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Effects of V substitution for Mn on charge ordering and spin-glass state in La0.45Ca0.55MnO3 sample

Wang Gui-Ying Guo Huan-Yin Mao Qiang Yang Gang Peng Zhen-Sheng

Effects of V substitution for Mn on charge ordering and spin-glass state in La0.45Ca0.55MnO3 sample

Wang Gui-Ying, Guo Huan-Yin, Mao Qiang, Yang Gang, Peng Zhen-Sheng
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  • The polycrystalline samples of La0.45Ca0.55Mn1-xVxO3(x=0.00, 0.10) have been prepared by the solid-phase reaction. Efects of V5+ substitution for Mn3+/Mn4+ on charge ordering and spin-glass state are studied by X-ray diffraction spectrum, temperature dependence of magnetization, and electron spin resonance spectra. The results indicate that charge ordering of the original system is almost destroyed, and spin-glass state at about 40 K is melted by 10% of V substitution for Mn. The charge ordering phase is destroyed mainly because of V5+ ions substitution for Mn3+/Mn4+, which increases the ratio of Mn3+ to Mn4+ and so causes ferromagnetic double-exchange to be superior to antiferromagnetic super-exchange. In addition, the spin-glass state is melted because V substitution for Mn destroys the formation condition of spin-glass state that a small quantity of ferromagnetic components exist under the antiferromagnetic backgrornd.
    • Funds:
    [1]

    Jin S, Tiefel T H, McConmack M, Fastnacht R A, Ramesh R, Chen L H, Rao C N R, Raveau B 1994 Science 264 413

    [2]

    Autret C, Gervais M, Gervais F, Raimboux N, Simon P 2004 Solid State Sci. 6 815

    [3]

    Salamon M B, Jaime M 2001 Rev. Mod. Phys. 73 583

    [4]

    Zener C 1951 Phys. Rev. 82 403

    [5]

    Millis A J, Littlewoo P B, Shraiman B I 1995 Phys. Rev. Lett. 74 5144

    [6]

    Yu J, Zhang J C, Cao G X, Wang S P, Jing C, Cao S X 2006 Acta Phys. Sin. 55 5190 (in Chinese) [俞 坚、 张金仓、 曹桂新、 王仕鹏、 敬 超、 曹世勋 2006 物理学报 55 5190]

    [7]

    Peng Z S, Guo H Y, Cai Z R, Wang G Y 2008 Chin. J. Low Temp. Phys. 30 298 (in Chinese) [彭振生、 郭焕银、 蔡之让、 王桂英 2008 低温物理学报 30 298]

    [8]

    Xu M X, Jiao Z K 1998 Acta Phys. Sin. 47 1007 (in Chinese) [徐明祥、 焦正宽1998 物理学报 47 1007]

    [9]

    Kiryukhin V, Casa D, Hill J P, Keimer B, Vigliante A, Tomioka Y, Tokura Y 1997 Nature 386 813

    [10]

    Li X J, Wang Q 2009 Acta Phys. Sin. 58 6482 (in Chinese) [李晓娟、 王 强 2009物理学报 58 6482]

    [11]

    Chen C H, Cheong S W 1996 Phys. Rev. Lett. 76 4042

    [12]

    Mori S, Chen C H, Cheong S W 1998 Nature 392 473

    [13]

    Peng Z S 2004 J. Rare Earths 22 232

    [14]

    Vanitha P V, Singh R S, Natarajan S, Rao C N R 1998 J. Solid State Chem. 137 365

    [15]

    Wang G Y, Yan G Q, Mao Q, Liu N, Peng Z S, Guo H Y 2009 Chin. Rare Earths 30 10 (in Chinese) [王桂英、 严国清、 毛 强、 刘 宁、 彭振生、 郭焕银 2009 稀土 30 10]

    [16]

    Liang Y, Peng Z S, Yan G Q, Guo H Y, Cai Z R 2005 J. Rare Metals 28 513 (in Chinese) [梁 燕、 彭振生、 严国清、 郭焕银、 蔡之让 2005 稀有金属 28 513]

    [17]

    Qu Z, Pi L, Fan J Y, Zhang B, Zhang T, Tan S, Zhang B, Zhang M, Zhang Y H 2007 Chin. Phys. 16 258

    [18]

    Shu M M, Cao S X, Gao T, Yuan S J, Kang B J, Yu L M, Zhang J C 2009 Acta Phys. Sin. 58 3309 (in Chinese) [舒苗苗、 曹世勋、 高 湉、 袁淑娟、 康保娟、 郁黎明、 张金仓 2009 物理学报 58 3309]

    [19]

    Liu N, Yan G Q, Cai Z R, Guo H Y, Peng Z S, Qu Z, Zhang Y H 2005 Chin. Sci. Bull. 50 1492 (in Chinese) [刘 宁、 严国清、 蔡之让、 郭焕银、 彭振生、 曲 哲、 张裕恒 2005 科学通报 50 1492]

