搜索

x

留言板

尊敬的读者、作者、审稿人, 关于本刊的投稿、审稿、编辑和出版的任何问题, 您可以本页添加留言。我们将尽快给您答复。谢谢您的支持!

姓名
邮箱
手机号码
标题
留言内容
验证码

金刚石纳米颗粒中氮空位色心的电子自旋研究

刘东奇 常彦春 刘刚钦 潘新宇

引用本文:
Citation:

金刚石纳米颗粒中氮空位色心的电子自旋研究

刘东奇, 常彦春, 刘刚钦, 潘新宇

Electron spin studies of nitrogen vacancy centers in nanodiamonds

Liu Dong-Qi, Chang Yan-Chun, Liu Gang-Qin, Pan Xin-Yu
PDF
导出引用
  • 通过电子注入的方法制备了含氮空位色心单光子源的金刚石荧光纳米颗粒. 自旋回声测试结果表明, 纳米颗粒中氮空位色心的相干时间T2很短, 介于0.86 s至5.6 s之间. Ramsey干涉条纹测试结果表明, 氮空位色心NV1点的退相干时间T2* 最大, 为0.7 s, 其电子自旋共振谱可分辨的最小线宽为1.05 MHz. 并且NV1点的电子自旋共振谱可分辨氮空位色心本身的14N核自旋与 氮空位色心电子自旋之间的2.2 MHz超精细相互作用, 这对于在金刚石纳米颗粒中实现核自旋的操控和多个量子比特的门操作具有重要意义.
    Fluorescent nanodiamonds containing nitrogen vacancy centers are created by electron irradiation. The values of spin echo coherence time T2 of nitrogen vacancy centers in nanodiamonds are very small, which are between 0.86 s and 5.6 s. The results of Ramsey interference fringes show that the values of dephasing time T2* differ from each other and the T2* of nitrogen vacancy center NV1 is biggest (0.7 s). Its inhomogeneous linewidth obtained from Fourier transform frequency spectrum of Ramsey interference fringes is 1.05 MHz. The hyperfine structure for the nitrogen vacancy center electron spin coupled to the host nitrogen-14 nuclear spin can be detected by the electron spin resonance spectrum in nitrogen vacancy center NV1. It is important for the realization of the manipulation of nuclear spins and quantum gates of multiqubit in nanodiamonds.
    • 基金项目: 国家重点基础研究发展计划(批准号: 2009CB929103)和国家自然科学基金(批准号: 10974251)资助的课题.
    • Funds: Project supported by the National Basic Research Program of China (Grant No. 2009CB929103) and the National Natural Science Foundation of China (Grant No. 10974251).
    [1]

    Aharonovich I, Castelletto S, Simpson D A, Su C, Greentree A D, Prawer S 2011 Rep. Prog. Phys. 74 076501

    [2]

    Chen Q, Feng M, Du J F, Hai W H 2011 Chin. Phys. B 20 010308

    [3]

    Puzyr A P, Baron A V, Purtov K V, Bortnikov E V, Skobelev N N, Moginaya O A, Bondar V S 2007 Diamond Relat. Mater. 16 2124

    [4]

    Hartl A, Schmich E, Garrido J A, Hernando J, Catharino S C R, Walter S, Feulner P, Kromka A, Steinmuller D, Stutzmann M 2004 Nat. Mater. 3 736

    [5]

    Krueger A 2008 Chem. Eur. J. 14 1382

    [6]

    Maze J R, Stanwix P L, Hodges J S, Hong S, Taylor J M, Cappellaro P, Jiang L, Gurudev Dutt M V, Togan E, Zibrov A S, Yacoby A, Walsworth R L, Lukin M D 2008 Nature 455 644

    [7]

    Balasubramanian G, Chan I Y, Kolesov R, Al-Hmoud M, Tisler J, Shin C, Kim C, Wojcik A, Hemmer P R, Krueger A, Hanke T, Leitenstorfer A, Bratschitsch R, Jelezko F, Wrachtrup J 2008 Nature 455 648

    [8]

    Taylor J M, Cappellaro P, Childress L, Jiang L, Budker D, Hemmer P R, Yacoby A, Walsworth R, Lukin M D 2008 Nat. Phys. 4 810

