Search

Article

x

留言板

尊敬的读者、作者、审稿人, 关于本刊的投稿、审稿、编辑和出版的任何问题, 您可以本页添加留言。我们将尽快给您答复。谢谢您的支持!

姓名
邮箱
手机号码
标题
留言内容
验证码

Dielectric properties and nonlinear current-voltage behavior of MgTiO3-doped CaCu3Ti4O12 ceramics

Cao Lei Liu Peng Zhou Jian-Ping Wang Ya-Juan Su Li-Na Liu Cheng

Citation:

Dielectric properties and nonlinear current-voltage behavior of MgTiO3-doped CaCu3Ti4O12 ceramics

Cao Lei, Liu Peng, Zhou Jian-Ping, Wang Ya-Juan, Su Li-Na, Liu Cheng
PDF
Get Citation

(PLEASE TRANSLATE TO ENGLISH

BY GOOGLE TRANSLATE IF NEEDED.)

  • The CaCu3Ti4O12-xMgTiO3(x= 0, 0.25, 0.5, 1.0) ceramics have been prepared by a solid-state reaction method. The effects of MgTiO3 doping on the phase structure, microstructure and dielectric properties of CaCu3Ti4O12 ceramics have been investigated. The results indicate that MgTiO3 doping not only reduced the dielectric loss of low frequency range and raised the breakdown voltage but also significantly improved the I-V nonlinearity coefficient. The optimized properties of MgTiO3 doped CaCu3Ti4O12 can be well explained by the uniformity of the grains, the reduction of the average grain boundary thinkness and the enhancement of the grain boundary resistance. Among the CaCu3Ti4O12-MgTiO3 specimens in this work, the CaCu3Ti4O12-0.5MgTiO3 specimen has achieved the best comprehensive properties, which include a dielectric constant (εr) of 53958, dielectric loss (tanδ) of 0.06 at 1 kHz, breakdown voltage (Eb) of 295 V/mm and a large nonlinearity coefficient of 66.3.
    [1]

    Homes C C, Vogt T, Shapiro S M, Wakimoto S, Ramirez A P 2001 Science 293 673

    [2]

    Subramanian M A, Li D, Duan N, Reisner B A, Sleight A W 2000 J. Solid State Chem. 151 323

    [3]

    Ramirez A P, Subramanian M A, Gardel M, Blumberg G, Li D, Vogt T, Shapiro S M 2000 Solid State Commun. 115 217

    [4]

    Chung S Y, Kim I D, Kang S J L 2004 Nature Mater. 3 774

    [5]

    Zhao Y L, Jiao Z K, Cao G H 2003 Acta Phys. Sin. 52 1500 (in Chinese) [赵彦立、焦正宽、曹光旱 2003 物理学报 52 1500]

    [6]

    Zhou X L, Du P Y 2005 Acta Phys. Sin. 54 354 (in Chinese) [周小莉、杜丕一 2005 物理学报 54 354]

    [7]

    Shao S F, Zheng P, Zhang J L, Niu X K, Wang C L, Zhong W L 2006 Acta Phys. Sin. 55 6661 (in Chinese) [邵守福、郑 鹏、张家良、钮效鹍、王春雷、钟维烈 2006 物理学报 55 6661]

    [8]

    Marques V P B, Ries A, Sim es A Z, Ramírez M A, Varela J A, Longo E 2007 Ceramics International 33 1187

    [9]

    Singh D P, Mohapatra Y N, Agrawal D C Mater. 2009 Mater. Sci. Eng. B 157 58

    [10]

    Fang L, Shen M R, Li Z Y 2006 J. Appl. Phys. 100 104101

    [11]

    Li T, Chen Z P, Chang F G, Hao J H, Zhang J C 2009 J. Alloy Compd. 484 718

    [12]

    Lin Y H, Cai J N, Li M, Nan C W 2006 Appl. Phys. Lett. 88 172902

    [13]

    Luo F C, He J L, Hu J, Lin Y H 2009 J. Appl. Phys. 105 076104

    [14]

    Cai J N, Lin Y H, Cheng B, Nan C W, He J L, Wu Y J, Chen X M 2007 Appl. Phys. Lett. 91 252905

    [15]

    Xue H, Guan X F, Yu R, Xiong Z X 2009 J. Alloy Compd. 482 L14

    [16]

    Chung S Y, Lee S I, Choi J H, Chio S Y 2006 Appl. Phys. Lett. 89 191907

    [17]

