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分子间费米共振增强二元溶液体系的受激拉曼散射研究

门志伟 里佐威 李占龙 周密 孙成林 何丽桥

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分子间费米共振增强二元溶液体系的受激拉曼散射研究

门志伟, 里佐威, 李占龙, 周密, 孙成林, 何丽桥

Enhanced stimulated Raman scattering of binary solution by intermolecular Fermi resonance

Li Zhan-Long, Zhou Mi, He Li-Qiao, Sun Cheng-Lin, Li Zuo-Wei, Men Zhi-Wei
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  • 研究了液芯光纤内不同体积比的甲苯和间二甲苯二元混合溶液的受激拉曼散射.实验结果表明:在不同的体积比之下二元溶液的环呼吸振动模式1002 cm-1,甲基的CH伸缩振动模式2920 cm-1 以及芳香环CH对称伸缩振动模式3058 cm-1的拉曼带同时产生受激拉曼辐射,并且2920 cm-1 和 3058 cm-1 拉曼带的一阶受激拉曼散射阈值要低于1002 cm-1拉曼带的二阶
    Stimulated Raman scattering(SRS) of binary solution of toluene and m-xylene are studied at different volume concentrations in liquid-core optical fiber. The experimental results show that the vibration modes of 1002 cm-1, 2920 cm-1 and 3058 cm-1 bands are simultaneously stimulated to generate the SRS, and the SRS thresholds of the 1st-order Stokes of 2920 cm-1 and 3058 cm-1 bands are lowered compared with the 2nd-order Stokes of 1002 cm-1 band, and the main peaks of 2920 cm-1 and 3058 cm-1 bands are different as volume concentration changes. We assume that the intermolecular Fermi resonance is the main mechanism for these phenomena, which is explained by the Raman scattering cross section theory.
    • 基金项目: 国家自然科学基金(批准号:10974067),吉林省科技厅项目(批准号:20101508,201115033,201101037)和第四十八批中国博士后科学基金面上资助的课题.
    [1]

    Kaminskii A A, Rhee H, Eichler H J 2008 Laser Phys. Lett. 5 304

    [2]

    Garruthers T F, Duling I N, Horowitz M 2000 Opt .Lett. 25 153

    [3]

    Dirda P T, Millot G, Wabnicz S 1998 J.Opt.Soc.Am.B 15 1433

    [4]

    Guo L N, Tang Z L, Xing D 2008 Sci. China G 38 1 (in Chinese)[郭利娜、唐志列、邢 达 2008 中国科学G辑 1]

    [5]

    Zhang J T 2005 Chin. Phys. 14 169

    [6]

    Hasi W L J, Lü Z W, Li Q, Ba D X, He W M 2007 Acta Phys. Sin. 56 1385 (in Chinese)[哈斯乌力吉、吕志伟、李 强、巴德欣、何伟明 2007 物理学报 37

    [7]

    Zang J C, Xie L Y, Li X, Zhang D X, Feng B H 2007 Acta Phys. Sin. 56 1833 (in Chinese)[臧竞存、谢丽艳、李 晓、 张东香、 冯宝华 2007 物理学报 56

    [8]

    Zhang L, Dong Q L, Zhao J, Wang S J, Sheng Z M, He M Q, Zhang J 2009 Acta Phys. Sin. 58 1833 (in Chinese)[张 蕾、董全力、赵 静、 王首钧、 盛政明、 何民卿、 张 杰 2009 物理学报 58

    [9]

    Kwok A S, Chang R K 1992 Opt. Lett. 17 1262

    [10]

    Kwok A S, Chang R K 1993 Opt. Lett. 18 1597

    [11]

    Xie J G, Ruekgauer T E, Armstrong R L, Pinnick R G 1993 Opt. Lett.18 340

    [12]

    Chen Y Q, Wang L, Lu X B, Chen Y Q, Qiu M X 1991Opt.Lett.16 1469

    [13]

