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A THEORETICAL MODEL OF VIBRATIONAL PREDISSOCIA-TION VIA INTERMEDIATE STATE COUPLING

XIANG TIAN-XIANG

A THEORETICAL MODEL OF VIBRATIONAL PREDISSOCIA-TION VIA INTERMEDIATE STATE COUPLING

XIANG TIAN-XIANG
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  • Received Date:  29 April 1989
  • Published Online:  22 June 2005

A THEORETICAL MODEL OF VIBRATIONAL PREDISSOCIA-TION VIA INTERMEDIATE STATE COUPLING

  • 1. 南京大学化学系化学物理实验室,南京,210008

Abstract: In this paper, a theoretical model for vibrational predissociation (VP) of molecular clusters via intermediate states is proposed. It is shown that molecular intermediate states play an important role in inducing VP processes of molecular clusters. Based on this theory, a statistical dynamics model is established to describe and interpret qualitatively and semiquantatively the experimental line-broadening effects in various molecular clusters. Finally, we discuss the effects of a variety of coupling mechanisms on the energetic structures and the state relaxation processes in molecular clusters.

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