    Chung S Y, Choi S Y, Yamamoto T, Ikuhara Y, Kang S J L 2006 Appl. Phys. Lett. 88 091917

    [18]

    Leret P, Fernandez J F, Frutos J D, Hevia D F 2007 J. Eur. Ceram. Soc. 27 3901

    [19]

    Clarke D R 1999 J. Am. Ceram. Soc. 82 485

    [20]

    Ji S D, Fan F K 1997 J. Ceram. 18 52 (in Chinese) [纪士东、范福康 1997 陶瓷学报 18 52]

    [21]

    Liu P, He Y, Li J, Zhu G Q, Bian X B 2007 Acta Phys. Sin. 56 5489 (in Chinese) [刘 鹏、贺 颖、李 俊、朱刚强、边小兵 2007 物理学报 56 5489]

    [22]

    Mu C H, Liu P, He Y, Zhang D, Meng L, Bian X B 2008 Acta Phys. Sin. 57 2432 (in Chinese) [慕春红、刘 鹏、贺 颖、张 丹、孟 玲、边小兵 2008 物理学报 57 2432]

    [23]

    Shannon R D 1976 Acta Cryst. A 32 751

    [24]

    Wang J F, Luo J H 2007 B. Chinese Ceram. Soc. 26 514 (in Chinese) [王加芳、罗驹华 2007 硅酸盐通报 26 514]

    [25]

    Fang T T, Mei L T 2007 J. Am. Ceram. Soc. 90 638

    [26]

    Prakash B S, Varma K B R 2007 J. Phys. Chem. Solids 68 490

    [27]

    New Inorganic Material Teaching and Research Group of Shanghai Science and Technology University 1977 The Electronic Ceramics Processing Basics (Shanghai: Shanghai People Press) p111 (in Chinese) [上海科技大学新型无机材料教研组 1977 电子陶瓷工艺基础 (上海:上海人民出版社) 第111页]

    [28]

    Yan Y Y, Jin L, Feng L X, Cao G H 2006 Sci. Eng. B 130 146

  • [1]

    Homes C C, Vogt T, Shapiro S M, Wakimoto S, Ramirez A P 2001 Science 293 673

    [2]

    Subramanian M A, Li D, Duan N, Reisner B A, Sleight A W 2000 J. Solid State Chem. 151 323

    [3]

    Ramirez A P, Subramanian M A, Gardel M, Blumberg G, Li D, Vogt T, Shapiro S M 2000 Solid State Commun. 115 217

    [4]

    Chung S Y, Kim I D, Kang S J L 2004 Nature Mater. 3 774

    [5]

    Zhao Y L, Jiao Z K, Cao G H 2003 Acta Phys. Sin. 52 1500 (in Chinese) [赵彦立、焦正宽、曹光旱 2003 物理学报 52 1500]

    [6]

    Zhou X L, Du P Y 2005 Acta Phys. Sin. 54 354 (in Chinese) [周小莉、杜丕一 2005 物理学报 54 354]

    [7]

    Shao S F, Zheng P, Zhang J L, Niu X K, Wang C L, Zhong W L 2006 Acta Phys. Sin. 55 6661 (in Chinese) [邵守福、郑 鹏、张家良、钮效鹍、王春雷、钟维烈 2006 物理学报 55 6661]

    [8]

    Marques V P B, Ries A, Sim es A Z, Ramírez M A, Varela J A, Longo E 2007 Ceramics International 33 1187

    [9]

    Singh D P, Mohapatra Y N, Agrawal D C Mater. 2009 Mater. Sci. Eng. B 157 58

    [10]

    Fang L, Shen M R, Li Z Y 2006 J. Appl. Phys. 100 104101

    [11]

    Li T, Chen Z P, Chang F G, Hao J H, Zhang J C 2009 J. Alloy Compd. 484 718

    [12]

    Lin Y H, Cai J N, Li M, Nan C W 2006 Appl. Phys. Lett. 88 172902

    [13]

    Luo F C, He J L, Hu J, Lin Y H 2009 J. Appl. Phys. 105 076104

    [14]

    Cai J N, Lin Y H, Cheng B, Nan C W, He J L, Wu Y J, Chen X M 2007 Appl. Phys. Lett. 91 252905

    [15]

    Xue H, Guan X F, Yu R, Xiong Z X 2009 J. Alloy Compd. 482 L14

    [16]

    Chung S Y, Lee S I, Choi J H, Chio S Y 2006 Appl. Phys. Lett. 89 191907

    [17]

