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中国物理学会期刊

南氨酸高氯酸盐的晶体结构及分子的绝对构型

CSTR: 32037.14.aps.21.253

THE CRYSTAL STRUCTURE OF CUCURBITINE PERCHLORATE AND THE ABSOLUTE CONFIGURATION OF THE CUCURBITINE MOLECULE

CSTR: 32037.14.aps.21.253
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  • 南氨酸是一种新发现的天然氨基酸,其结构具有异于所有已知天然氨基酸的一些特点。本文叙述了利用X射线单晶体衍射方法对南氨酸高氯酸盐的晶体及分子结构所作的研究。从晶体的外形及X射线鉴定判明晶体属单斜晶系,劳埃(Laue)点羣为C2h,宝间羣为P21;测得晶胞参数a=5.68?、b=12.78?、c=6.23?、β=107°26′。利用三维帕特逊(Patterson)函数求出全部原子在晶胞中的粗略位置,经修正后获得了有关分子及晶体的结构化学数据。利用氯原子的反常散射效应决定了南氨酸分子的绝对构型。本文还讨论了南氨酸分子及其高氯酸盐晶体的结构特点。

     

    Cucurbitine is a natural amino acid newly found as the effective component in the crude drug, Cucurbita moschata Duch, which inhibits the growth of immature Schisto soma japonicum. This paper describes the X-ray diffraction studies on the structure of the perchlorate of the amino acid. Preliminary examinations show that the crystal belongs to the monoclinic system with space group P21 and unit cell dimensions a = 5.68 ± 0.01?, b = 12.78 ± 0.01?, c = 6.23 ± 0.01?, β = 107°26′± 12′. The trial structure has been derived by the three-dimensional Patterson analysis and refined by the two-dimensional Fourier syntheses. The absolute configuration of the Cucurbitine molecule has been determined by the anomalous scattering effect of the chlorine atom with CuKx radiation. It is of the form: Some important features of the structure of both the molecule and the crystal are described.

     

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