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中国物理学会期刊

Nd1.67Sr0.33NiO4中的热导反常

CSTR: 32037.14.aps.53.3853

Anomalous thermal conductivity in Nd_1.67Sr0.33NiO_4

CSTR: 32037.14.aps.53.3853
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  • 报道了两个典型掺杂的镍氧化物Nd_2-xSr_xNiO_4(x =0.33,1.35)的低温热导率、电阻率和低场交流磁化率,测试温区为77—300K. 在Nd_2-xSr_xNiO_4 (x=0.33)样品的热导率-温度曲线上在电荷有序转 变温度(T_CO)和自旋有序转变温度(T_SO)附近分别观测到反常, 电荷有序使热导率在T_CO以下有所增加,反铁磁自旋有序使热导率在T_SO附近被压制. 在低场交流磁化率-温度曲线上也分别观测到对电荷有序和自旋有 序的响应,而在其电阻率-温度曲线上仅观测到电荷有序. 作为比较,Nd_1.67Sr0.33NiO_4样品中没有观测到输运性质和磁性质上的反常. 两个样品中声子热导占 主导地位. Nd_1.67Sr0.33NiO_4样品中电荷有序和自旋有序导致的热导 率的反常表明样品中存在强的电荷-声子和自旋-声子相互作用.

     

    The temperature dependence of thermal conductivity (K),resistivity (ρ) and low field ac susceptibility (χ) of perovskite nick elates Nd_2-xSr_xNiO_4(x =0.33,1.35) have been measured at temperatures from 77 to 300 K. The thermal conductivity an omalies associated with charge_order (CO) and spin_order (SO) are observed simultaneously in Nd_1.67Sr0.33NiO_4 for the firs t time so far as we know. The thermal conductivity is enhanced belowT_CO , but is suppressed near T_SO. There is also response to CO and S O in the χ-Τ curve. Only CO is observed in the ρ-Τ curve. In contrast, th ere are no anomalies in K-Τ, ρ-Τ andχ-Τ of Nd_1.67Sr0.33NiO_4. The anomalous phonon thermal conductivi ty in Nd_1.67Sr0.33NiO_4 indicates that there are strong charg e_phonon interaction and the spin_phonon interaction in this compound.

     

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