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中国物理学会期刊

LiKSO4的无公度相

CSTR: 32037.14.aps.33.235

THE INCOMMENSURATE PHASE OF LiKSO4

CSTR: 32037.14.aps.33.235
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  • 本文用多晶X射线衍射配合差热分析的方法研究了LiKSO4室温以上的相变。发现当温度在熔点以下到675℃之间,晶体结沟与α-K2SO4的高温相同构,α相最可能的空间群为P63/mmc.在Ti=675℃以下出现调制结构,类似K2WO4,K2MoO4等的无公度相;参数κ的值由0.492(640℃)而随温度变化。在470℃出现整合相变κ=0.500,整合后的结构为室温相的超点阵。然后在439℃转变为室温相(空间群为P63)。

     

    The phase transitions of LiKSO4 have been investigated by means of X-ray powder diffraction and thermal analysis above room temperature. It is established that the crystal structure of LiKSO4 between the melting point and 675℃ is isostructural with the high temperature phase of α-K2SO4 and its space group is probably P63/mmc. Cooling below Ti=675℃ , there appears an incommensurately modulated structure analogous to the incommensurate phase in K2WO4, K2MoO4, etc. The parameter κ changes with temperature from 0.492(640℃ ) to 0.500(470℃ ). At 470℃ , I→C phase transition (lock-in) takes place, after which the crystal structure becomes the superstructure lattice of the room temperature phase. At 439℃ the superstructure disappears yielding to the room temperature phase (P63).

     

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