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Intercomparison of slant column measurements of NO2 by ground-based MAX-DOAS

Wang Ting Wang Pu-Cai Yu Huan Zhang Xing-Ying Zhou Bin Si Fu-Qi Wang Shan-Shan Bai Wen-Guang Zhou Hai-Jin Zhao Heng

Intercomparison of slant column measurements of NO2 by ground-based MAX-DOAS

Wang Ting, Wang Pu-Cai, Yu Huan, Zhang Xing-Ying, Zhou Bin, Si Fu-Qi, Wang Shan-Shan, Bai Wen-Guang, Zhou Hai-Jin, Zhao Heng
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  • In September 2011, we used 3 ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) instruments of different designs and operation protocols to measure tropospheric NO2 for about 20 days, at the Station of Atmospheric Comprehensive Observatory, Institute of Atmospheric Physics, Chinese Academy of Sciences (Xianghe 117.0N, 39.77E). All instruments are oriented to an azimuth angle of 270 (north), in a common wavelength range and with a set of cross sections for the inversion of NO2 slant column in visible and UV wavelength range respectively. Intercomparison of NO2 slant columns among three MAX-DOAS is introduced. The results obtained from the different instruments are in good accordance with each other, and the correlation coefficients are all higher than 0.95, but systematical errors exist. Daily average errors of three MAX-DOAS instruments are almost below 6%, showing that the instruments work steadily and the data are cogent. The UV results are smaller than those in the visible range, especially on the overcast days, related to the wavelength dependence of Rayleigh and Mie scattering. After the correction of systematical errors, there is better consistency among different results, which indicates that the three MAX-DOAS instruments have a capability to validate the atmospheric component products of satellite.
    • Funds: Project supported by the Special Scientific Research Fund of Meteorological Public Welfare Profession of China (Grant No. GYHY201106045-52), the National Natural Science Foundation of China (Grant Nos. 41175030, 40975076), and the Strategic Priority Research Program - Climate Change: Carbon Budget and Relevant Issues of the Chinese Academy of Sciences (Grant No. XDA05000000).
    [1]

    Zhou B, Liu W Q, Qi F, Li Z B, Chui Y J 2001 Acta Phys. Sin. 50 1818 (in Chinese) [周斌, 刘文清, 齐峰, 李振壁, 崔延军 2001 物理学报 50 1818]

    [2]

    Si F Q, Liu J G, Xie P H, Zhang Y J, Dou K, Liu W Q 2006 Acta Phys. Sin. 55 3165 (in Chinese) [司福祺, 刘建国, 谢品华, 张玉钧, 窦科, 刘文清 2006 物理学报 55 3165]

    [3]

    Platt U, Stutz J 2008 Differential optical absorption spectroscopy: Principles and applications (1st Edn.) (Heidelberg: Springer Verlag) pp135-160

    [4]

    Roscoe H K, Roozendael M, Fayt C, Piesanie A, Abuhassan N, Adams C, Akrami M, Cede A, Chong J, Clemer K, Friess U, Ojeda M G, Goutail F, Graves R, Griesfeller A, Grossmann K, Hemerijckx G, Hendrick F, Herman J, Hermans C, Irie H, Johnston P V, Kanaya Y, Kreher K, Leigh R, Merlaud A, Mount G H, Navarro M, Oetjen H, Pazmino A, Perez C M, Peters E, Pinardi G, Puentedura O, Richter A, Schonhardt A, Shaiganfar R, Spinei E, Strong K, Takashima H, Vlemmix T, Vrekoussis M, Wagner T, Wittrock F, Yela M, Yilmaz S, Boersma F, Hains J, Kroon M, Piters A, Kim Y J 2010 Atmos. Meas. Tech. 3 1629

    [5]

    Noxon J 1975 Science 189 547

    [6]

    Hönninger G, Friedeburg C V, Platt U 2004 Atmos. Chem. Phys. 4 231

    [7]

    Friedeburg C V, Pundt I, Mettendorf K U, Wagner T, Platt U 2005 Atmos. Environ. 39 977

    [8]

    Wittrock F, Clémer K, Berkhout S, Boersma F, Brunner D, Friess U, Hay T, Irie H, Peters E, Piters A, Shaiganfar R, Sluis W, Spinei E, Vlemmix T, Wagner T, Yilmaz S, Roozendael M, Richter A, Burrows J P 2010 American Geophysical Union Fall Meeting San Francisco, USA, December 13-17, 2010 p219

