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中国物理学会期刊

超快强激光场中原子分子的里德伯态激发

CSTR: 32037.14.aps.71.20221258

Rydberg state excitation of atoms and molecules in ultrafast intense laser field

CSTR: 32037.14.aps.71.20221258
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  • 作为超快强激光场与原子分子相互作用的基本过程之一, 里德伯态激发被认为是强场隧穿电离诱导的物理过程的一个重要补充, 受到了研究者的广泛关注. 过去几十年来, 不断涌现了出色的理论和实验工作, 对超快强激光场下里德伯态激发的物理机制形成了更加深入的理解和更为系统的全新认识, 使得该研究课题逐步发展成为强场原子分子物理领域的一个重要研究方向. 本文系统地综述了超快强激光场中原子分子的里德伯态激发的研究进展, 着重介绍近年来在原子强场里德伯态激发的物理机制、分子强场里德伯态激发中的结构效应以及基于强场里德伯态激发的中性粒子加速和相干辐射研究等方面的研究工作, 在此基础上, 总结和展望了强场激发研究方向未来的发展趋势. 希望本文能够为强场激发相关研究提供较为详尽的文献综述, 为进一步开展深入的研究工作提供参考.

     

    When atoms or molecules are irradiated by a strong laser field with pulse duration of tens of femtoseconds and intensity larger than 1013 W/cm2, they will generally undergo tunneling ionization, which will induce various non-perturbative and highly nonlinear phenomena. Investigations into the strong field physical processes is of significance in studying attosecond physics, molecular orbital imaging, ultrafast electron diffraction and advanced short ultraviolet light sources. While there is a relatively long history of the studies of tunneling ionization induced physics including high-order above threshold ionization (HATI), high-order harmonic generation (HHG) and non-sequential double ionization (NSDI), it is until recently to surprisedly find that in the tunneling ionization region, neutral atoms or molecules can survive in strong laser fields in highly excited Rydberg states. As a basic process of the interaction between ultrafast strong laser fields and atoms or molecules, such a Rydberg state excitation (RSE) has been viewed as an important supplement to the physical picture of the tunneling ionization. During the past several years, the extensive research attention has been paid to the RSE process in strong laser field. Various theoretical and experimental methods have been developed to investigate the strong field RSE of both atoms and molecules, to understand the underlying physical mechanism behind the recapture of the tunneling electrons and to reveal the quantum features and molecular structure effect in RSE. These advances have brought about an in-depth understanding and a systematic view of the atomic and molecular RSE in strong laser fields, as well as their relations to the other tunneling ionization induced physical processes such as ATI, HHG and NSDI. Here, we systematically review recent research progress of the atomic and molecular RSE in strong laser fields. We particularly focus on several aspects of this strong field process, i.e. the physical mechanism of the recapture, the quantum feature and the interference of different orbits, and the structure effect in molecular RSE. In addition, neutral particle acceleration and coherent radiation which can be induced by the strong field RSE, are also discussed. Finally, we provide a short summary and prospect of the future studies on the strong field RSE.

     

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