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中国物理学会期刊

Sr2CoO4-δ薄膜中的自旋玻璃态的磁性质研究

CSTR: 32037.14.aps.59.6585

Glassy magnetic behaviors in oxygen-deficient Sr2CoO4-δ films

CSTR: 32037.14.aps.59.6585
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  • 用脉冲激光沉积方法(PLD)在铝酸镧衬底上制备了c取向的高氧空位含量的锶钴氧薄膜.X射线衍射分析表明薄膜单一取向且没有明显杂相.原位的高气压反射式高能电子衍射仪(RHEED)监测显示,薄膜为层状生长.通过对薄膜磁化强度随温度、磁场及时间的变化曲线进行测量,发现零场冷曲线上可能存在两个特征温度:Tf和Ta.Tf为对应玻璃态的冻结温度而Ta对应少量的不缺

     

    We have fabricated c-axis-oriented Sr2CoO4-δ thin films under relatively low oxygen pressure by the pulsed laser deposition method (PLD) on LaAlO3 substrates. X-ray diffraction and high-pressure reflection high energy electron diffraction (RHEED) demonstrate that the films were well deposited. There exist two different characteristic temperatures, Tf and Ta, in the ZFC curve of temperature dependence of magnetization. Tf may correspond to the freezing temperature while Ta may be related with the anisotropic field of c-axis. Further investigations including magnetic relaxation, memory effect and hysteresis behaviour measurements suggest a main phase of spin glass, which starts the frozen-in process even above the freezing temperature. We ascribe the spin glass behaviour to the competition betwcen double-exchange and super-exchange interactions which could have originated from the coexistence of Co4+ and Co3+ caused by oxygen deficiency in the films.

     

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