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本文研究了近共振增强的四能级系统有机染料溶液中简并的四波混频后向波和前向波的位相复共轭特性。用有效长度为5毫米、浓度为2.5×10-5克分子的叶绿素A甲醇溶液作介质,当调QNd:YAG倍频抽运光能量为8毫焦耳时,非线性反射率为22%。研究了若丹明6G酒精溶液双光子共振增强的简并的四波混频作用。测量了非线性反射率与介质浓度及抽运波和物波强度的关系曲线。理论分析了四波混频前向波的位相复共轭特性,实验证实了理论的预言。另外,把四重简并的四波混频推广到二重简并。用9740有机染料二氯乙烷饱和吸收溶液作介质,实现了1.06微米到5320埃的象转换。介质长度为5毫米,抽运光能量为5毫焦耳时,转换效率达25%。理论分析表明,用对红外近共振吸收而对可见辐射是透明的介质可实现高效率红外象转换。Phase conjugation of backward-and forward-wave produced by degenerate four-wave mixing using a nearly resonantly enhanced nonlinearity in four-level organic dye solutions was investigated. The conversion efficiency of 22% had been obtained in a 2.5 X 10-5 - molar solution of Chlorophyll A in methylalcohol with a 5 mm interaction length and a pumping energy of ~ 8 mJ from SH of a Q-switched Nd: YAG. Degene-rate four-wave mixing by two-photon resonant-enhancement in the solution of rhodamine 6G in alcohol was studied. Measurements were performed which described the dependence of nonlinear reflectivities on the molar concentrations of the media and the intensities of the pumping and object waves. Phase conjugation characteristics of forward-wave in four-wave mixing process were theoretically analysed. Experiments have cofirmed the theoretical prediction. The method of quartet degenerate four-wave mixing had been ex-tended to the doublet degenerate case. Using this method image conversion from 1.06 μm to 5320 ? had been realized with a conversion efficiency of 25% in a 5 mm long satu-rable absorber made of organic dye 9740 solution in dichloroethane. Theoretical analy-sis showed that using a medium, which is a near resonant absorber for the infrared object wave but is transparent for the visible reconstruction wave, the conversion efficiency may be well in excess of unity.
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