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基于高精细度光腔锁频激光的分子吸收光谱测量

康鹏 孙羽 王进 刘安雯 胡水明

基于高精细度光腔锁频激光的分子吸收光谱测量

康鹏, 孙羽, 王进, 刘安雯, 胡水明
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  • 利用高精细度光腔锁定激光频率,实现了对分子吸收光谱的高精度测量.光腔采用低热膨胀系数的殷钢结构设计和温度控制,实现了腔长度的稳定;通过将激光频率锁定在光腔纵模上,实现了高频率精度和高灵敏度的光腔衰荡光谱测量.利用该装置示范性地测量了二氧化碳分子在6470.42 cm-1附近的光腔衰荡光谱和色散光谱,得到了高精度的谱线参数,并和数据库谱线参数进行了对比.
      通信作者: 胡水明, smhu@ustc.edu.cn
    • 基金项目: 国家自然科学基金(批准号:21688102,21427804)资助的课题.
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  • [1]

    Daussy C, Guinet M, Amy-Klein A, Djerroud K, Hermier Y, Briaudeau S, Borde Ch J, Chardonnet C 2007 Phys. Rev. Lett. 98 250801

    [2]

    Moretti L, Castrillo A, Fasci E, de Vizia M D, Casa G, Galzerano G, Merlone A, Laporta P, Gianfrani L 2013 Phys. Rev. Lett. 111 060803

    [3]

    Cheng C F, Wang J, Sun Y R, Tan Y, Kang P, Hu S M 2015 Metrologia 52 S385

    [4]

    Morville J, Chenevier M, Kachanov A A, Romanini D 2002 Proc. SPIE 4485 236

    [5]

    Dudek J B, Tarsa P B, Velasquez A, Wladyslawski M, Rabinowitz P, Lehmann K K 2003 Anal. Chem. 75 4599

    [6]

    Crosson E R 2008 Appl. Phys. B 92 403

    [7]

    Chen B, Kang P, Li J Y, He X L, Liu A W, Hu S M 2015 Chin. J. Chem. Phys. 28 6

    [8]

    Rothman L S, Gordon I E, Babikov Y, Barbe A, Benner D C, Bernath P F, Birk M, Bizzocchi L, Boudon V, Brown L R, Campargue A, Chance K, Cohen E A, Coudert L H, Devi V M, Drouin B J, Fayt A, Flaud J M, Gamache R R, Harrison J J, Hartmann J M, Hill C, Hodges J T, Jacquemart D, Jolly A, Lamouroux J, Le Roy R J, Li G, Long D A, Lyulin O M, Mackie C J, Massie S T, Mikhailenko S, Muller H S P, Naumenko O V, Nikitin A V, Orphal J, Perevalov V, Perrin A, Polovtseva E R, Richard C, Smith M A H, Starikova E, Sung K, Tashkun S, Tennyson J, Toon G C, Tyuterev V G, Wagner G 2013 J. Quant. Spectrosc. Radiat. Transf. 130 4

    [9]

    Jiang J, Bernard J E, Madej A A, Czajkowski A, Drissler S, Jones D J 2007 J. Opt. Soc. Am. B 24 2727

    [10]

    Madej A A, Alcock A J, Czajkowski A, Bernard J E, Chepurov S 2006 J. Opt. Soc. Am. B 23 2200

    [11]

    Okubo S, Nakayama H, Iwakuni K, Inaba H, Sasada H 2011 Opt. Express 19 23878

    [12]

    Robichaud D J, Hodges J T, Maslowski P, Yeung L Y, Okumura M, Miller C E, Brown L R 2008 J. Mol. Spectrosc. 251 27

    [13]

    Swann W C, Gilbert S L 2002 J. Opt. Soc. Am. B 19 2461

    [14]

    Takahata K, Kobayashi T, Sasada H, Nakajima Y, Inaba H, Hong F L 2009 Phys. Rev. A 80 032518

    [15]

    Titov D V, Svedhem H, Mccoy D, Lebreton J P, Barabash S, Bertaux J L, Drossart P, Formisano V, Haeusler B, Korablev O I, Markiewicz W, Neveance D, Petzold M, Piccioni G, Zhang T L, Taylor F W, Lellouch E, Koschny D, Witasse O, Warhaut M, Acomazzo A, Rodrigues-Cannabal J, Fabrega J, Schirmann T, Clochet A, Coradini M 2006 Cosmic. Res. 44 334

    [16]

    Ammannito E, Filacchione G, Coradini A, Capaccioni F, Piccioni G, de Sanctis M C, Dami M, Barbis A 2006 Rev. Sci. Instrum. 77 093109

    [17]

    Graf J E, Zurek R W, Erickson J K, Jai B, Johnston M D, de Paula R 2007 Acta Astronaut. 61 44

    [18]

    Krasnopolsky V A 2006 Icarus 185 153

    [19]

    Bailey J, Simpson A, Crisp D 2007 Publ. Astron. Soc. Pac. 119 228

    [20]

    Butz A, Guerlet S, Hasekamp O, Schepers D, Galli A, Aben I, Frankenberg C, Hartmann J M, Tran H, Kuze A, Keppel-Aleks G, Toon G, Wunch D, Wennberg P, Deutscher N, Griffith D, Macatangay R, Messerschmidt J, Notholt J, Warneke T 2011 Geophys. Res. Lett. 38 L14812

    [21]

