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从纳米原子到巨型分子的软物质研究

张文彬 陈尔强 王晶 张维 王林格 程正迪

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从纳米原子到巨型分子的软物质研究

张文彬, 陈尔强, 王晶, 张维, 王林格, 程正迪

Soft matters from nano-atoms to giant molecules

Zhang Wen-Bin, Chen Er-Qiang, Wang Jing, Zhang Wei, Wang Lin-Ge, Cheng Stephen Z. D.
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  • 本文通过分析软物质科学发展的趋势,回顾了纳米原子与巨型分子这类新型软物质材料的发展历程,总结了纳米原子的结构特点以及巨型分子自组装的若干特色,提出将纳米原子作为巨型分子的基本结构子和功能子,以实现模块化的精确结构高分子理性设计与精准合成,并进一步实现其可控组装,调节其多级结构(特别是1-100 nm尺度的结构),最终实现其多样的功能化. 这种具有高度刚性构型和固定形状尺寸的大分子有别于传统大分子的柔性链式结构,在组装中也呈现出了与传统大分子截然不同的有趣相态和相结构,是大分子科学的一类新元素,值得进行深入研究.
    In this brief review, we look back on the conception of nano-atoms and their gradual evolutions into a new class of giant molecules in the context of soft matter science. The structural features and the characteristics about giant molecular self-assembly are summarized. It is found that these giant molecules with high conformational rigidities and precisely-defined shapes and symmetries can exhibit unusual phase structures and phase transition behaviors which are not commonly observed in conventional polymers. Their self-assembly is robust due to collective and cooperative interactions among nano-atoms, forming hierarchical structures that are sensitive to their primary structures. This modular feature is reminiscent to the domain concept in protein science. It is thus proposed that nano-atoms can serve as unique elements for macromolecular science.
      通信作者: 张文彬, wenbin@pku.edu.cn;scheng@uakron.edu ; 程正迪, wenbin@pku.edu.cn;scheng@uakron.edu
    • 基金项目: 国家自然科学基金(批准号:21674003,21474003,91427304)、国家高技术研究发展计划(批准号:2015AA020941)和NSF of USA(批准号:DMR-1409972,DMR-0906898)资助的课题.
      Corresponding author: Zhang Wen-Bin, wenbin@pku.edu.cn;scheng@uakron.edu ; Cheng Stephen Z. D., wenbin@pku.edu.cn;scheng@uakron.edu
    • Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 21674003, 21474003, 91427304), the National High Technology Research and Development Program of China (Grant No. 2015AA020941), and the National Science Foundation of USA (Grant Nos. DMR-1409972, DMR-0906898).
    [1]

    Ouyang Z C 2000 Soft Matters-Scientific Frontiers at the Crossroad of Physics, Chemistry, and Biology at 21st Century (Changsha: Hunan Education Publishing House) (in Chinese) [欧阳钟灿 2000 软物质21世纪跨物理、化学、生物三大学科的前沿科学 (长沙: 湖南教育出版社)]

    [2]

    Hamley I W 2007 Introduction to Soft Matter: Synthetic and Biological Self-assembling Materials (Rev. Ed.) (Chichester, England: John Wiley Sons)

    [3]

    Degennes P G 1992 Angew. Chem. Int. Ed. 31 842

    [4]

    Doi M 2013 Soft Matter Physics (1st Ed.) (Oxford, UK, Oxford University Press)

    [5]

    Cheng S Z D 2005 J. Polym. Sci. Part B: Polym. Phys. 43 3361

    [6]

    Cheng S Z D 2008 Phase Transitions in Polymers: The Role of Metastable States (1st) (Amsterdam, Boston: Elsevier)

    [7]

    Feynman R P 1960 Eng. Sci. 23 22

    [8]

    Zhang W B, Cheng S Z D 2015 Chin. J. Polym. Sci. 33 797

    [9]

    Zhang W B, Yu X, Wang C L, Sun H J, Hsieh I F, Li Y, Dong X H, Yue K, van Horn R, Cheng S Z D 2014 Macromolecules 47 1221

    [10]

    Kastner M A 1993 Phys. Today 46 24

    [11]

    Tomalia D A, Christensen J B, Boas U 2012 Dendrimers, Dendrons, and Dendritic Polymers: Discovery, Application, and the Future (Cambridge, UK: Cambridge University Press)

    [12]

    Tomalia D A, Jensen A 2007 Periodic Patterns, Relationships and Categories of Well-Defined Nanoscale Building Blocks (National Science Foundation Workshop Report)

    [13]

    Roy X, Lee C H, Crowther A C, Schenck C L, Besara T, Lalancette R A, Siegrist T, Stephens P W, Brus L E, Kim P, Steigerwald M L, Nuckolls C 2013 Science 341 157

    [14]

