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中国物理学会期刊

Ce填充分数对p型CeyFe1.5Co2.5Sb12化合 物热电传输特性的影响

CSTR: 32037.14.aps.49.2460

EFFECT OF Ce FILLING FRACTION ON THERMOELECTRIC TRANSPORT PROPERTIES OF p-TYPE C eyFe1.5Co2.5Sb12

CSTR: 32037.14.aps.49.2460
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  • 研究了Ce填充分数对富Co组成的填充式skutterudite化合物:CeyFe1.5Co2.5Sb12(y=0—0.46)的热电传输特性的影响.CeyFe1.5Co2.5Sb12有现为p型传导.霍尔系数RH随Ce填充分数的增加而增加,空穴浓度p和电导率σ随Ce填充分数的增加而减少.泽贝克 系数α随Ce填

     

    Effect of Ce filling fraction on the thermoelectric transport properties of p-ty pe Co-rich filled skutteudite compounds:CeyFe1.5Co2.5 Sb12 (y=0—0.46) were investigated. CeyFe1.5Co2.5Sb12 showed p-type conduction. Hall coefficient RH increased with increasing Ce filling fraction. Hole concentration p and electrical conductivity σ decreased with increasing Ce filling fraction. Se ebeck coefficient α increased with increasing Ce filling fraction. when Ce fill ing fraction was about 0.3, the lattice thermal conductivity κl reac hed the minimum value.It indicated that the effect of Ce rattling on phonon scat tering was the strongest as Sb-dodecahedron partial voids were filled by Ce. A m aximum ZT value of 1.1 was obtained for Co-rich Ce0.28Fe1.52Co2.48Sb12 at 750K.

     

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