    [20]

    Rivadulla F, Freita-Alvite M, Lopez-Quinteal M A 2002 J. Appl. Phys. 91 785

    [21]

    Kuwahara H, Tomioka Y, Asamitsu A, Moritomo Y, Tokura Y 1995 Science 270 961

    [22]

    Asamitsu A, TomiokaY, Kuwahara H, Tokura Y 1997 Nature 388 55

    [23]

    Tokunaga M, Miura N , TomikaY, Tokura Y 1998 Phys. Rev. B 57 5259

    [24]

    Damay F, Maignan A, Martin C, Raveah B 1997 J. Appl. Phys. 82 1458

    [25]

    Li R W, Sun J R, Wang Z H, Zhang S Y, Tong N, Shen B G 2000 J. Appl. Phys. 88 7041

    [26]

    Damay F, Martin C, Maignan A, Hervien M, Raveah B 1998 Appl. Phys. Lett. 73 3772

    [27]

    Zhu Y W, Fang J, Huang Z, Gao B J 2003 Chin. J. Low Temp. Phys. 25 151 (in Chinese) [朱永文、 方 军、 黄 真、 高秉钧 2003 低温物理学报 25 151]

    [28]

    Guo H Y, Liu N, Cai Z R, Zhang Y H 2006 Acta Phys. Sin. 55 865 (in Chinese) [郭焕银、 刘 宁、 蔡之让、 张裕恒 2006 物理学报 55 865]

    [29]

    Wang S P, Zhang J C, Cao G X, Yu J, Jing C, Cao S X 2006 Acta Phys. Sin. 55 367 (in Chinese) [王仕鹏、 张金仓、 曹桂新、 俞 坚、 敬 超、 曹世勋 2006 物理学报 55 367]

    [30]

    Kundaliya D C, Vij R, Kulkarni R G, Tulapurkar A A, Pinto R, Malik S K, Yelon W B 2003 J. Magn. Magn. Mater. 264 62

    [31]

    Chen Z P, Wang C M, Li Y F, Su Y L, Liu D W, Li T, Zhang J C 2009 Cryo. Supercond. 37 76 (in Chinese) [陈镇平、 王春梅、 李越峰、 苏玉玲、 刘德伟、 李 涛、 张金仓 2009 低温与超导 37 76]

  • [1]

    Jin S, Tiefel T H, McConmack M, Fastnacht R A, Ramesh R, Chen L H, Rao C N R, Raveau B 1994 Science 264 413

    [2]

    Autret C, Gervais M, Gervais F, Raimboux N, Simon P 2004 Solid State Sci. 6 815

    [3]

    Salamon M B, Jaime M 2001 Rev. Mod. Phys. 73 583

    [4]

    Zener C 1951 Phys. Rev. 82 403

    [5]

    Millis A J, Littlewoo P B, Shraiman B I 1995 Phys. Rev. Lett. 74 5144

    [6]

    Yu J, Zhang J C, Cao G X, Wang S P, Jing C, Cao S X 2006 Acta Phys. Sin. 55 5190 (in Chinese) [俞 坚、 张金仓、 曹桂新、 王仕鹏、 敬 超、 曹世勋 2006 物理学报 55 5190]

    [7]

    Peng Z S, Guo H Y, Cai Z R, Wang G Y 2008 Chin. J. Low Temp. Phys. 30 298 (in Chinese) [彭振生、 郭焕银、 蔡之让、 王桂英 2008 低温物理学报 30 298]

    [8]

    Xu M X, Jiao Z K 1998 Acta Phys. Sin. 47 1007 (in Chinese) [徐明祥、 焦正宽1998 物理学报 47 1007]

    [9]

    Kiryukhin V, Casa D, Hill J P, Keimer B, Vigliante A, Tomioka Y, Tokura Y 1997 Nature 386 813

    [10]

    Li X J, Wang Q 2009 Acta Phys. Sin. 58 6482 (in Chinese) [李晓娟、 王 强 2009物理学报 58 6482]

    [11]

    Chen C H, Cheong S W 1996 Phys. Rev. Lett. 76 4042

    [12]

    Mori S, Chen C H, Cheong S W 1998 Nature 392 473

    [13]

    Peng Z S 2004 J. Rare Earths 22 232

    [14]

    Vanitha P V, Singh R S, Natarajan S, Rao C N R 1998 J. Solid State Chem. 137 365

    [15]

    Wang G Y, Yan G Q, Mao Q, Liu N, Peng Z S, Guo H Y 2009 Chin. Rare Earths 30 10 (in Chinese) [王桂英、 严国清、 毛 强、 刘 宁、 彭振生、 郭焕银 2009 稀土 30 10]

    [16]

