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中国物理学会期刊

Mn5Ge2.7M0.3 (M=Ga,Al,Sn) 化合物的磁性和磁熵变

CSTR: 32037.14.aps.54.5884

Magnetic properties and magnetocaloric effects of Mn5Ge2.7M0.3 (M=Ga, Al, Sn) compounds

CSTR: 32037.14.aps.54.5884
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  • 研究了Mn5Ge2.7M0.3(M=Ga,Al,Sn)化合物的磁性和磁熵变. x射线衍射实验表明,研究的化合物均呈六角Mn5Si3型结构. 三种原子对Ge原子的替代,使得平均Mn原子磁矩下降,但居里温度没有明显的变化. 由于磁矩的降低,导致磁熵变值的下降,在磁场变化为4.0×106A·m-1时,对应于M=Ga,Al和Sn的样品,最大磁熵变值ΔSmaxM分别为6.1,6.3和5.3J·kg-1K-1,但磁熵变峰值的半高宽ΔTFWHM有所增加. 另外,Mn5Ge2.7M0.3(M=Ga,Al,Sn)化合物在高于居里温度的Arrott曲线上出现了一个不连续点,即样品在一定温度下的顺磁磁化率在某一临界磁场下发生了突变,临界磁场与温度几乎呈正比关系.这可能是由于样品在加一定磁场时3d带的费米能级发生了变化,使得有效电子数的减少所致.

     

    The magnetic properties and magnetocaloric effects of Mn5Ge2.7M0.3(M=Ga, Al, Sn) compounds have been studied. All samples crystallize in the hexagonal Mn5Si3-type structure with space group P63/mcm. The average Mn magnetic moment decreases and the Curie temperature remains almost unchanged by the substitution of M for Ge. The magnetic entropy changes in these compounds are determined from the temperature and field dependence of the magnetization using the thermodynamic Maxwell relation. The substitution of M for Ge reduces the magnitude of the magnetic entropy change owing to the decrease of the magnetic moment but broadens the magnetic entropy change peak. The maximum magnetic entropy changes for a field changes of 4.0×106A·m-1 are 6.1, 6.3, and 5.3J·kg-1K-1 for M=Ga, Al, and Sn, respectively. In addition, anomalies are found in the Arrott curves of Mn5Ge2.7M0.3(M=Ga Al, Sn) compounds under a critical field Hc when the temperature is higher than the Curie temperature TC, which indicates that the paramagnetic susceptibilities of these compounds change sharply. The value of Hc increases almost linearly with increasing temperature. This phenomenon is probably due to the change of Fermi energy by the applied magnetic field, which reduces the number of the effective charges.

     

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