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中国物理学会期刊

化合物HoMn6Sn6的磁晶各向异性及自旋重取向相变研究

CSTR: 32037.14.aps.54.5879

Magnetocrystalline anisotropy and spin-reorientation transition of intermetallic compound HoMn6Sn6

CSTR: 32037.14.aps.54.5879
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  • 采用交换相互作用的分子场理论模型对金属间化合物HoMn6Sn6的自旋重取向相变进行了研究. 从理论上计算了HoMn6Sn6的易磁化方向以及Ho和Mn离子磁矩与c轴夹角随温度的变化. 基于单离子模型计算了Ho离子的一阶和二阶磁晶各向异性常数K1R和K2R随温度的变化. 研究表明,为了很好描述该化合物的自旋重取向相变,必须考虑Ho离子的四阶晶场项及相应的二阶磁晶各向异性常数K2R,K2R与K1R和Mn离子磁晶各向异性常数K1t之间的相互竞争是导致HoMn6Sn6自旋重取向相变的重要因素.

     

    The molecular field theory of exchange interaction has been applied to investigate the spin-reorientation transition in intermetallic compound HoMn6Sn6. The theoretically calculated temperature dependence of easy magnetization direction is in good agreement with experimental data. The temperature dependence of magnetocrystalline anistropic constants of Ho ion K1R and K2R have been calcullated in the framework of single ion model. It is shown that the fourth-order crystal field parameter B04 and the corresponding second-order magnetocrystalline anistropic constant K2R of Ho ion have to be taken into account in order to explain the spin-reorientation transition. The competition between K2R and K1R plays an important role in the spin-reorientation transition in HoMn6Sn6.

     

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