    [9]

    Rondin L, Tetienne J P, Spinicelli P, Dal Savio C, Karrai K, Dantelle G, Thiaville A, Rohart S, Roch J F, Jacques V 2012 Appl. Phys. Lett. 100 153118

    [10]

    Shi F, Rong X, Xu N, Wang Y, Wu J, Chong B, Peng X H, Kniepert J, Schoenfeld R S, Harneit W, Feng M, Du J F 2010 Phys. Rev. Lett. 105 040504

    [11]

    Pan X Y, Liu G Q, Yang L L, Fan H 2011 Appl. Phys. Lett. 99 051113

    [12]

    Chang Y C, Liu G Q, Liu D Q, Fan H, Pan X Y 2013 Sci. Rep. 3 1498

    [13]

    Kolesov R, Grotz B, Balasubramanian G, Stohr R J, Nicolet A A L, Hemmer P R, Jelezko F, Wrachtrup J 2009 Nat. Phys. 5 470

    [14]

    Lassen E A, Simpson D A, Gibson B C, Trpkovski S, Hossain F M, Huntington S T, Ganesan K, Hollenberg L C, Prawer S 2011 Opt. Express 17 9588

    [15]

    Marcos D, Wubs M, Taylor J M, Aguado R, Lukin M D, Sorensen A S 2010 Phys. Rev. Lett. 105 210501

    [16]

    Schrand A M, Hens S A C, Shenderova O A 2009 Crit. Rev. Solid State Mater. Sci. 34 18

    [17]

    Wang K Y, Li Z H, Gao K, Zhu Y M 2012 Acta Phys. Sin. 61 097803 (in Chinese) [王凯悦, 李志宏, 高凯, 朱玉梅 2012 物理学报 61 097803]

    [18]

    Hu X, Liu D Q, Pan X Y 2011 Chin. Phys. B 20 117801

    [19]

    Gruber A, Drabenstedt A, Tietz C, Fleury L, Wrachtrup J, von Borczyskowski C 1997 Science 276 2012

    [20]

    Vandersypen L M K, Chuang I L 2005 Rev. Mod. Phys. 76 1037

    [21]

    Cui J M, Chen X D, Fan L L, Gong Z J, Zou C W, Sun F W, Han Z F, Guo G C 2012 Chin. Phys. Lett. 29 036103

    [22]

    Scully M O, Zubairy M S 1997 Quantum Optics (UK, Cambrige: Cambridge University Press)

    [23]

    Ryan C A, Hodges J S, Cory D G 2010 Phys. Rev. Lett. 105 200402

    [24]

    Rondin L, Dantelle G, Slablab A, Grosshans F, Treussart F, Bergonzo P, Perruchas S, Gacoin T, Chaigneau M, Chang H C, Jacques V, Roch J F 2010 Phys. Rev. B 82 115449

    [25]

    Tisler J, Balasubramanian G, Naydenov B, Kolesov R, Grotz B, Reuter R, Boudou J P, Curmi P A, Sennour M, Thorel A, Borsch M, Aulenbacher K, Erdmann R, Hemmer P R, Jelezko F, Wrachtrup J 2009 ACS Nano 3 1959

    [26]

    Laraoui A, Hodges J S, Meriles C A 2012 Nano Lett. 12 3477

    [27]

    Hanson R, Dobrovitski V V, Feiguin A E, Gywat O, Awschalom D D 2008 Science 320 352

    [28]

    Dreau A, Lesik M, Rondin L, Spinicelli P, Arcizet O, Roch J F, Jacques V 2011 Phys. Rev. B 84 195204

    [29]

    Rabeau J R, Reichart P, Wrachtrup J 2006 Appl. Phys. Lett. 88 023113

    [30]

    Smeltzer B, Childress L, Gali A 2011 New J. Phys. 13 025021

    [31]

    Steiner M, Neumann P, Beck J, Jelezko F, Wrachtrup J 2010 Phys. Rev. B 81 035205

    [32]

    Fuchs G D, Dobrovitski V V, Toyli D M, Heremans F J, Awschalom D D 2009 Science 326 1520

    [33]

    Hahn E L 1950 Phys. Rev. 80 580

    [34]

