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We investigate the effect of delay time, pulse width and pump wavelength on photoelectron spectra and wave packet forming process of the three-level K2 molecules via time-dependent wave packet approach. There is no Autler-Townes splitting for weaker pump intensity or shorter pulse width. Delay time and pump wavelength can affect peak structure, position, and relative height. The vibration period of wave packet does not vary with pump wavelength, while the oscillating amplitude decreases with increasing pulse width. Results may provide important basis for realizing the optical control of molecules experimentally.
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Keywords:
- three-state ladder K2 molecules /
- time-dependent wave packet approach /
- photoelectron spectra /
- wave packet dynamic processes
[1] Henriksen N E, Engel V 2001 Int. Rev. Phys. Chem. 20 93
[2] Stolow A, Bragg A E, Neumark D M 2004 Chem. Rev. 104 1719
[3] Meier C, Engel V 1994 Phys. Rev. Lett. 73 3207
[4] Frohnmeyer T, Baumert T 2000 Appl. Phys. B 71 259
[5] Wollenhaupt M, Assion A, Bazhan O, Liese D, Sarpe-Tudoran C, Baumert T 2002 Appl. Phys. B 74 S121
[6] Hu W H, Yuan K J, Han Y C, Shu C C, Cong S L 2007 Chin. Phys. Lett. 24 1556
[7] Hu W H, Yuan K J, Han Y C, Shu C C, Cong S L 2010 Int. J. Quantum Chem. 110 1224
[8] Yao H B, Zheng Y J 2011 Phys. Chem. Chem. Phys. 13 8900
[9] Guo W, Lu X Q, Wang X L, Yao H B 2014 Europhys. Lett. 108 53002
[10] Sun Z G, Lou N Q 2003 Phys. Rev. Lett. 91 023002
[11] Yuan K J, Sun Z G, Cong S L, Lou N Q 2006 Phys. Rev. A 74 043421
[12] Liu Y F, Liu R Q, Ding J X 2009 Chin. Phys. Lett. 26 073301
[13] Liu Y F, Liu R Q, Ding J X 2010 Chin. Phys. B 19 033301
[14] Wollenhaupt M, Baumert T 2006 J. Photochem. Photobiol. A 180 248
[15] von den Hoff P, Kowalewski M, de Vivie-Riedle R 2011 Faraday Disscuss. 153 159
[16] Yao H B, Zheng Y J 2012 Chin. Phys. B 21 023302
[17] Yao H B, Li W L, Zhang J, Peng M 2014 Acta Phys. Sin. 63 178201 (in Chinese) [姚洪斌, 李文亮, 张季, 彭敏 2014 物理学报 63 178201]
[18] Peng Y G, Zheng Y J 2009 Phys. Rev. A 80 043831
[19] Yuan K J, Sun Z G, Cong S L, Wang S M, Yu J, Lou N Q 2005 Chem. Phys. 316 245
[20] Yao H B, Lin S Y, Zhen Y J 2011 J. Theor. Comp. Chem. 10 509
[21] Yao H B, Zheng Y J 2011 Acta Phys. Sin. 60 128201 (in Chinese) [姚洪斌, 郑雨军 2011 物理学报 60 128201]
[22] Zhang M, Tang T T, Zhang C M 2014 Acta Phys. Sin. 63 023302 (in Chinese) [张敏, 唐田田, 张朝民 2014 物理学报 63 023302]
[23] Schwoerer H, Pausch R, Heid M, Heid M, Engel V, Kiefer W 1997 J. Chem. Phys. 107 9749
[24] Zhang H, Han K L, Zhao Y, He G Z, Nan L Q 1997 Chem. Phys. Lett. 271 204