    Crisp D, Atlas R M, Breon F M, Brown L R, Burrows J P, Ciais P, Connor B J, Doney S C, Fung I Y, Jacob D J, Miller C E, O'Brien D, Pawson S, Randerson J T, Rayner P, Salawitch R J, Sander S P, Sen B, Stephens G L, Tans P P, Toon G C, Wennberg P O, Wofsy S C, Yung Y L, Kuang Z, Chudasama B, Sprague G, Weiss B, Pollock R, Kenyon D, Schroll S 2004 Adv. Space. Res. Ser. 34 700

    [22]

    Zhang H, Lin C, Zheng Y Q, Wang W Q, Tian L F, Liu D B, Li S 2016 J. Appl. Remote. Sens. 10 024003

    [23]

    Miller C E, Brown L R, Toth R A, Benner D C, Devi V M 2005 C. R. Phys. 6 876

    [24]

    Miller C E, Crisp D, de Cola P L, Olsen S C, Randerson J T, Michalak A M, Alkhaled A, Rayner P, Jacob D J, Suntharalingam P, Jones D B A, Denning A S, Nicholls M E, Doney S C, Pawson S, Boesch H, Connor B J, Fung I Y, O'Brien D, Salawitch R J, Sander S P, Sen B, Tans P, Toon G C, Wennberg P O, Wofsy S C, Yung Y L, Law R M 2007 J. Geophys. Res. Atmos. 112 D10314

    [25]

    Boudjaadar D, Mandin J Y, Dana V, Picque N, Guelachvili G 2006 J. Mol. Spectrosc. 236 158

    [26]

    Jacquemart D, Borkov Y G, Lyulin O M, Tashkun S A, Perevalov V I 2015 J. Quant. Spectrosc. Radiat. Transf. 160 1

    [27]

    Karlovets E V, Campargue A, Mondelain D, Beguier S, Kassi S, Tashkun S A, Perevalov V I 2013 J. Quant. Spectrosc. Radiat. Transf. 130 116

    [28]

    O'keefe A, Deacon D A G 1988 Rev. Sci. Instrum. 59 2544

    [29]

    Gagliardi G, Loock H P 2014 Cavity Enhanced Spectroscopy and Sensing (Berlin:Springer) pp1-60

    [30]

    Pan H, Cheng C F, Sun Y R, Gao B, Liu A W, Hu S M 2011 Rev. Sci. Instrum. 82 103110

    [31]

    Gatti D, Sala T, Gotti R, Cocola L, Poletto L, Prevedelli M, Laporta P, Marangoni M 2015 J. Chem. Phys. 142 074201

    [32]

    Martinez R Z, Metsala M, Vaittinen O, Lantta T, Halonen L 2006 J. Opt. Soc. Am. B 23 727

    [33]

    Hodges J T, Layer H P, Miller W W, Scace G E 2004 Rev. Sci. Instrum. 75 849

    [34]

    Cygan A, Lisak D, Maslowski P, Bielska K, Wojtewicz S, Domyslawska J, Trawinski R S, Ciurylo R, Abe H, Hodges J T 2011 Rev. Sci. Instrum. 82 063107

    [35]

    Wang J, Sun Y R, Tao L G, Liu A W, Hua T P, Meng F, Hu S M 2017 Rev. Sci. Instrum. 88 043108

    [36]

    Wang J, Sun Y R, Tao L G, Liu A W, Hu S M 2017 J. Chem. Phys. 147 091103

    [37]

    Chen B, Sun Y R, Zhou Z Y, Chen J, Liu A W, Hu S M 2014 Appl. Opt. 53 7716

    [38]

    Cygan A, Lisak D, Morzynski P, Bober M, Zawada M, Pazderski E, Ciurylo R 2013 Opt. Express 21 29744

    [39]

    Cygan A, Wcislo P, Wojtewicz S, Maslowski P, Hodges J T, Ciurylo R, Lisak D 2015 Opt. Express 23 14472

    [40]

    Cygan A, Wojtewicz S, Zaborowski M, Wcislo P, Guo R M, Ciurylo R, Lisak D 2016 Meas. Sci. Technol. 27 045501

    [41]

    Ma W G, Foltynowicz A, Axner O 2008 J. Opt. Soc. Am. B 25 1144

    [42]

    Toth R A, Brown L R, Miller C E, Devi V M, Benner D C 2006 J. Mol. Spectrosc. 239 243

    [43]

    ftp://ftp.iao.ru/pub/CDSD-296/[2017-11-27]

    [44]

    Perevalov B V, Kassi S, Perevalov V I, Tashkun S A, Campargue A 2008 J. Mol. Spectrosc. 252 143

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  • 收稿日期:  2017-11-27
  • 修回日期:  2018-03-12
  • 刊出日期:  2018-05-20

基于高精细度光腔锁频激光的分子吸收光谱测量

  • 1. 中国科学技术大学, 合肥微尺度物质科学国家实验室, 合肥 230026
  • 通信作者: 胡水明, smhu@ustc.edu.cn
    基金项目: 

    国家自然科学基金(批准号:21688102,21427804)资助的课题.

摘要: 利用高精细度光腔锁定激光频率,实现了对分子吸收光谱的高精度测量.光腔采用低热膨胀系数的殷钢结构设计和温度控制,实现了腔长度的稳定;通过将激光频率锁定在光腔纵模上,实现了高频率精度和高灵敏度的光腔衰荡光谱测量.利用该装置示范性地测量了二氧化碳分子在6470.42 cm-1附近的光腔衰荡光谱和色散光谱,得到了高精度的谱线参数,并和数据库谱线参数进行了对比.

English Abstract

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