    Lange G D, Wang Z, Riste D, Dobrovitski V, Hanson R 2010 Science 330 60

    [35]

    Childress L, Gurudev Dutt M V, Taylor J M, Zibrov A S, Jelezko F, Wrachtrup J, Hemmer P R, Lukin M D 2006 Science 314 281

    [36]

    Jahnke K D, Naydenov B, Teraji T, Koizumi S, Umeda T, Isoya J, Jelezko F 2012 Appl. Phys. Lett. 101 012405

    [37]

    Boudou J, Curmi P, Jelezko F, Wrachtrup J, Aubert P, Sennour M, Balasubramanian G, Reuter R, Thorel A, Gaffet E 2009 Nanotechnology 20 235602

  • [1]

    Aharonovich I, Castelletto S, Simpson D A, Su C, Greentree A D, Prawer S 2011 Rep. Prog. Phys. 74 076501

    [2]

    Chen Q, Feng M, Du J F, Hai W H 2011 Chin. Phys. B 20 010308

    [3]

    Puzyr A P, Baron A V, Purtov K V, Bortnikov E V, Skobelev N N, Moginaya O A, Bondar V S 2007 Diamond Relat. Mater. 16 2124

    [4]

    Hartl A, Schmich E, Garrido J A, Hernando J, Catharino S C R, Walter S, Feulner P, Kromka A, Steinmuller D, Stutzmann M 2004 Nat. Mater. 3 736

    [5]

    Krueger A 2008 Chem. Eur. J. 14 1382

    [6]

    Maze J R, Stanwix P L, Hodges J S, Hong S, Taylor J M, Cappellaro P, Jiang L, Gurudev Dutt M V, Togan E, Zibrov A S, Yacoby A, Walsworth R L, Lukin M D 2008 Nature 455 644

    [7]

    Balasubramanian G, Chan I Y, Kolesov R, Al-Hmoud M, Tisler J, Shin C, Kim C, Wojcik A, Hemmer P R, Krueger A, Hanke T, Leitenstorfer A, Bratschitsch R, Jelezko F, Wrachtrup J 2008 Nature 455 648

    [8]

    Taylor J M, Cappellaro P, Childress L, Jiang L, Budker D, Hemmer P R, Yacoby A, Walsworth R, Lukin M D 2008 Nat. Phys. 4 810

    [9]

    Rondin L, Tetienne J P, Spinicelli P, Dal Savio C, Karrai K, Dantelle G, Thiaville A, Rohart S, Roch J F, Jacques V 2012 Appl. Phys. Lett. 100 153118

    [10]

    Shi F, Rong X, Xu N, Wang Y, Wu J, Chong B, Peng X H, Kniepert J, Schoenfeld R S, Harneit W, Feng M, Du J F 2010 Phys. Rev. Lett. 105 040504

    [11]

    Pan X Y, Liu G Q, Yang L L, Fan H 2011 Appl. Phys. Lett. 99 051113

    [12]

    Chang Y C, Liu G Q, Liu D Q, Fan H, Pan X Y 2013 Sci. Rep. 3 1498

    [13]

    Kolesov R, Grotz B, Balasubramanian G, Stohr R J, Nicolet A A L, Hemmer P R, Jelezko F, Wrachtrup J 2009 Nat. Phys. 5 470

    [14]

    Lassen E A, Simpson D A, Gibson B C, Trpkovski S, Hossain F M, Huntington S T, Ganesan K, Hollenberg L C, Prawer S 2011 Opt. Express 17 9588

    [15]

    Marcos D, Wubs M, Taylor J M, Aguado R, Lukin M D, Sorensen A S 2010 Phys. Rev. Lett. 105 210501

    [16]

    Schrand A M, Hens S A C, Shenderova O A 2009 Crit. Rev. Solid State Mater. Sci. 34 18

    [17]

    Wang K Y, Li Z H, Gao K, Zhu Y M 2012 Acta Phys. Sin. 61 097803 (in Chinese) [王凯悦, 李志宏, 高凯, 朱玉梅 2012 物理学报 61 097803]

    [18]

    Hu X, Liu D Q, Pan X Y 2011 Chin. Phys. B 20 117801

    [19]