    [9]

    Irie H, Takashima H, Kanaya Y, Boersma K, Gast L, Wittrock F, Brunner D, Zhou Y, Roozendael M 2011 Atmos. Meas. Tech. 4 1027

    [10]

    Takashima H, Irie H, Kanaya Y, Syamsudin F 2012 Atmos. Meas. Tech. 5 2351

    [11]

    Frins E, Osorio M, Casaballe N, Belsterli G, Wagner T, Platt U 2012 Atmos. Meas. Tech. 5 1165

    [12]

    Si F Q, Xie P H, Heue K P, Liu C, Peng F M, Liu W Q 2008 Acta Phys. Sin. 57 6018 (in Chinese) [司福祺, 谢品华, Klaus-Peter Heue, 刘诚, 彭夫敏, 刘文清 2008 物理学报 57 6018]

    [13]

    Xu J, Xie P H, Si F Q, Dou K, Li A, Liu Y, Liu W Q 2010 Spectrosc. Spect. Anal. 30 2464 (in Chinese) [徐晋, 谢品华, 司福祺, 窦科, 李昂, 刘宇, 刘文清 2010 光谱学与光谱分析 30 2464]

    [14]

    Yang S N, Wang S S, Wang Z R, Zhou B 2011 J. Fudan Univ. Nat. Sci. 50 199 (in Chinese) [杨素娜, 王珊珊, 王焯如, 周斌 2011 复旦学报(自然科学版) 50 199]

    [15]

    Wang Y, Li A, Xie P H, Zeng Y, Wang R B, Chen H, Pei X, Liu J G, Liu W Q 2012 Chin. Phys. B 21 114211

    [16]

    Xu J, Xie P H, Si F Q, Li A, Liu W Q 2012 Acta Phys. Sin. 61 024204 (in Chinese) [徐晋, 谢品华, 司福祺, 李昂, 刘文清 2012 物理学报 61 024204]

    [17]

    Wang S, Zhou B, Wang Z, Yang S, Hao N, Valks P, Trautmann T, Chen L 2012 J. Geophys. Res. 117 D13305

    [18]

    Hofmann D, Bonasoni P, Maziere M D, Evangelisti F, Giovanelli G, Goldman A, Goutail F, Harder J, Jakoubek R, Johnston P, Kerr J, Matthews W A, McElroy T, McKenzie R, Mount G, Platt U, Pommereau J P, Sarkissian A, Simon P, Solomon S, Stutz J, Thomas A, Roozendael M, Wu E 1995 J. Geophys. Res. 100 16765

    [19]

    Vandaele A, Hermans C, Simon P, Roozendael M, Guilmot J, Carleer M, Colin R 1996 J. Atmos. Chem. 25 289

    [20]

    Bogumil K, Orphal J, Homann T, Voigt S, Spietz P, Fleischmann O C, Vogel A, Hartmann M, Bovensmann H, Frerick J, Burrows J P 2003 J. Photochem. Photobiol A 159 167

    [21]

    Rothman L, Barbe A, Chris D, Hitran T 2003 J. Quant. Spectrosc. Radiat. Transfer 82 5

    [22]

    Fleischmann O, Hartmann M, Burrows J P, Orphal J 2004 J. Photochem. Photobiol A 168 117

    [23]

    Meller R, Moortgat G 2000 J. Geophys. Res. 105 7089

    [24]

    Chance K, Spurr R 1997 Appl. Opt. 36 5224

    [25]

    Clémer K, Roozendael M, Fayt C, Hendrick F, Hermans C, Pinardi G, Spurr R, Wang P, Maziére M 2010 Atmos. Meas. Tech. 3 863

    [26]

    Yu H 2011 Ph. D. Dissertation (Beijing: Institute of Atmospheric Physics, Chinese Academy of Sciences) (in Chinese) [余环 2011 博士学位论文 (北京: 中国科学院大气物理研究所)

    [27]

    Si F Q, Xie P H, Dou K, Zhan K, Liu Y, Xu J, Liu W Q 2010 Acta Phys. Sin. 59 2867 (in Chinese) [司福祺, 谢品华, 窦科, 詹铠, 刘宇, 徐晋, 刘文清 2010 物理学报 59 2867]