    Liang Y, Peng Z S, Yan G Q, Guo H Y, Cai Z R 2005 J. Rare Metals 28 513 (in Chinese) [梁 燕、 彭振生、 严国清、 郭焕银、 蔡之让 2005 稀有金属 28 513]

    [17]

    Qu Z, Pi L, Fan J Y, Zhang B, Zhang T, Tan S, Zhang B, Zhang M, Zhang Y H 2007 Chin. Phys. 16 258

    [18]

    Shu M M, Cao S X, Gao T, Yuan S J, Kang B J, Yu L M, Zhang J C 2009 Acta Phys. Sin. 58 3309 (in Chinese) [舒苗苗、 曹世勋、 高 湉、 袁淑娟、 康保娟、 郁黎明、 张金仓 2009 物理学报 58 3309]

    [19]

    Liu N, Yan G Q, Cai Z R, Guo H Y, Peng Z S, Qu Z, Zhang Y H 2005 Chin. Sci. Bull. 50 1492 (in Chinese) [刘 宁、 严国清、 蔡之让、 郭焕银、 彭振生、 曲 哲、 张裕恒 2005 科学通报 50 1492]

    [20]

    Rivadulla F, Freita-Alvite M, Lopez-Quinteal M A 2002 J. Appl. Phys. 91 785

    [21]

    Kuwahara H, Tomioka Y, Asamitsu A, Moritomo Y, Tokura Y 1995 Science 270 961

    [22]

    Asamitsu A, TomiokaY, Kuwahara H, Tokura Y 1997 Nature 388 55

    [23]

    Tokunaga M, Miura N , TomikaY, Tokura Y 1998 Phys. Rev. B 57 5259

    [24]

    Damay F, Maignan A, Martin C, Raveah B 1997 J. Appl. Phys. 82 1458

    [25]

    Li R W, Sun J R, Wang Z H, Zhang S Y, Tong N, Shen B G 2000 J. Appl. Phys. 88 7041

    [26]

    Damay F, Martin C, Maignan A, Hervien M, Raveah B 1998 Appl. Phys. Lett. 73 3772

    [27]

    Zhu Y W, Fang J, Huang Z, Gao B J 2003 Chin. J. Low Temp. Phys. 25 151 (in Chinese) [朱永文、 方 军、 黄 真、 高秉钧 2003 低温物理学报 25 151]

    [28]

    Guo H Y, Liu N, Cai Z R, Zhang Y H 2006 Acta Phys. Sin. 55 865 (in Chinese) [郭焕银、 刘 宁、 蔡之让、 张裕恒 2006 物理学报 55 865]

    [29]

    Wang S P, Zhang J C, Cao G X, Yu J, Jing C, Cao S X 2006 Acta Phys. Sin. 55 367 (in Chinese) [王仕鹏、 张金仓、 曹桂新、 俞 坚、 敬 超、 曹世勋 2006 物理学报 55 367]

    [30]

    Kundaliya D C, Vij R, Kulkarni R G, Tulapurkar A A, Pinto R, Malik S K, Yelon W B 2003 J. Magn. Magn. Mater. 264 62

    [31]

    Chen Z P, Wang C M, Li Y F, Su Y L, Liu D W, Li T, Zhang J C 2009 Cryo. Supercond. 37 76 (in Chinese) [陈镇平、 王春梅、 李越峰、 苏玉玲、 刘德伟、 李 涛、 张金仓 2009 低温与超导 37 76]

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  • Received Date:  27 March 2010
  • Accepted Date:  26 July 2010
  • Published Online:  05 June 2010

Effects of V substitution for Mn on charge ordering and spin-glass state in La0.45Ca0.55MnO3 sample

  • 1. (1)Department of Electronic and Electrical Engineering, Suzhou University, Suzhou 234000, China; (2)Department of Electronic and Electrical Engineering, Suzhou University, Suzhou 234000, China;Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei 230026, China

Abstract: The polycrystalline samples of La0.45Ca0.55Mn1-xVxO3(x=0.00, 0.10) have been prepared by the solid-phase reaction. Efects of V5+ substitution for Mn3+/Mn4+ on charge ordering and spin-glass state are studied by X-ray diffraction spectrum, temperature dependence of magnetization, and electron spin resonance spectra. The results indicate that charge ordering of the original system is almost destroyed, and spin-glass state at about 40 K is melted by 10% of V substitution for Mn. The charge ordering phase is destroyed mainly because of V5+ ions substitution for Mn3+/Mn4+, which increases the ratio of Mn3+ to Mn4+ and so causes ferromagnetic double-exchange to be superior to antiferromagnetic super-exchange. In addition, the spin-glass state is melted because V substitution for Mn destroys the formation condition of spin-glass state that a small quantity of ferromagnetic components exist under the antiferromagnetic backgrornd.

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