    Luo Z, Castleman A W 2014 Acc. Chem. Res. 47 2931

    [15]

    Nimmala P R, Knoppe S, Jupally V R, Delcamp J H, Aikens C M, Dass A 2014 J. Phys. Chem. B 118 14157

    [16]

    Wu K, Huang M, Yue K, Liu C, Lin Z, Liu H, Zhang W, Hsu C H, Shi A C, Zhang W B, Cheng S Z D 2014 Macromolecules 47 4622

    [17]

    Yu X, Zhong S, Li X, Tu Y, Yang S, van Horn R M, Ni C, Pochan D J, Quirk R P, Wesdemiotis C, Zhang W B, Cheng S Z D 2010 J. Am. Chem. Soc. 132 16741

    [18]

    Wang Z, Li Y, Dong X H, Yu X, Guo K, Su H, Yue K, Wesdemiotis C, Cheng S Z D, Zhang W B 2013 Chem. Sci. 4 1345

    [19]

    Zhang WB, Tu Y, Ranjan R, van Horn R M, Leng S, Wang J, Polce M, Wesdemiotis C, Quirk R P, Newkome G R, Cheng S Z D 2008 Macromolecules 41 515

    [20]

    Yu X, Li Y, Dong X H, Yue K, Lin Z, Feng X, Huang M, Zhang W B, Cheng S Z D 2014 J. Polym. Sci. Part B: Polym. Phys. 52 1309

    [21]

    Huang M, Hsu C H, Wang J, Mei S, Dong X, Li Y, Li M, Liu H, Zhang W, Aida T, Zhang W B, Yue K, Cheng S Z D 2015 Science 348 424

    [22]

    Li Y, Zhang W B, Hsieh I F, Zhang G, Cao Y, Li X, Wesdemiotis C, Lotz B, Xiong H, Cheng S Z D 2011 J. Am. Chem. Soc. 133 10712

    [23]

    Lin M C, Hsu C H, Sun H J, Wang C L, Zhang W B, Li Y, Chen H L, Cheng S Z D 2014 Polymer 55 4514

    [24]

    Cesareni G 2005 Modular Protein Domains (Weinheim: Wiley-VCH)

    [25]

    Zhang W B 2010 Ph. D. Dissertation (Akron, OH: University of Akron)

    [26]

    Zhang W B, Wang X M, Wang X W, Liu D, Han S Y, Cheng S Z D 2015 Prog. Chem. 27 1333

    [27]

    Corey E J 1967 Pure Appl. Chem. 14 19

    [28]

    Corey E J, Cheng X M 1989 The Logic of Chemical Synthesis (New York: Wiley)

    [29]

    Desiraju G R 1995 Angew. Chem. Int. Ed. 34 2311

    [30]

    Desiraju G R 2003 J. Mol. Struct. 656 5

    [31]

    Arnold F H 1998 Acc. Chem. Res. 31 125

    [32]

    Romero P A, Arnold F H 2009 Nat. Rev. Mol. Cell Biol. 10 866

    [33]

    Ober C K, Cheng S Z D, Hammond P T, Muthukumar M, Reichmains E, Wooley K L, Lodge T P 2009 Macrmolecules 42 465

    [34]

    Feng X, Zhu S, Yue K, Su H, Guo K, Wesdemiotis C, Zhang W B, Cheng S Z D, Li Y 2014 ACS Macro Lett. 3 900

    [35]

    Hirsch A, Brettreich M 2005 Fullerenes: Chemistry and Reactions (Weinheim: Wiley-VCH)

    [36]

    Wang X M, Guo Q Y, Han S Y, Wang J Y, Han D, Fu Q, Zhang W B 2015 Chem. Eur. J. 21 15246

    [37]

    Han S Y, Wang X M, Shao Y, Guo Q Y, Li Y, Zhang W B 2016 Chem. Eur. J. 22 6397

    [38]

    Shao Y, Yin H, Wang X M, Han S Y, Yan X, Xu J, He J, Ni P, Zhang W B 2016 Polym. Chem. 7 2381

    [39]

    Oguri N E Y, Takeda N, Unno M 2016 Angew. Chem. Int. Ed. 55 DOI: 10.1002/anie.201602413

    [40]

    Blazquez-Moraleja A, Eugenia Perez-Ojeda M, Suarez J R, Luisa Jimeno M, Chiara J L 2016 Chem. Commun. 52 5792

    [41]

    Kolb H C, Finn M G, Sharpless K B 2001 Angew. Chem. Int. Ed. 40 2004

    [42]

    Iha R K, Wooley K L, Nystrom A M, Burke D J, Kade M J, Hawker C J 2009 Chem. Rev. 109 5620

    [43]

    Barner-Kowollik C, Du Prez F E, Espeel P, Hawker C J, Junkers T, Schlaad H, van Camp W 2011 Angew. Chem. Int. Ed. 50 60