    Chung S Y, Choi S Y, Yamamoto T, Ikuhara Y, Kang S J L 2006 Appl. Phys. Lett. 88 091917

    [18]

    Leret P, Fernandez J F, Frutos J D, Hevia D F 2007 J. Eur. Ceram. Soc. 27 3901

    [19]

    Clarke D R 1999 J. Am. Ceram. Soc. 82 485

    [20]

    Ji S D, Fan F K 1997 J. Ceram. 18 52 (in Chinese) [纪士东、范福康 1997 陶瓷学报 18 52]

    [21]

    Liu P, He Y, Li J, Zhu G Q, Bian X B 2007 Acta Phys. Sin. 56 5489 (in Chinese) [刘 鹏、贺 颖、李 俊、朱刚强、边小兵 2007 物理学报 56 5489]

    [22]

    Mu C H, Liu P, He Y, Zhang D, Meng L, Bian X B 2008 Acta Phys. Sin. 57 2432 (in Chinese) [慕春红、刘 鹏、贺 颖、张 丹、孟 玲、边小兵 2008 物理学报 57 2432]

    [23]

    Shannon R D 1976 Acta Cryst. A 32 751

    [24]

    Wang J F, Luo J H 2007 B. Chinese Ceram. Soc. 26 514 (in Chinese) [王加芳、罗驹华 2007 硅酸盐通报 26 514]

    [25]

    Fang T T, Mei L T 2007 J. Am. Ceram. Soc. 90 638

    [26]

    Prakash B S, Varma K B R 2007 J. Phys. Chem. Solids 68 490

    [27]

    New Inorganic Material Teaching and Research Group of Shanghai Science and Technology University 1977 The Electronic Ceramics Processing Basics (Shanghai: Shanghai People Press) p111 (in Chinese) [上海科技大学新型无机材料教研组 1977 电子陶瓷工艺基础 (上海:上海人民出版社) 第111页]

    [28]