  • [1]

    Zhou B, Liu W Q, Qi F, Li Z B, Chui Y J 2001 Acta Phys. Sin. 50 1818 (in Chinese) [周斌, 刘文清, 齐峰, 李振壁, 崔延军 2001 物理学报 50 1818]

    [2]

    Si F Q, Liu J G, Xie P H, Zhang Y J, Dou K, Liu W Q 2006 Acta Phys. Sin. 55 3165 (in Chinese) [司福祺, 刘建国, 谢品华, 张玉钧, 窦科, 刘文清 2006 物理学报 55 3165]

    [3]

    Platt U, Stutz J 2008 Differential optical absorption spectroscopy: Principles and applications (1st Edn.) (Heidelberg: Springer Verlag) pp135-160

    [4]

    Roscoe H K, Roozendael M, Fayt C, Piesanie A, Abuhassan N, Adams C, Akrami M, Cede A, Chong J, Clemer K, Friess U, Ojeda M G, Goutail F, Graves R, Griesfeller A, Grossmann K, Hemerijckx G, Hendrick F, Herman J, Hermans C, Irie H, Johnston P V, Kanaya Y, Kreher K, Leigh R, Merlaud A, Mount G H, Navarro M, Oetjen H, Pazmino A, Perez C M, Peters E, Pinardi G, Puentedura O, Richter A, Schonhardt A, Shaiganfar R, Spinei E, Strong K, Takashima H, Vlemmix T, Vrekoussis M, Wagner T, Wittrock F, Yela M, Yilmaz S, Boersma F, Hains J, Kroon M, Piters A, Kim Y J 2010 Atmos. Meas. Tech. 3 1629

    [5]

    Noxon J 1975 Science 189 547

    [6]

    Hönninger G, Friedeburg C V, Platt U 2004 Atmos. Chem. Phys. 4 231

    [7]

    Friedeburg C V, Pundt I, Mettendorf K U, Wagner T, Platt U 2005 Atmos. Environ. 39 977

    [8]

    Wittrock F, Clémer K, Berkhout S, Boersma F, Brunner D, Friess U, Hay T, Irie H, Peters E, Piters A, Shaiganfar R, Sluis W, Spinei E, Vlemmix T, Wagner T, Yilmaz S, Roozendael M, Richter A, Burrows J P 2010 American Geophysical Union Fall Meeting San Francisco, USA, December 13-17, 2010 p219

    [9]

    Irie H, Takashima H, Kanaya Y, Boersma K, Gast L, Wittrock F, Brunner D, Zhou Y, Roozendael M 2011 Atmos. Meas. Tech. 4 1027

    [10]

    Takashima H, Irie H, Kanaya Y, Syamsudin F 2012 Atmos. Meas. Tech. 5 2351

    [11]

    Frins E, Osorio M, Casaballe N, Belsterli G, Wagner T, Platt U 2012 Atmos. Meas. Tech. 5 1165

    [12]

    Si F Q, Xie P H, Heue K P, Liu C, Peng F M, Liu W Q 2008 Acta Phys. Sin. 57 6018 (in Chinese) [司福祺, 谢品华, Klaus-Peter Heue, 刘诚, 彭夫敏, 刘文清 2008 物理学报 57 6018]

    [13]

    Xu J, Xie P H, Si F Q, Dou K, Li A, Liu Y, Liu W Q 2010 Spectrosc. Spect. Anal. 30 2464 (in Chinese) [徐晋, 谢品华, 司福祺, 窦科, 李昂, 刘宇, 刘文清 2010 光谱学与光谱分析 30 2464]

    [14]

    Yang S N, Wang S S, Wang Z R, Zhou B 2011 J. Fudan Univ. Nat. Sci. 50 199 (in Chinese) [杨素娜, 王珊珊, 王焯如, 周斌 2011 复旦学报(自然科学版) 50 199]

    [15]

    Wang Y, Li A, Xie P H, Zeng Y, Wang R B, Chen H, Pei X, Liu J G, Liu W Q 2012 Chin. Phys. B 21 114211

    [16]

    Xu J, Xie P H, Si F Q, Li A, Liu W Q 2012 Acta Phys. Sin. 61 024204 (in Chinese) [徐晋, 谢品华, 司福祺, 李昂, 刘文清 2012 物理学报 61 024204]

