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中国物理学会期刊

基于金刚石NV色心系综可调谐毫米波受激辐射

Controllable millimeter-wave stimulated radiations from NV-centres in diamond

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  • 高品质毫米波光源的匮乏是制约毫米波相干技术发展的重要瓶颈之一,而在室温条件下实现高效、稳定的毫米波受激辐射,已成为该技术领域亟待攻克的关键挑战。针对这一难题,本文提出一种基于强磁场调控氮空位(NV)色心基态零场分裂的室温毫米波受激辐射实现方案。具体而言,我们选取轴向强人造磁场(约2 T)作用下基态三重态能级发生塞曼分裂的NV色心作为毫米波激射的自旋介质——其优异的长自旋相干时间特性与可实现的光学初始化能力,使得通过532 nm激光泵浦即可达成塞曼能级的布居数反转。借助高品质因子(Q ≈ 5×104)谐振腔构建的自旋-光子集体耦合模型,本研究证实该方案的泵浦阈值可低至约270 s−1;在理想条件下,可输出功率达微瓦级的毫米波相干辐射,从而有望在室温条件下,为6G无线通信、深空探测等领域提供高品质毫米波相干光源。

     

    The scarcity of high-quality millimeter-wave coherent light sources constitutes a critical bottleneck for the development of 6G communications, deep-space exploration, and related fields. Conventional approaches, such as low-frequency synthesis and high-frequency beating, suffer from low output power and poor coherence, while cryogenic microwave coherent sources cannot operate at room temperature. Hence, there is an urgent demand for efficient, stable, millimeter-wave stimulated-emission coherent sources that function under ambient conditions. Leveraging the unique advantages of the nitrogen-vacancy (NV) center system—including long spin coherence times at room temperature, optical initializability, and precise tunability of Zeeman levels—combined with a high-quality-factor millimeter-wave resonator, we can construct a coupled system of light and artificial atoms operable at room temperature. This paper proposes a scheme for room-temperature millimeter-wave stimulated emission based on tuning the ground-state zero-field splitting of diamond NV centers via a strong axial magnetic field, aiming to achieve a high-quality coherent millimeter-wave radiation source.
    Through Zeeman-level engineering of NV centers under tesla-level magnetic fields, we propose that by applying a strong axial magnetic field B_\textNV > 1.18\ \textT along the 111 crystallographic direction of the NV^- center, the radiative transition frequency of the NV-center artificial atom can be shifted into the millimeter-wave band. Subsequently, a millimeter-wave stimulated-emission system is constructed, comprising a 2 T superconducting magnet, an ensemble of NV centers in diamond, a high-quality-factor cylindrical resonant cavity, and a 532 nm pump laser. A diamond single crystal containing \sim 10^13 NV centers is placed at the center of the cavity and resonantly coupled to the cavity’s TE_01\delta mode. Optical pumping with 532-nm laser light enables population inversion of the NV centers. The stimulated-emission millimeter-wave photons can establish coherent oscillation inside the cavity, thereby yielding a coherent millimeter-wave output. Based on numerical simulations with typical parameters, the threshold conditions for achieving millimeter-wave stimulated emission are derived, and the linewidth of the obtained coherent radiation is evaluated. The results indicate that, using a cavity with a quality factor of Q = 5 \times 10^4 and a diamond sample with N = 4 \times 10^13 NV centers, the optimal pumping rate can be attained with a remarkably low laser-pump threshold of w_\textth \approx 270\ \texts^-1. Under these conditions, the collective coherence of the atomic ensemble is maximized, enabling the generation of coherent millimeter-wave radiation with a power exceeding 10^-6\ \textW (microwatt level) and a linewidth as narrow as 10^-4\ \textHz. Higher output power can be achieved by increasing the number of NV centers, improving the cavity quality factor, or raising the pump rate.
    Specifically, this work demonstrates that, by applying a 2 T axial magnetic field and employing a high-quality resonator with Q = 5 \times 10^4, stimulated emission of millimeter waves at a frequency of 53.13\ \textGHz can be realized at room temperature. Moreover, by adjusting the strength of the applied magnetic field, it is theoretically feasible to achieve a fully tunable coherent millimeter-wave source covering the entire 30\ \text–\ 300\ \textGHz band. This provides a viable pathway toward a high-performance room-temperature millimeter-wave light source. The methodology adopted here—combining quantum Langevin equations with the mean-field approximation to describe stimulated-emission amplification—can be extended to other microwave gain-media systems for realizing various coherent radiation sources based on stimulated emission. In particular, the fact that the coherence properties of NV centers are only weakly affected by strong magnetic fields makes the proposed magnetic-field-tuning scheme for millimeter-wave stimulated emission from diamond color centers experimentally verifiable, paving the way for the generation of highly coherent wave sources across the entire microwave frequency range.

     

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