    Yan Y Y, Jin L, Feng L X, Cao G H 2006 Sci. Eng. B 130 146

  • [1] Li Shi-Jia, Wang Zhen-Xing, Niu Yan, Wang Bin, Sang Sheng-Bo, Zhang Wen-Dong, Gao Yang, Ji Jian-Long. I-V characteristics and voltage dependence of pH-sensitive organic electrochemical transistors. Acta Physica Sinica, 2022, 71(13): 138501. doi: 10.7498/aps.71.20220241
    [2] Guo Qi-Qi, Chen Yi-Hang. Enhanced nonlinear optical effects based on strong coupling between epsilon-near-zero mode and gap surface plasmons. Acta Physica Sinica, 2021, 70(18): 187303. doi: 10.7498/aps.70.20210290
    [3] Cheng Peng-Fei, Li Sheng-Tao, Li Jian-Ying. Dielectric spectra of ZnO varistor ceramics. Acta Physica Sinica, 2012, 61(18): 187302. doi: 10.7498/aps.61.187302
    [4] Jia Ran, Gu Fang, Wu Zhen-Hua, Zhao Xue-Tong, Li Jian-Ying. Dielectric properties of CaCu3Ti4O12 ceramics prepared by a simplified coprecipitation method. Acta Physica Sinica, 2012, 61(20): 207701. doi: 10.7498/aps.61.207701
    [5] Zhao Xue-Tong, Li Jian-Ying, Li Xuan, Li Sheng-Tao. Characterization of defects and research on impulse aging in ZnO varistor ceramics. Acta Physica Sinica, 2012, 61(15): 153103. doi: 10.7498/aps.61.153103
    [6] Yang Chang-Ping, Li Min-Yi, Song Xue-Ping, Xiao Hai-Bo, Xu Ling-Fang. Effect of oxygen content on giant dielectric constant and dielectric process in CaCu3Ti4O12. Acta Physica Sinica, 2012, 61(19): 197702. doi: 10.7498/aps.61.197702
    [7] Deng Heng, Yang Chang-Ping, Huang Chang, Xu Ling-Fang. Magnetically correlated I-V nonlinearity and electrical transport property of the double-layered perovskite La1.8Ca1.2Mn2O7 compound. Acta Physica Sinica, 2010, 59(10): 7390-7395. doi: 10.7498/aps.59.7390
    [8] Luo Xiao-Jing, Yang Chang-Ping, Song Xue-Ping, Xu Ling-Fang. Dielectric and impedance performances of giant dielectric constant oxide CaCu3Ti4O12. Acta Physica Sinica, 2010, 59(5): 3516-3522. doi: 10.7498/aps.59.3516
    [9] Yin Gui-Lai, Li Jian-Ying, Yao Guang, Cheng Peng-Fei, Li Sheng-Tao. Research on electronic process of impulse degradation of ZnO-based ceramics. Acta Physica Sinica, 2010, 59(9): 6345-6350. doi: 10.7498/aps.59.6345
    [10] Mu Chun-Hong, Liu Peng, He Ying, Zhang Dan, Meng Ling, Bian Xiao-Bing. Study on the dielectric properties and dielectric relaxation of Fe-doped CaCu3Ti4O12 ceramics. Acta Physica Sinica, 2008, 57(4): 2432-2437. doi: 10.7498/aps.57.2432
    [11] Liu Peng, He Ying, Li Jun, Zhu Gang-Qiang, Bian Xiao-Bing. Influence of Nb doping on the dielectric properties of CaCu3Ti4O12 ceramics. Acta Physica Sinica, 2007, 56(9): 5489-5493. doi: 10.7498/aps.56.5489
    [12] Yang Xue-Wen, Zheng Jia-Gui, Zhang Jing-Quan, Feng Liang-Huan, Cai Wei, Cai Ya-Ping, Li Wei, Li Bing, Lei Zhi, Wu Li-Li. Characteristics of CdTe solar cell device. Acta Physica Sinica, 2006, 55(5): 2504-2507. doi: 10.7498/aps.55.2504
    [13] Liang Rui-Hong, Dong Xian-Lin, Chen Ying, Cao Fei, Wang Yong-Ling. Mechanism of nonlinear dielectric constant of BaTiO3-based ceramics under high DC electric field. Acta Physica Sinica, 2005, 54(10): 4914-4919. doi: 10.7498/aps.54.4914
    [14] Shen Han, Xu Hua, Chen Min, Li Jing-De. Non-ferroelectric single crystal of ultra-high dielectric constant. Acta Physica Sinica, 2004, 53(5): 1529-1533. doi: 10.7498/aps.53.1529
    [15] Liu Xue-Rong, Hu Bo, Liu Wen-Han, Gao Chen. The theoretical calibration coefficient in the measurement of nonlinear dielectric constant with a scanning tip microwave near-field microscopy. Acta Physica Sinica, 2003, 52(1): 34-38. doi: 10.7498/aps.52.34
    [16] Zhao Yan-Li, Jiao Zheng-Kuan, Gao Guang-Han. High dielectric constant in CaCu3Ti4O12 bulk an d thin films. Acta Physica Sinica, 2003, 52(6): 1500-1504. doi: 10.7498/aps.52.1500
    [17] LIU ZENG-RONG, JIANG XIA-MEI, HUN ZHI-BIN, GU GUO-QING. THE SUB-STEPS OF I-V CHARACTERISTICS IN JOSEPHSON JUNCTION. Acta Physica Sinica, 1990, 39(5): 823-829. doi: 10.7498/aps.39.823
    [18] QIAN MIN, PAN TAO, LIU ZHENG-RONG. THEORETIC ANALYSIS OF I-V CHARACTERISTICS IN JOSEPHSON JUNCTION. Acta Physica Sinica, 1987, 36(2): 149-156. doi: 10.7498/aps.36.149
    [19] SHI LONG-PEI, LIAO SHAO-BIN. MEASUREMENT OF THE DIELECTRIC CONSTANTS AND THE PERMEABILITIES OF MICROWAVE FERRITES. Acta Physica Sinica, 1974, 23(3): 61-72. doi: 10.7498/aps.23.61
    [20] SUN CHIA-CHUNG, CHIANG TUNG-CHEN, CHOU MO-YI, SHI AN-TON. THE CONTRIBUTION OF THE ELECTRONIC POLARIZATION TO THE ELASTIC AND PIEZOELECTRIC CONSTANTS AND THE DIELECTRIC TENSOR FOR THE CALCIUM FLUORIDE CRYSTAL. Acta Physica Sinica, 1965, 21(2): 402-413. doi: 10.7498/aps.21.402
Metrics
  • Abstract views:  11610
  • PDF Downloads:  715
  • Cited By: 0
Publishing process
  • Received Date:  27 January 2010
  • Accepted Date:  07 June 2010
  • Published Online:  15 March 2011

/

返回文章
返回