

    [75]

    Panissod P, Guerra D A, Amamou A, Durand J, Johnson W L, Carter W L, Poon S J 1980 Phys. Rev. Lett. 44 1465

    [76]

    Xi X K, Li L L, Zhang B, Wang W H, Wu Y 2007 Phys. Rev. Lett. 99 095501.

    [77]

    Zhang Y D, Budnick J I, Ford J C, Hines W A 1991 J. Magn. Magn. Mater. 100 13

    [78]

    Pokatillov V S 2007 Phys. Solid State 49 2217

    [79]

    Imafuku M, Saito K, Kanehashi K, Saida J, Sato S, Inoue A 2005 J. Non-Cryst. Solids 351 3587

    [80]

    Breitzke H, Luders K, Scudino S, Kuhn U, Eckert J 2004 Phys. Rev. B 70 014201

    [81]

    Panissod P, Bakonyi I, Hasegawa R 1983 Phys. Rev. B 28 2374

    [82]

    Yuan C C, Xiang J F, Xi X K, Wang W H 2011 Phys. Rev. Lett. 107 236403

    [83]

    Yuan C C, Yang Y F, Xi X K 2013 J. Appl. Phys. 114 213511

    [84]

    Yuan C C, Shen X, Cui J, Gu L, Yu R C, Xi X K 2012 Appl. Phys. Lett. 101 021902

    [85]

    Yang W M, Liu H S, Zhao Y C, Inoue A, Jiang K M, Huo J T, Ling H B, Li Q, Shen B L 2014 Sci. Rep. 4 6233

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  • 收稿日期:  2017-06-01
  • 修回日期:  2017-06-27
  • 刊出日期:  2017-09-05

金属玻璃的键态特征与塑性起源

    基金项目: 

    国家自然科学基金(批准号:51601038,51631003)、江苏省自然科学基金(批准号:BK20171354)、国家重点基础研究发展计划(批准号:2016YFB0300502)和中央高校基本科研业务费(批准号:2242017K40189)资助的课题.

摘要: 由于缺乏位错、晶界等典型的晶格缺陷,金属玻璃体系中承载力的形变单元为短程序或中程序原子团簇,键的强度及成键方向是影响原子间协调变形能力主要因素.本文通过与晶态合金对比,指出金属玻璃中原子键合方式与宏观力学性能的潜在关系,综述了金属材料电子结构与力学性能内在关系的最新研究进展,并系统介绍了金属玻璃电子结构特征、表征参量和主要测试手段,使读者对金属玻璃体系中原子间的键态特征有较清晰的认识,对进一步探索本征塑性较好的金属玻璃体系具有一定指导意义.

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