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用脉冲激光沉积法制备了非金属Te掺杂的钙钛矿锰氧化物La0.82Te0.18MnO3单晶薄膜.该薄膜从83 K升温至373 K过程中发生金属-绝缘体相变,转变点温度为283 K.其电阻率在TTMI时符合电子-电子、电子-磁振子散射公式;在T>TMI时为小极化子输运.薄膜在低温段连续激光(波长为532 nm,40 mW)作用下电阻率显著增大,电阻变化率在253 K达到最大值51.1%,该变化率远大于相同条件下的空穴掺杂材料;在高温段产生了较小的光电导,电阻变化率小于10%.这些现象主要与激光激励下自旋系统和小极化子的变化有关.La0.82Te0.18MnO3薄膜在激光诱导下具有明显的与自旋相关的弛豫现象.激光开始作用时薄膜电阻率随时间的变化符合指数关系.
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关键词:
- La0.82Te0.18MnO3薄膜 /
- 光诱导 /
- 输运特性 /
- 电子掺杂
The transition from the metallic phase to the nonconductive phase occurred at 283 K in La0.82Te0.18MnO3 thin film prepared by pulse laser deposition method. The transport results show that the data satisfy the formula of electro-electro and electro-magnon scattering for TTMI; when T>TMI it agrees with small polaron transport model. The effect of the continuous wave laser(532 nm,40 mW) on the film was also investigated. Below TMI, the resistivity has a photo-induced increase. The maximum rate of resistivity changes(Δρ/ρ0) can reach 51.1%, which is much greater than that of hole-doped manganites. Above TMI there is a photoconduction. The relaxation was observed in the experiment when the laser was turned on and off. The resistively is exponentially related with the time.-
Keywords:
- La0.82Te0.18MnO3 film /
- photo-induced /
- transport properties /
- electron-doped







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