    Gruber A, Drabenstedt A, Tietz C, Fleury L, Wrachtrup J, von Borczyskowski C 1997 Science 276 2012

    [20]

    Vandersypen L M K, Chuang I L 2005 Rev. Mod. Phys. 76 1037

    [21]

    Cui J M, Chen X D, Fan L L, Gong Z J, Zou C W, Sun F W, Han Z F, Guo G C 2012 Chin. Phys. Lett. 29 036103

    [22]

    Scully M O, Zubairy M S 1997 Quantum Optics (UK, Cambrige: Cambridge University Press)

    [23]

    Ryan C A, Hodges J S, Cory D G 2010 Phys. Rev. Lett. 105 200402

    [24]

    Rondin L, Dantelle G, Slablab A, Grosshans F, Treussart F, Bergonzo P, Perruchas S, Gacoin T, Chaigneau M, Chang H C, Jacques V, Roch J F 2010 Phys. Rev. B 82 115449

    [25]

    Tisler J, Balasubramanian G, Naydenov B, Kolesov R, Grotz B, Reuter R, Boudou J P, Curmi P A, Sennour M, Thorel A, Borsch M, Aulenbacher K, Erdmann R, Hemmer P R, Jelezko F, Wrachtrup J 2009 ACS Nano 3 1959

    [26]

    Laraoui A, Hodges J S, Meriles C A 2012 Nano Lett. 12 3477

    [27]

    Hanson R, Dobrovitski V V, Feiguin A E, Gywat O, Awschalom D D 2008 Science 320 352

    [28]

    Dreau A, Lesik M, Rondin L, Spinicelli P, Arcizet O, Roch J F, Jacques V 2011 Phys. Rev. B 84 195204

    [29]

    Rabeau J R, Reichart P, Wrachtrup J 2006 Appl. Phys. Lett. 88 023113

    [30]

    Smeltzer B, Childress L, Gali A 2011 New J. Phys. 13 025021

    [31]

    Steiner M, Neumann P, Beck J, Jelezko F, Wrachtrup J 2010 Phys. Rev. B 81 035205

    [32]

    Fuchs G D, Dobrovitski V V, Toyli D M, Heremans F J, Awschalom D D 2009 Science 326 1520

    [33]

    Hahn E L 1950 Phys. Rev. 80 580

    [34]

    Lange G D, Wang Z, Riste D, Dobrovitski V, Hanson R 2010 Science 330 60

    [35]

    Childress L, Gurudev Dutt M V, Taylor J M, Zibrov A S, Jelezko F, Wrachtrup J, Hemmer P R, Lukin M D 2006 Science 314 281

    [36]

    Jahnke K D, Naydenov B, Teraji T, Koizumi S, Umeda T, Isoya J, Jelezko F 2012 Appl. Phys. Lett. 101 012405

    [37]

    Boudou J, Curmi P, Jelezko F, Wrachtrup J, Aubert P, Sennour M, Balasubramanian G, Reuter R, Thorel A, Gaffet E 2009 Nanotechnology 20 235602