    [17]

    Wang S, Zhou B, Wang Z, Yang S, Hao N, Valks P, Trautmann T, Chen L 2012 J. Geophys. Res. 117 D13305

    [18]

    Hofmann D, Bonasoni P, Maziere M D, Evangelisti F, Giovanelli G, Goldman A, Goutail F, Harder J, Jakoubek R, Johnston P, Kerr J, Matthews W A, McElroy T, McKenzie R, Mount G, Platt U, Pommereau J P, Sarkissian A, Simon P, Solomon S, Stutz J, Thomas A, Roozendael M, Wu E 1995 J. Geophys. Res. 100 16765

    [19]

    Vandaele A, Hermans C, Simon P, Roozendael M, Guilmot J, Carleer M, Colin R 1996 J. Atmos. Chem. 25 289

    [20]

    Bogumil K, Orphal J, Homann T, Voigt S, Spietz P, Fleischmann O C, Vogel A, Hartmann M, Bovensmann H, Frerick J, Burrows J P 2003 J. Photochem. Photobiol A 159 167

    [21]

    Rothman L, Barbe A, Chris D, Hitran T 2003 J. Quant. Spectrosc. Radiat. Transfer 82 5

    [22]

    Fleischmann O, Hartmann M, Burrows J P, Orphal J 2004 J. Photochem. Photobiol A 168 117

    [23]

    Meller R, Moortgat G 2000 J. Geophys. Res. 105 7089

    [24]

    Chance K, Spurr R 1997 Appl. Opt. 36 5224

    [25]

    Clémer K, Roozendael M, Fayt C, Hendrick F, Hermans C, Pinardi G, Spurr R, Wang P, Maziére M 2010 Atmos. Meas. Tech. 3 863

    [26]

    Yu H 2011 Ph. D. Dissertation (Beijing: Institute of Atmospheric Physics, Chinese Academy of Sciences) (in Chinese) [余环 2011 博士学位论文 (北京: 中国科学院大气物理研究所)

    [27]

    Si F Q, Xie P H, Dou K, Zhan K, Liu Y, Xu J, Liu W Q 2010 Acta Phys. Sin. 59 2867 (in Chinese) [司福祺, 谢品华, 窦科, 詹铠, 刘宇, 徐晋, 刘文清 2010 物理学报 59 2867]

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  • Received Date:  14 September 2012
  • Accepted Date:  12 October 2012
  • Published Online:  05 March 2013

Intercomparison of slant column measurements of NO2 by ground-based MAX-DOAS

  • 1. Key Laboratory of Middle Atmosphere and Global Environment Observation, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China;
  • 2. University of Chinese Academy of Sciences, Beijing 100049, China;
  • 3. National Satellite Meteorological Center, China Meteorological Administration, Beijing 100081, China;
  • 4. Department of Environmental Science and Engineering, Fudan University, Shanghai 200433, China;
  • 5. Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China
Fund Project:  Project supported by the Special Scientific Research Fund of Meteorological Public Welfare Profession of China (Grant No. GYHY201106045-52), the National Natural Science Foundation of China (Grant Nos. 41175030, 40975076), and the Strategic Priority Research Program - Climate Change: Carbon Budget and Relevant Issues of the Chinese Academy of Sciences (Grant No. XDA05000000).

Abstract: In September 2011, we used 3 ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) instruments of different designs and operation protocols to measure tropospheric NO2 for about 20 days, at the Station of Atmospheric Comprehensive Observatory, Institute of Atmospheric Physics, Chinese Academy of Sciences (Xianghe 117.0N, 39.77E). All instruments are oriented to an azimuth angle of 270 (north), in a common wavelength range and with a set of cross sections for the inversion of NO2 slant column in visible and UV wavelength range respectively. Intercomparison of NO2 slant columns among three MAX-DOAS is introduced. The results obtained from the different instruments are in good accordance with each other, and the correlation coefficients are all higher than 0.95, but systematical errors exist. Daily average errors of three MAX-DOAS instruments are almost below 6%, showing that the instruments work steadily and the data are cogent. The UV results are smaller than those in the visible range, especially on the overcast days, related to the wavelength dependence of Rayleigh and Mie scattering. After the correction of systematical errors, there is better consistency among different results, which indicates that the three MAX-DOAS instruments have a capability to validate the atmospheric component products of satellite.

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