硅烯的化学功能化

杨硕; 程鹏; 陈岚; 吴克辉

doi:10.7498/aps.66.216805

摘要

硅烯是一种零能隙的狄拉克费米子材料，对其能带结构的有效调控进而打开带隙是硅烯进一步器件化的基础.而化学功能化是调控二维材料的结构和电子性质的一种有效方法.本文简要介绍了近几年在硅烯的化学功能化方面取得的进展，主要包括硅烯的氢化、氧化、氯化以及其他几种可能的化学修饰方法.

关键词:

Silicene exhibits extraordinary physical properties especially Dirac fermion characteristics. However, the zero-gap band structure of silicene hinders its applications in nanoelectronic and optoelectronic devices. It is thus desirable to open a finite band gap in silicene. Chemical functionalization is a commonly used method to tailor the structures and electronic properties of two-dimensional materials. In this paper we review the recent 3-year progress of silicene, including its hydrogenation, oxidization, halogenation, and other methods to modify silicene.

Keywords:

作者及机构信息

1.
中国科学院物理研究所, 北京 100190

通信作者: 程鹏, pcheng@iphy.ac.cn

基金项目: 国家自然科学基金（批准号：11674368）资助的课题.

Authors and contacts

1.
Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China

Corresponding author: Cheng Peng, pcheng@iphy.ac.cn

Funds: Project supported by the National Natural Science Foundation of China (Grant No. 11674368).

参考文献

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[32]	Du Y, Zhuang J, Liu H, Xu X, Eilers S, Wu K, Cheng P, Zhao J, Pi X, See K W, Peleckis G, Wang X, Dou S X 2014 ACS Nano 8 10019
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[34]	Du Y, Zhuang J C, Wang J, Li Z, Liu H S, Zhao J J, Xu X, Feng H F, Chen L, Wu K H, Wang X L, Dou S X 2016 Sci. Adv. 2 e1600067
[35]	Gao N, Zheng W T, Jiang Q 2012 Phys. Chem. Chem. Phys. 14 257
[36]	Fu H X, Ren J, Chen L, Si C, Qiu J L, Li W B, Zhang J, Sun J T, Li H, Wu K H, Duan W H, Meng S 2016 Euro Phys. Lett. 113 67003
[37]	Li W B, Sheng S X, Chen J, Cheng P, Chen L, Wu K H 2016 Phys. Rev. B 93 155410
[38]	Osborn T H, Farajian A A 2012 J. Phys. Chem. C 116 22916
[39]	Sivek J, Sahin H, Partoens B, Peeters F M 2013 Phys. Rev. B 87 085444
[40]	Pi X D, Ni Z Y, Liu Y, Ruan Z, Xu M, Yang D 2015 Phys. Chem. Chem. Phys. 17 4146
[41]	Wang R, Xu M S, Pi X D 2015 Chin. Phys. B 24 086807
[42]	Zheng R, Lin X, Ni J 2014 Appl. Phys. Lett. 105 092410
[43]	Friedlein R, van Bui H, Wiggers F B, Yamada-Takamura Y, Kovalgin A Y, de Jong M P 2014 J. Chem. Phys. 140 204705
[44]	Friedlein R, Fleurence A, Sadowski J T, Yamada-Takamura Y 2013 Appl. Phys. Lett. 102 221603
[45]	Zhao T, Zhang S, Wang Q, Kawazoe Y, Jena P 2014 Phys. Chem. Chem. Phys. 16 22979

