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Solidification transformation of benzene under quasi-isentropic compression

Cheng Xiao-Li Liu Fu-Sheng Li Yong-Hong Peng Xiao-Juan Zhang Ming-Jian

Solidification transformation of benzene under quasi-isentropic compression

Cheng Xiao-Li, Liu Fu-Sheng, Li Yong-Hong, Peng Xiao-Juan, Zhang Ming-Jian
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  • Kinetics of solidification of liquid benzene under high pressure has attracted much attention of scientists, and it is also one of long-standing disputes. In the present work, the gas-gun technique is combined with a recently developed measurement method of light transmittance, and the time dependence of light transmittance of liquid benzene is directly observed during successive multiply shock-compressions. The analysis shows that the transmittance decrease is caused by light scattering effects in a non-uniform optical medium, which is formed by local phase transformation of liquid-solid, and that the scattering feature reflects both the time relaxation and the spacial accumulation of transition process. The argument whether the liquid-solid phase transformation happens under multi-shock compression is clarified, and important experimental evidence is provided for the study of phase transformation Kinetics.
    • Funds:
    [1]

    Xu Z Y 1988 Principle of phase transition (Beijing: Science Press ) p1—34,412—418 (in Chinese) [徐祖耀 1988 相变原理(北京:科学出版社)第1—34,412—418页]

    [2]

    Tang Z P 2008 Shock-induced Phase Transformation (Beijing: Science Press) p88—105 (in Chinese) [唐志平 2008 冲击相变(北京:科学出版社)第88—105页]

    [3]

    Zhang S L, Liu F S, Peng X J, Zhang M J, Li Y H, Ma X J, Xue X D 2010 Acta Phys. Sin. 59 (in Chinese)[张世来、刘福生、彭小娟、张明建、李永宏、马小娟、薛学东 2010 物理学报 59]

    [4]

    Klein R M, Nourbakhsh M, Adler P M 1968 J.Mater.Sci. 3 657

    [5]

    Dick R 1970 J. Chem. Phys. 52 6021

    [6]

    Adams D M, Appleby 1977 Proc. R. Soc. London Ser. A 296 1896

    [7]

    Matsuda A, Kondo K, Nakamura K G 2004 Jpn. J. Appl. Phys. Part 243 L1614

    [8]

    Wang C, Zhang P 2010 J.Appl.Phys.107 083502

    [9]

    Maillet J B, Pineau 2008 J. Chem. Phys. 128 224502

    [10]

    Schmidt S C, Moore D S, Schiferl D, Shaner J W 1983 Phys. Rev. Lett. 50 661

    [11]

    Thiery M M, Leger J M 1988 J. Chem. Phys. 89 4255

    [12]

    Walsh J M, Rice M H 1957 J. Chem. Phys. 26 815

    [13]

    Matsuda A, Kondo K, Nakamura K G 2006 J. Chem. Phys. 124 054501

    [14]

    Root S, Gupta Y M 2007 Chem. Phys. Lett. 442 293

    [15]

    Bridgman P W 1914 Phys.Rev. 3 153

    [16]

    Akella J, Kennedy G 1971 J. Chem. Phys. 55 793

    [17]

    Cansell F, Fabre D, Petitet J 1993 J. Chem. Phys. 99 7300

    [18]

    Ciabini L, Gorelli F A, Santoro M, Bini R, Schettino V, Mezour M 2005 Phys. Rev. B 72 094108

    [19]

    Block S, Weir C E, Piermarini G J 1970 Science 169 586

    [20]

    Piermarini G J, Mighell A D, Weir C E, Block S 1969 Science 165 1250

    [21]

    Klein R M, Nourbakhsh M, Adler P M 1968 J. Mater. Sci. 3 657

    [22]

    Ciabini L, Santoro M, Bini R, Schettino V 2001 J.Chem.Phys. 115 3742

    [23]

    Wang L L, Yu T X, Li Y C 1992 Advance in Shock Dynamics (Hefei:University of Science and Technology of China Press) p117—120 (in Chinese) [王礼立、余同希、李永池 1992 冲击动力学进展(合肥:中国科学技术大学出版社)第117—120页]

    [24]

    Li Y H, Liu F S, Ma H Y, Cheng X L, Ma X J, Sun Y Y, Zhang M J, Xue X D 2010 Acta Phy.Sin. 59 2104 (in Chinese) [李永宏、刘福生、马海云、程小理、马小娟、孙燕云、张明建、薛学东 2010 物理学报 59 2104]

    [25]

    Kobayashi T, Sekine T 2000 Phys.Rev. B 62 5281

    [26]

    Jing F Q 1999 Introduction to Experimental Equation of State (Beijing: Science Press ) p204—209,352—356 (in Chinese) [经福谦 1999 实验物态方程导引(北京:科学出版社) 第204—209,352—356页]

    [27]