[25] Xie T X, Zhang Y, Zhao M Y, Han K L 2003 Phys. Chem. Chem. Phys. 5 2034
[26] Hu J, Han K L, He G Z 2005 Phys. Rev. Lett. 95 123001
[27] Chu T S, Zhang Y, Han K L 2006 Int. Rev. Phy. Chem. 25 201
[28] Baumert T, Engel V, Meier C, Gerber G 1992 Chem. Phys. Lett. 200 488
[29] Li Y J, Jiang W Y, Khait Y G, Hoffmann M R 2011 J. Chem. Phys. 134 174108
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[1] Henriksen N E, Engel V 2001 Int. Rev. Phys. Chem. 20 93
[2] Stolow A, Bragg A E, Neumark D M 2004 Chem. Rev. 104 1719
[3] Meier C, Engel V 1994 Phys. Rev. Lett. 73 3207
[4] Frohnmeyer T, Baumert T 2000 Appl. Phys. B 71 259
[5] Wollenhaupt M, Assion A, Bazhan O, Liese D, Sarpe-Tudoran C, Baumert T 2002 Appl. Phys. B 74 S121
[6] Hu W H, Yuan K J, Han Y C, Shu C C, Cong S L 2007 Chin. Phys. Lett. 24 1556
[7] Hu W H, Yuan K J, Han Y C, Shu C C, Cong S L 2010 Int. J. Quantum Chem. 110 1224
[8] Yao H B, Zheng Y J 2011 Phys. Chem. Chem. Phys. 13 8900
[9] Guo W, Lu X Q, Wang X L, Yao H B 2014 Europhys. Lett. 108 53002
[10] Sun Z G, Lou N Q 2003 Phys. Rev. Lett. 91 023002
[11] Yuan K J, Sun Z G, Cong S L, Lou N Q 2006 Phys. Rev. A 74 043421
[12] Liu Y F, Liu R Q, Ding J X 2009 Chin. Phys. Lett. 26 073301
[13] Liu Y F, Liu R Q, Ding J X 2010 Chin. Phys. B 19 033301
[14] Wollenhaupt M, Baumert T 2006 J. Photochem. Photobiol. A 180 248
[15] von den Hoff P, Kowalewski M, de Vivie-Riedle R 2011 Faraday Disscuss. 153 159
[16] Yao H B, Zheng Y J 2012 Chin. Phys. B 21 023302
[17] Yao H B, Li W L, Zhang J, Peng M 2014 Acta Phys. Sin. 63 178201 (in Chinese) [姚洪斌, 李文亮, 张季, 彭敏 2014 物理学报 63 178201]
[18] Peng Y G, Zheng Y J 2009 Phys. Rev. A 80 043831
[19] Yuan K J, Sun Z G, Cong S L, Wang S M, Yu J, Lou N Q 2005 Chem. Phys. 316 245
[20] Yao H B, Lin S Y, Zhen Y J 2011 J. Theor. Comp. Chem. 10 509
[21] Yao H B, Zheng Y J 2011 Acta Phys. Sin. 60 128201 (in Chinese) [姚洪斌, 郑雨军 2011 物理学报 60 128201]
[22] Zhang M, Tang T T, Zhang C M 2014 Acta Phys. Sin. 63 023302 (in Chinese) [张敏, 唐田田, 张朝民 2014 物理学报 63 023302]
[23] Schwoerer H, Pausch R, Heid M, Heid M, Engel V, Kiefer W 1997 J. Chem. Phys. 107 9749
[24] Zhang H, Han K L, Zhao Y, He G Z, Nan L Q 1997 Chem. Phys. Lett. 271 204
[25] Xie T X, Zhang Y, Zhao M Y, Han K L 2003 Phys. Chem. Chem. Phys. 5 2034
[26] Hu J, Han K L, He G Z 2005 Phys. Rev. Lett. 95 123001
[27] Chu T S, Zhang Y, Han K L 2006 Int. Rev. Phy. Chem. 25 201
[28] Baumert T, Engel V, Meier C, Gerber G 1992 Chem. Phys. Lett. 200 488
[29] Li Y J, Jiang W Y, Khait Y G, Hoffmann M R 2011 J. Chem. Phys. 134 174108
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