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中国物理学会期刊

尺寸效应对Er3+掺杂纳米Y2O3的发光特性的影响

CSTR: 32037.14.aps.58.165

Size dependent luminescence properties of Er3+ doped nano-crystalline Y2O3

CSTR: 32037.14.aps.58.165
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  • 采用燃烧法制备了不同尺寸的Er3+掺杂Y2O3粉体材料,研究了尺寸效应对Er3+掺杂纳米Y2O3材料发光特性的影响.光声光谱显示,对于不同晶粒尺寸的样品,Er3+离子光声峰位置几乎保持不变.这表明小尺寸效应对稀土离子能级位置影响很小.对488nm激光激发下的发射谱的分析发现,随着样品颗粒尺寸的减小,4S3/2能级和 

    Er3+ doped Y2O3 nano-crystals with different size are prepared using combustion method. Size effect on luminescence properties of Er3+ doped Y2O3 nano crystals are investigated. No shift of the absorption peak in the photo-acoustic spectra is observed with the decrease of the Y2O3particle size, indicating that the size induced energy shifts of the rare-earth levels are negligible. However, the emission spectra under 488nm excitation indicate that the ratio of the intensity of 4S3/2→4I15/2 transition to that of 2H11/2→4I15/2 decreases with the decrease of the particle size. It is believed that the rate of hypersensitive transition of 2H11/2→4I15/2 increases with the decrease of the particle size more quickly than that of transition of 4S3/2→4I15/2. The time dependence of the 554nm luminescence decay excited by 518nm reveals that the rate of up-converted energy transfer occurring between two Er3+ ions in 4S3/2 state increases with the decrease of the particle size.

     

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