    Bobovich Y S, Bortkevich A V 1968 J. Exp. and Theor. Phys. Lett.7 13

    [14]

    Zuo J, Tian Y J, Chen J, Wang Y C, Gao S Q, Lu G H, Li Z W 2008 Appl.Phys.B 91 467

    [15]

    Men Z W, Fang W H, Ding Y F, Li Z W 2009 J.Raman Spectrosc 40 1039

    [16]

    Veas C, McHale J L 1989 J.Am.Chem.Soc.111 7042

    [17]

    Li Z W, Li J N, Gao S Q 1998 Jpn.J.Appl.Phys.37 1889

    [18]

    Li Z W, Gao S Q, Sun X 2001 Spectrosc Lett.34 569

    [19]

    Tian YJ, Zuo J, Zhang L Y 2007 Appl.Phys.B 87 727

  • [1]

    Kaminskii A A, Rhee H, Eichler H J 2008 Laser Phys. Lett. 5 304

    [2]

    Garruthers T F, Duling I N, Horowitz M 2000 Opt .Lett. 25 153

    [3]

    Dirda P T, Millot G, Wabnicz S 1998 J.Opt.Soc.Am.B 15 1433

    [4]

    Guo L N, Tang Z L, Xing D 2008 Sci. China G 38 1 (in Chinese)[郭利娜、唐志列、邢 达 2008 中国科学G辑 1]

    [5]

    Zhang J T 2005 Chin. Phys. 14 169

    [6]

    Hasi W L J, Lü Z W, Li Q, Ba D X, He W M 2007 Acta Phys. Sin. 56 1385 (in Chinese)[哈斯乌力吉、吕志伟、李 强、巴德欣、何伟明 2007 物理学报 37

    [7]

    Zang J C, Xie L Y, Li X, Zhang D X, Feng B H 2007 Acta Phys. Sin. 56 1833 (in Chinese)[臧竞存、谢丽艳、李 晓、 张东香、 冯宝华 2007 物理学报 56

    [8]

    Zhang L, Dong Q L, Zhao J, Wang S J, Sheng Z M, He M Q, Zhang J 2009 Acta Phys. Sin. 58 1833 (in Chinese)[张 蕾、董全力、赵 静、 王首钧、 盛政明、 何民卿、 张 杰 2009 物理学报 58

    [9]

    Kwok A S, Chang R K 1992 Opt. Lett. 17 1262

    [10]

    Kwok A S, Chang R K 1993 Opt. Lett. 18 1597

    [11]

    Xie J G, Ruekgauer T E, Armstrong R L, Pinnick R G 1993 Opt. Lett.18 340

    [12]

    Chen Y Q, Wang L, Lu X B, Chen Y Q, Qiu M X 1991Opt.Lett.16 1469

    [13]

    Bobovich Y S, Bortkevich A V 1968 J. Exp. and Theor. Phys. Lett.7 13

    [14]

    Zuo J, Tian Y J, Chen J, Wang Y C, Gao S Q, Lu G H, Li Z W 2008 Appl.Phys.B 91 467

    [15]

    Men Z W, Fang W H, Ding Y F, Li Z W 2009 J.Raman Spectrosc 40 1039

    [16]

    Veas C, McHale J L 1989 J.Am.Chem.Soc.111 7042

    [17]

    Li Z W, Li J N, Gao S Q 1998 Jpn.J.Appl.Phys.37 1889

    [18]

    Li Z W, Gao S Q, Sun X 2001 Spectrosc Lett.34 569

    [19]

    Tian YJ, Zuo J, Zhang L Y 2007 Appl.Phys.B 87 727

计量
  • 文章访问数:  7371
  • PDF下载量:  1031
  • 被引次数: 0
出版历程
  • 收稿日期:  2011-01-25
  • 修回日期:  2011-02-18
  • 刊出日期:  2011-09-15

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