施引文献

[1]	Guzmn-Verri G G, Lew Yan Voon L C 2007 Phys. Rev. B 76 075131
[2]	Cahangirov S, Topsakal M, Aktrk E, Şahin H, Ciraci S 2009 Phys. Rev. Lett. 102 236804
[3]	Liu C C, Feng W, Yao Y G 2011 Phys. Rev. Lett. 107 076802
[4]	Vogt P, de Padova P, Quaresima C, Avila J, Frantzeskakis E, Asensio M C, Resta A, Ealet B, Le Lay G 2012 Phys. Rev. Lett. 108 155501
[5]	Feng B J, Ding Z J, Meng S, Yao Y G, He X Y, Cheng P, Chen L, Wu K H 2012 Nano Lett. 12 3507
[6]	Lin C L, Arafune R, Kawahara K, Tsukahara N, Minamitani E, Kim Y, Takagi N, Kawai M 2012 Appl. Phys. Express 5 045802
[7]	Jamgotchian H, Colignon Y, Hamzaoui N, Ealet B, Hoarau J Y, Aufray B, Bibrian J P 2012 J. Phys.: Condens. Matter 24 172001
[8]	Enriquez H, Vizzini S, Kara A, Lalmi B, Oughaddou H 2012 J. Phys.: Condens. Matter 24 314211
[9]	Gou J, Zhong Q, Sheng S X, Li W B, Cheng P, Li H, Chen L, Wu K H 2016 2D Mater. 3 045005
[10]	Zhu F F, Chen W J, Xu Y, Gao C L, Guan D D, Liu C H, Qian D, Zhang S C, Jia J F 2015 Nat. Mater. 14 1020
[11]	Li K L, Yu Y J, Ye G J, Ge Q Q, Ou X D, Wu H, Feng D L, Chen X H, Zhang Y B 2014 Nat. Nanotech. 9 372
[12]	Feng B J, Zhang J, Zhong Q, Li W, Li S, Li H, Wu K 2016 Nat. Chem. 8 563
[13]	Chen L, Liu C C, Feng B J, He X Y, Cheng P, Ding Z J, Meng S, Yao Y G, Wu K H 2012 Phys. Rev. Lett. 109 056804
[14]	Chen J, Du Y, Li Z, Li W B, Feng B J, Qiu J L, Cheng P, Dou S X, Chen L, Wu K H 2015 Sci. Rep. 5 13590
[15]	Zhuang J C, Xu X, Du Y, Wu K H, Chen L, Hao W, Dou S X 2015 Phys. Rev. B 91 161409
[16]	Tao L, Cinquanta E, Chiappe D, Grazianetti C, Fanciulli M, Dubey M, Molle A, Akinwande D 2015 Nat. Nanotechnol. 10 227
[17]	Tsai W F, Huang C Y, Chang T, Lin R H, Jeng H T, Bansil A 2013 Nat. Commun. 4 1500
[18]	Ezawa M 2012 Phys. Rev. Lett. 109 055502
[19]	Ezawa M 2013 Phys. Rev. Lett. 110 026603
[20]	Tabert C J, Nicol E J 2013 Phys. Rev. Lett. 110 197402
[21]	Pan H, Li Z, Liu C C, Zhu G, Qiao Z, Yao Y G 2014 Phys. Rev. Lett. 112 106802
[22]	Sofo J O, Chaudhari A S, Barber G D 2007 Phys. Rev. B 75 153401
[23]	Lebgue S, Klintenberg M, Eriksson O, Katsnelson M 2009 Phys. Rev. B 79 245117
[24]	Voon L C L Y, Sandberg E, Aga R S, Farajian A A 2010 Appl. Phys. Lett. 97 163114
[25]	Houssa M, Scalise E, Sankaran K, Pourtois G, Afanas'ev V V, Stesmans A 2011 Appl. Phys. Lett. 98 223107
[26]	Zhang P, Li X D, Hu C H, Wu S Q, Zhu Z Z 2012 Phys. Lett. A 376 1230
[27]	Qiu J L, Fu H X, Xu Y, Oreshkin A I, Shao T N, Li H, Meng S, Chen L, Wu K H 2015 Phys. Rev. Lett. 114 126101
[28]	Qiu J L, Fu H X, Xu Y, Zhong Q, Meng S, Li H, Chen L, Wu K H 2015 ACS Nano 9 11192
[29]	Padova P D, Ottaviani C, Quaresima C, Olivieri B, Imperatori P, Salomon E, Angot T, Quagliano L, Romano C, Vona A, Muniz-Miranda M, Generosi A, Paci B, Lay G L 2014 2D Mater. 1 021003
[30]	Molle A, Grazianetti C, Chiappe D, Cinquanta E, Cianci E, Tallarida G, Fanciulli M 2013 Adv. Funct. Mater. 23 4340
[31]	Wang R, Pi X, Ni Z, Liu Y, Lin S, Xu M, Yang D 2013 Sci. Rep. 3 3507
[32]	Du Y, Zhuang J, Liu H, Xu X, Eilers S, Wu K, Cheng P, Zhao J, Pi X, See K W, Peleckis G, Wang X, Dou S X 2014 ACS Nano 8 10019
[33]	Xu X, Zhuang J C, Du Y, Feng H F, Zhang N, Liu C, Lei T, Wang J, Spencer M, Morishita T, Wang X L, Dou S X 2014 Sci. Rep. 4 7543
[34]	Du Y, Zhuang J C, Wang J, Li Z, Liu H S, Zhao J J, Xu X, Feng H F, Chen L, Wu K H, Wang X L, Dou S X 2016 Sci. Adv. 2 e1600067
[35]	Gao N, Zheng W T, Jiang Q 2012 Phys. Chem. Chem. Phys. 14 257
[36]	Fu H X, Ren J, Chen L, Si C, Qiu J L, Li W B, Zhang J, Sun J T, Li H, Wu K H, Duan W H, Meng S 2016 Euro Phys. Lett. 113 67003
[37]	Li W B, Sheng S X, Chen J, Cheng P, Chen L, Wu K H 2016 Phys. Rev. B 93 155410
[38]	Osborn T H, Farajian A A 2012 J. Phys. Chem. C 116 22916
[39]	Sivek J, Sahin H, Partoens B, Peeters F M 2013 Phys. Rev. B 87 085444
[40]	Pi X D, Ni Z Y, Liu Y, Ruan Z, Xu M, Yang D 2015 Phys. Chem. Chem. Phys. 17 4146
[41]	Wang R, Xu M S, Pi X D 2015 Chin. Phys. B 24 086807
[42]	Zheng R, Lin X, Ni J 2014 Appl. Phys. Lett. 105 092410
[43]	Friedlein R, van Bui H, Wiggers F B, Yamada-Takamura Y, Kovalgin A Y, de Jong M P 2014 J. Chem. Phys. 140 204705
[44]	Friedlein R, Fleurence A, Sadowski J T, Yamada-Takamura Y 2013 Appl. Phys. Lett. 102 221603
[45]	Zhao T, Zhang S, Wang Q, Kawazoe Y, Jena P 2014 Phys. Chem. Chem. Phys. 16 22979

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