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中国物理学会期刊

铁掺杂Tl-1223超导相的额外氧缺陷研究

CSTR: 32037.14.aps.45.1570

EXTRA OXYGEN DEFECT INDUCED BY Fe-DOPING IN Tl-SYSTEM SUPERCONDUCTOR

CSTR: 32037.14.aps.45.1570
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  • 在铁掺杂的Tl-1223相中,铁对超导电性有明显的破坏作用,霍尔系数测量、热重分析和穆斯堡尔谱表明占据铜晶位的铁杂质原子不仅直接破坏CuO2面的完整性而使超导转变温度降低,更重要的是铁的掺入诱导了额外氧原子进入晶格,形成了对载流子的强局域束缚作用,致使载流子浓度随铁掺杂量呈线性下降.额外氧导致了与其近邻的铁和铜原子产生了偏离CuO2平面的位移,从而形成新的铁氧配位.针对额外氧缺陷精细结构的讨论,对研究额外氧和阳离子在CuO2平面上的无序排列

     

    In Fe-doped Tl-1223 superconducting phase, Fe-dopants significantly destroy superconductivity . Hall coefficient, thermogravimetric measurements and M?ssbauer effect show that Fe-dopants not only directly destroy the integrity of Cu-O layers to low superconduction transition temperature, but also induce extra oxygen to enter lattice. These extra oxygen defects can strengtheningly bind carriers in Cu-O layers, Such binding effect gives rise to decreasing of the carrier density with Fe-doping level increasing. In addition. the extra oxygen results in a deviation of its neibouring Fe(Cu) from center of Cu-O network, and from a new Fe-O coordination. It is important for high-Tc superconducting mechanism to study the structural details and carrier-binding effect of extra oxygen defect on superconducticity.

     

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