    Matsuda A, Nakamura K G, Kondo K 2002 Phys. Rev. B 65 17411

  • [1]

    Xu Z Y 1988 Principle of phase transition (Beijing: Science Press ) p1—34,412—418 (in Chinese) [徐祖耀 1988 相变原理(北京:科学出版社)第1—34,412—418页]

    [2]

    Tang Z P 2008 Shock-induced Phase Transformation (Beijing: Science Press) p88—105 (in Chinese) [唐志平 2008 冲击相变(北京:科学出版社)第88—105页]

    [3]

    Zhang S L, Liu F S, Peng X J, Zhang M J, Li Y H, Ma X J, Xue X D 2010 Acta Phys. Sin. 59 (in Chinese)[张世来、刘福生、彭小娟、张明建、李永宏、马小娟、薛学东 2010 物理学报 59]

    [4]

    Klein R M, Nourbakhsh M, Adler P M 1968 J.Mater.Sci. 3 657

    [5]

    Dick R 1970 J. Chem. Phys. 52 6021

    [6]

    Adams D M, Appleby 1977 Proc. R. Soc. London Ser. A 296 1896

    [7]

    Matsuda A, Kondo K, Nakamura K G 2004 Jpn. J. Appl. Phys. Part 243 L1614

    [8]

    Wang C, Zhang P 2010 J.Appl.Phys.107 083502

    [9]

    Maillet J B, Pineau 2008 J. Chem. Phys. 128 224502

    [10]

    Schmidt S C, Moore D S, Schiferl D, Shaner J W 1983 Phys. Rev. Lett. 50 661

    [11]

    Thiery M M, Leger J M 1988 J. Chem. Phys. 89 4255

    [12]

    Walsh J M, Rice M H 1957 J. Chem. Phys. 26 815

    [13]

    Matsuda A, Kondo K, Nakamura K G 2006 J. Chem. Phys. 124 054501

    [14]

    Root S, Gupta Y M 2007 Chem. Phys. Lett. 442 293

    [15]

    Bridgman P W 1914 Phys.Rev. 3 153

    [16]

    Akella J, Kennedy G 1971 J. Chem. Phys. 55 793

    [17]

    Cansell F, Fabre D, Petitet J 1993 J. Chem. Phys. 99 7300

    [18]

    Ciabini L, Gorelli F A, Santoro M, Bini R, Schettino V, Mezour M 2005 Phys. Rev. B 72 094108

    [19]

    Block S, Weir C E, Piermarini G J 1970 Science 169 586

    [20]

    Piermarini G J, Mighell A D, Weir C E, Block S 1969 Science 165 1250

    [21]

    Klein R M, Nourbakhsh M, Adler P M 1968 J. Mater. Sci. 3 657

    [22]

    Ciabini L, Santoro M, Bini R, Schettino V 2001 J.Chem.Phys. 115 3742

    [23]

    Wang L L, Yu T X, Li Y C 1992 Advance in Shock Dynamics (Hefei:University of Science and Technology of China Press) p117—120 (in Chinese) [王礼立、余同希、李永池 1992 冲击动力学进展(合肥:中国科学技术大学出版社)第117—120页]

    [24]

    Li Y H, Liu F S, Ma H Y, Cheng X L, Ma X J, Sun Y Y, Zhang M J, Xue X D 2010 Acta Phy.Sin. 59 2104 (in Chinese) [李永宏、刘福生、马海云、程小理、马小娟、孙燕云、张明建、薛学东 2010 物理学报 59 2104]

    [25]

    Kobayashi T, Sekine T 2000 Phys.Rev. B 62 5281

    [26]

    Jing F Q 1999 Introduction to Experimental Equation of State (Beijing: Science Press ) p204—209,352—356 (in Chinese) [经福谦 1999 实验物态方程导引(北京:科学出版社) 第204—209,352—356页]

    [27]

    Matsuda A, Nakamura K G, Kondo K 2002 Phys. Rev. B 65 17411

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  • Received Date:  19 August 2010
  • Accepted Date:  20 December 2010
  • Published Online:  15 September 2011

Solidification transformation of benzene under quasi-isentropic compression

  • 1. Laboratory of High Pressure Physics, Southwest Jiaotong University, Chengdu 610031, China

Abstract: Kinetics of solidification of liquid benzene under high pressure has attracted much attention of scientists, and it is also one of long-standing disputes. In the present work, the gas-gun technique is combined with a recently developed measurement method of light transmittance, and the time dependence of light transmittance of liquid benzene is directly observed during successive multiply shock-compressions. The analysis shows that the transmittance decrease is caused by light scattering effects in a non-uniform optical medium, which is formed by local phase transformation of liquid-solid, and that the scattering feature reflects both the time relaxation and the spacial accumulation of transition process. The argument whether the liquid-solid phase transformation happens under multi-shock compression is clarified, and important experimental evidence is provided for the study of phase transformation Kinetics.

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