  • [1] 刘旺旺, 张克学, 王军, 夏国栋. 过渡区内纳米颗粒的曳力特性模拟研究. 物理学报, 2024, 73(7): 075101. doi: 10.7498/aps.73.20231861
    [2] 何健, 贾燕伟, 屠菊萍, 夏天, 朱肖华, 黄珂, 安康, 刘金龙, 陈良贤, 魏俊俊, 李成明. 碳离子注入金刚石制备氮空位色心的机理. 物理学报, 2022, 71(18): 188102. doi: 10.7498/aps.71.20220794
    [3] 马奥杰, 陈颂佳, 李玉秀, 陈颖. 纳米颗粒布朗扩散边界条件的分子动力学模拟. 物理学报, 2021, 70(14): 148201. doi: 10.7498/aps.70.20202240
    [4] 崔杰, 苏俊杰, 王军, 夏国栋, 李志刚. 自由分子区内纳米颗粒的热泳力计算. 物理学报, 2021, 70(5): 055101. doi: 10.7498/aps.70.20201629
    [5] 田宇, 林子栋, 王翔宇, 车良宇, 鲁大为. 基于自旋体系的量子机器学习实验进展. 物理学报, 2021, 70(14): 140305. doi: 10.7498/aps.70.20210684
    [6] 张旋, 张天赐, 葛际江, 蒋平, 张贵才. 表面活性剂对气-液界面纳米颗粒吸附规律的影响. 物理学报, 2020, 69(2): 026801. doi: 10.7498/aps.69.20190756
    [7] 冯园耀, 李中豪, 张扬, 崔凌霄, 郭琦, 郭浩, 温焕飞, 刘文耀, 唐军, 刘俊. 固态金刚石氮空位色心光学调控优化. 物理学报, 2020, 69(14): 147601. doi: 10.7498/aps.69.20200072
    [8] 李鑫, 黄忠梅, 刘世荣, 彭鸿雁, 黄伟其. 掺氧纳米硅局域态中的电子自旋能级展宽效应. 物理学报, 2020, 69(17): 174206. doi: 10.7498/aps.69.20200336
    [9] 张淑亭, 孙志, 赵磊. 石墨烯纳米片大自旋特性第一性原理研究. 物理学报, 2018, 67(18): 187102. doi: 10.7498/aps.67.20180867
    [10] 黄丛亮, 冯妍卉, 张欣欣, 李静, 王戈, 侴爱辉. 金属纳米颗粒的热导率. 物理学报, 2013, 62(2): 026501. doi: 10.7498/aps.62.026501
    [11] 徐波, 王树林, 李生娟, 李来强. 超声强化合成MgFe2O4纳米颗粒及其机理研究. 物理学报, 2012, 61(3): 030703. doi: 10.7498/aps.61.030703
    [12] 王新亮, 狄勤丰, 张任良, 丁伟朋, 龚玮, 程毅翀. 纳米颗粒吸附岩心表面的强疏水特征. 物理学报, 2012, 61(21): 216801. doi: 10.7498/aps.61.216801
    [13] 臧渡洋, 张永建, Langevin Dominique. SiO2纳米颗粒单层膜流变特性的双Wilhelmy片法研究. 物理学报, 2011, 60(7): 076801. doi: 10.7498/aps.60.076801
    [14] 陈慧敏, 刘恩隆. 纳米颗粒与纳米块材摩尔定压热容的理论计算. 物理学报, 2011, 60(6): 066501. doi: 10.7498/aps.60.066501
    [15] 刘演华, 干富军, 张凯. 平面射流场中纳米颗粒的成核与凝并. 物理学报, 2010, 59(6): 4084-4092. doi: 10.7498/aps.59.4084
    [16] 徐忠锋, 刘丽莉, 赵永涛, 陈亮, 朱键, 王瑜玉, 肖国青. 不同能量的高电荷态Ar12+离子辐照对Au纳米颗粒尺寸的影响. 物理学报, 2009, 58(6): 3833-3838. doi: 10.7498/aps.58.3833
    [17] 陈小雪, 滕利华, 刘晓东, 黄绮雯, 文锦辉, 林位株, 赖天树. InGaN薄膜中电子自旋偏振弛豫的时间分辨吸收光谱研究. 物理学报, 2008, 57(6): 3853-3856. doi: 10.7498/aps.57.3853
    [18] 刘锦宏, 张凌飞, 田庚方, 李济晨, 李发伸. 低温固相反应法制备的NiFe2O4纳米颗粒的结构与磁性. 物理学报, 2007, 56(10): 6050-6055. doi: 10.7498/aps.56.6050
    [19] 李 晖, 谢二庆, 张洪亮, 潘孝军, 张永哲. 火焰喷雾法合成ZnO和MgxZn1-xO纳米颗粒的光学性能研究. 物理学报, 2007, 56(6): 3584-3588. doi: 10.7498/aps.56.3584
    [20] 孟利军, 张凯旺, 钟建新. 硅纳米颗粒在碳纳米管表面生长的分子动力学模拟. 物理学报, 2007, 56(2): 1009-1013. doi: 10.7498/aps.56.1009
计量
  • 文章访问数:  7433
  • PDF下载量:  1083
  • 被引次数: 0
出版历程
  • 收稿日期:  2013-04-16
  • 修回日期:  2013-04-24
  • 刊出日期:  2013-08-05

/

返回文章
返回