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Research progress of metal catalysts enhanced synthesized by cold plasma

Li Zhuang Di Lan-Bo Yu Feng Zhang Xiu-Ling

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Research progress of metal catalysts enhanced synthesized by cold plasma

Li Zhuang, Di Lan-Bo, Yu Feng, Zhang Xiu-Ling
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  • Cold plasma is a kind of non-thermal plasma, and characterized by high electron temperature (1-10 eV) and low gas temperature, which can be close to room temperature. It has been proved to be a fast, facile and environmentally friendly new method for synthesizing supported metal catalysts. Enhanced synthesis of metal catalysts by cold plasma consists of complex physical and chemical reactions. On the one hand, the active environment provided by cold plasma, can not only speed up the chemical reactions, shorten the reaction time from a few hours to several minutes, but also realize the kinetically or thermodynamically infeasible chemical reactions to achieve unconventional preparation. On the other hand, the phase contact behavior on a mesoscopic scale is influenced during cold plasma enhanced preparation, thereby the metal catalysts with structure different from that synthesized by traditional method. This review summarizes the reactor structure, physical and chemical mechanism for synthesizing metal catalysts by cold plasma, as well as the structure characteristics of the obtained metal catalysts. According to the working pressure, cold plasma can be categorized into low-pressure (LP) cold plasma and atmospheric-pressure (AP) cold plasma. The LP cold plasma is often generated by radio frequency glow discharge or direct current glow discharge, while the AP cold plasma is generally generated by dielectric barrier discharge and AP cold plasma jet. Energetic electrons are deemed to be the reducing agents for LP cold plasma. However, due to the frequent collisions among the electrons and gas molecules at atmospheric pressure, the electron energy in AP cold plasma is not high enough to reduce the metal ions directly. Therefore, hydrogen-containing gases are often adopted to generate active hydrogen species to reduce the metal ions. The process of synthesizing the metal catalysts by using the cold plasma is a fast, low-temperature process, and in the preparation process there exists a strong Coulomb repulsion. Therefore, metal catalysts with small size and high dispersion of metal nanoparticles, strong metal-support interaction, as well as specific metal structures (alloying degree and crystallinity) and modified supports can be obtained. Correspondingly, metal catalysts with high catalytic activity and stability can be synthesized. In addition, the challenges of preparing the cold plasma are discussed, and the future development is also prospected.
      Corresponding author: Di Lan-Bo, dilanbo@163.com;xiulz@sina.com ; Zhang Xiu-Ling, dilanbo@163.com;xiulz@sina.com
    • Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 21773020, 21673026), the Young Scientists Fund of the National Natural Science Foundation of China (Grant No. 11505019), the Liaoning Innovative Talents in University, China (Grant No. LR2017025), and the Natural Science Foundation of Liaoning Province, China (Grant No. 20180550085).
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    Wang L, Yi Y, Wu C, Guo H, Tu X 2017 Angew. Chem. 129 13867

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    [4]

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    Zhou T, Jang K, Jang B W L 2013 Catal. Today 211 147

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    Zhu B, Li X S, Liu J L, Liu J B, Zhu X, Zhu A M 2015 Appl. Catal. B 179 69

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    Wang N, Shen K, Yu X, Qian W, Chu W 2013 Catal. Sci. Technol. 3 2278

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    Guo F, Xu J Q, Chu W 2015 Catal. Today 256 124

    [9]

    Zhang C, Zhou Y, Shao T, Xie Q, Xu J, Yang W 2014 Appl. Surf. Sci. 311 468

    [10]

    Shao T, Zhang C, Long K, Zhang D, Wang J, Yan P, Zhou Y 2010 Appl. Surf. Sci. 256 3888

    [11]

    Pakhare D, Spivey J 2014 Chem. Soc. Rev. 43 7813

    [12]

    Liu C, Ye J, Jiang J, Pan Y 2011 ChemCatChem 3 529

    [13]

    Zheng Y, Jiao Y, Jaroniec M, Qiao S Z 2015 Angew. Chem. Int. Ed. 54 52

    [14]

    Cheng N, Stambula S, Wang D, Banis M, Liu J, Riese A, Xiao B, Li R, Sham T K, Liu L M, Botton G A, Sun X 2016 Nat. Commun. 7 13638

    [15]

    Qiao B, Liu J, Wang Y G, Lin Q, Liu X, Wang A, Li J, Zhuang T, Liu J 2015 ACS Catal. 5 6249

    [16]

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    Huang H, Xu Y, Feng Q, Leung D Y C 2015 Catal. Sci. Technol. 5 2649

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    [19]

    Liu C, Li M, Wang J, Zhou X, Guo Q, Yan J, Li Y 2016 Chin. J. Catal. 37 340

    [20]

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    Di L, Zhang J, Zhang X 2018 Plasma Processes Polym. 15 1700234

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    [24]

    Yang W, Yu Y, Wang L, Yang C, Li H 2015 Nanoscale 7 2877

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    Yu Y, Yang W, Sun X, Zhu W, Li X Z, Sellmyer D J, Sun S 2014 Nano Lett. 14 2778

