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中国物理学会期刊

亚乙基硫脲的表面增强拉曼极化率研究:电磁和电荷转移机制

CSTR: 32037.14.aps.55.6315

A study of the surface enhanced Raman bond polarizability derivatives of ethylene thiourea:electromagnetic and charge transfer mechanisms

CSTR: 32037.14.aps.55.6315
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  • 测量了吸附在银电极表面的亚乙基硫脲分子在不同电位下的表面增强拉曼光谱,对光谱强度变化进行了分析.从拉曼光谱强度计算出分子的键极化率数值,分析极化率大小和变化情况,提出了分子在不同电位下表面增强效应的增强机制.

     

    The surface enhanced Raman spectra of ethylene thiourea adsorbed on the silver electrode were measured at different electrode potentials. Based on the analysis of the Raman spectra, especially the bond polarizability derivatives elucidated from the Raman intensities by our algorithm, important information on the surface enhancement mechanisms was collected. The results show that both the electromagnetic and charge transfer mechanisms are responsible for the large enhancement, the former operating in the whole potential range between -0.3 and -1.2 V while the latter only in the range lower than -0.7 V.

     

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