搜索

x
中国物理学会期刊

电子关联对C60激子极化子的影响

CSTR: 32037.14.aps.43.1833

ELECTRON CORRELATION EFFECT ON C60 EXCITON POLARON

CSTR: 32037.14.aps.43.1833
PDF
导出引用
  • 本文采用扩展的Hubbard模型,在电子-晶格耦合的紧束缚近似下,研究了光激发下的C60,分子的激子态和极化子态。我们发现,电子关联效应相当敏感地影响到单态和三态激子的束缚能。同时,C60分子动力学晶格弛豫使激子极化子得以形成。光激发下的C60分子,在电子相互作用U~5.0eV,V~2.0eV时,能够定性地解释荧光发射谱。

     

    Exciton polaron states in C60 molecular are theoretically studied in the tight-binding approach supplemented by the extended Hubbard interaction. The binding energies of the lowest singlet and triplet excitons depend sensitively upon the electron correlation. Then the exciton polaron is formed due to the electron-lattice coupling. Relevent experiments in photo-luminescence spectrum of Cso can be explained qualitatively by the present model with moderate interaction strength U~5.0eV,V~2.0eV.

     

    目录

    /

    返回文章
    返回