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    Yu Y, Sun K, Tian Y, Li X Z, Kramer M J, Sellmyer D J, Shield J E, Sun S 2013 Nano Lett. 13 4975

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    Yu Y, Mukherjee P, Tian Y, Li X Z, Shield J E, Sellmyer D J 2014 Nanoscale 6 12050

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    Qiao B, Wang A, Yang X, Allard L F, Jiang Z, Cui Y, Liu J, Li J, Zhang T 2011 Nat. Chem. 3 634

    [30]

    Abbet S, Sanchez A, Heiz U, Schneider W D, Ferrari A M, Pacchioni G, Rösch N 2000 J. Am. Chem. Soc. 122 3453

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    Moses-DeBusk M, Yoon M, Allard L F, Mullins D R, Wu Z, Yang X, Veith G, Stocks G M, Narula C K 2013 J. Am. Chem. Soc. 135 12634

    [32]

    Lu J, Aydin C, Browning N D, Gates B C 2012 Angew. Chem. 124 5944

    [33]

    Kistler J D, Chotigkrai N, Xu P, Enderle B, Praserthdam P, Chen C Y, Browning N D, Gates B C 2014 Angew. Chem. Int. Ed. 53 8904

    [34]

    Sun S, Zhang G, Gauquelin N, Chen N, Zhou J, Yang S, Chen W, Meng X, Geng D, Banis M N, Li R, Ye S, Knights S, Botton G A, Sham T K, Sun X 2013 Sci. Rep. 3 1775

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    [36]

    Huang Z, Gu X, Cao Q, Hu P, Hao J, Li J, Tang X 2012 Angew. Chem. 124 4274

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    [43]

    Wang W, Wang Z, Wang J, Zhong C J, Liu C J 2017 Adv. Sci. 4 1600486

    [44]

    Zhou Y 2014 Ph. D. Dissertation (Tianjin: Tianjin University) (in Chinese)[周游 2014 博士学位论文 (天津: 天津大学)]

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    Hong J, Chu W, Chernavskii P A, Khodakov A Y 2010 J. Catal. 273 9

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    Wu Y W, Chung W C, Chang M B 2015 Int. J. Hydrogen Energy 40 8071

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    Dao V D, Tran C Q, Ko S H, Choi H S 2013 J. Mater. Chem. A 1 4436

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    Wang W, Anderson C F, Wang Z, Wu W, Cui H, Liu C J 2017 Chem. Sci. 8 3310

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    Li Z, Meng J, Wang W, Wang Z, Li M, Chen T, Liu C J 2017 Carbohydr. Polym. 161 270

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    Li Z, Zhang X, Zhang Y, Duan D, Di L 2018 Plasma Sci. Technol. 20 014016

    [62]

    Di L, Zhang X, Lee B, Lu P, Ahn W S, Park D W 2017 Plasma Chem. Plasma Process. 37 1535

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    Zou J J, Zhang Y P, Liu C J 2006 Langmuir 22 11388

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    Sawada Y, Taguchi N, Tachibana K 1999 Jpn. J. Appl. Phys. 38 6506

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    Di L, Zhang X, Xu Z, Wang K 2014 Plasma Chem. Plasma Process. 34 301

    [68]

    Kim T, Lee D H, Jo S, Pyun S H, Kim K T, Song Y H 2016 ChemCatChem 8 685

    [69]

    Di L, Zhang X, Xu Z 2014 Plasma Sci. Technol. 16 41

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    Dao V D, Jin I K, Choi H S 2016 Electrochim. Acta 201 1

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    Oh H J, Dao V D, Choi H S 2017 J. Alloy. Compd. 705 610

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    Peng H, Ma Y, Liu W, Xu X, Fang X, Lian J, Wang X, Li C, Zhou W, Yuan P 2015 J. Energy Chem. 24 416

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    Wang X, Xu W, Liu N, Yu Z, Li Y, Qiu J 2015 Catal. Today 256 203

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    Di L, Duan D, Zhang X, Qi B, Zhan Z 2016 IEEE Trans. Plasma Sci. 44 2692

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    Xu Z, Qi B, Di L, Zhang X 2014 J. Energy Chem. 23 679

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    [85]

    Fu Y, Yang S, Zou X, Luo H, Wang X 2016 Phys. Plasmas 23 093509

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    Fu Y, Zhang P, Verboncoeur J P 2018 Appl. Phys. Lett. 113 054102

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    Cole J, Zhang Y, Liu T, Liu C J, Sankaran R M 2017 J. Phys. D: Appl. Phys. 50 304001

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    Wang Y, Yu F, Zhu M, Ma C, Zhao D, Wang C, Zhou A, Dai B, Ji J, Guo X 2018 J. Mater. Chem. A 6 2011

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Metrics
  • Abstract views:  5693
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Publishing process
  • Received Date:  30 July 2018
  • Accepted Date:  05 September 2018
  • Published Online:  05 November 2018

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