    [44]

    Li Y, Wang Z, Zheng J, Su H, Lin F, Guo K, Feng X, Wesdemiotis C, Becker M L, Cheng S Z D, Zhang W B 2013 ACS Macro Lett. 2 1026

    [45]

    Xi W, Scott T F, Kloxin C J, Bowman C N 2014 Adv. Funct. Mater. 24 2572

    [46]

    Sletten E M, Bertozzi C R 2009 Angew. Chem. Int. Ed. 48 6974

    [47]

    Hoyle C E, Bowman C N 2010 Angew. Chem. Int. Ed. 49 1540

    [48]

    Li Y, Zhang W B, Janoski J E, Li X, Dong X, Wesdemiotis C, Quirk R P, Cheng S Z D 2011 Macromolecules 44 3328

    [49]

    Li Y, Su H, Feng X, Wang Z, Guo K, Wesdemiotis C, Fu Q, Cheng S Z D, Zhang W B 2014 Polym. Chem. 5 6111

    [50]

    Zhang W B, Li Y, Li X, Dong X, Yu X, Wang C L, Wesdemiotis C, Quirk R P, Cheng S Z D 2011 Macromolecules 44 2589

    [51]

    Li Y, Guo K, Su H, Li X, Feng X, Wang Z, Zhang W, Zhu S, Wesdemiotis C, Cheng S Z D, Zhang W B 2014 Chem. Sci. 5 1046

    [52]

    Yue K, Liu C, Guo K, Yu X, Huang M, Li Y, Wesdemiotis C, Cheng S Z D, Zhang W B 2012 Macromolecules 45 8126

    [53]

    Su H, Li Y, Yue K, Wang Z, Lu P, Feng X, Dong X H, Zhang S, Cheng S Z D, Zhang W B 2014 Polym. Chem. 5 3697

    [54]

    Li Y, Su H, Feng X, Yue K, Wang Z, Lin Z, Zhu X, Fu Q, Zhang Z, Cheng S Z D, Zhang W B 2015 Polym. Chem. 6 827

    [55]

    Lin Z, Lu P, Yu X, Zhang W B, Huang M, Wu K, Guo K, Wesdemiotis C, Zhu X, Zhang Z, Yue K, Cheng S Z D 2014 Macromolecules 47 4160

    [56]

    Li Y, Dong X H, Guo K, Wang Z, Chen Z, Wesdemiotis C, Quirk R P, Zhang W B, Cheng S Z D 2012 ACS Macro Lett. 1 834

    [57]

    Zhang W, Huang M, Su H, Zhang S, Yue K, Dong X H, Li X, Liu H, Zhang S, Wesdemiotis C, Lotz B, Zhang W B, Li Y, Cheng S Z D 2016 ACS Cent. Sci. 2 48

    [58]

    Yue K, Liu C, Guo K, Wu K, Dong X H, Liu H, Huang M, Wesdemiotis C, Cheng S Z D, Zhang W B 2013 Polym. Chem. 4 1056

    [59]

    Yu X, Yue K, Hsieh I F, Li Y, Dong X H, Liu C, Xin Y, Wang H F, Shi A C, Newkome G R, Ho R M, Chen E Q, Zhang W B, Cheng S Z D 2013 Proc. Natl. Acad. Sci. USA 110 10078

    [60]

    Ni B, Huang M, Chen Z, Chen Y, Hsu C H, Li Y, Pochan D, Zhang W B, Cheng S Z D, Dong X H 2015 J. Am. Chem. Soc. 137 1392

    [61]

    Liu H, Hsu C H, Lin Z, Shan W, Wang J, Jiang J, Huang M, Lotz B, Yu X, Zhang W B, Yue K, Cheng S Z D 2014 J. Am. Chem. Soc. 136 10691

    [62]

    Liu H, Luo J, Shan W, Guo D, Wang J, Hsu C H, Huang M, Zhang W, Lotz B, Zhang W B, Liu T, Yue K, Cheng S Z D 2016 ACS Nano DOI: 10.1021/acsnano.6b01336

    [63]

    Fierer J O, Veggiani G, Howarth M 2014 Proc. Natl. Acad. Sci. USA 111 E1176

    [64]

    Veggiani G, Nakamura T, Brenner M D, Gayet R V, Yan J, Robinson C V, Howarth M 2016 Proc. Natl. Acad. Sci. USA 113 1202

    [65]

    Zakeri B, Fierer J O, Celik E, Chittock E C, Schwarz-Linek U, Moy V T, Howarth M 2012 Proc. Natl. Acad. Sci. USA 109 E690

    [66]

    Reddington S C, Howarth M 2015 Curr. Opin. Chem. Biol. 29 94

    [67]

    Veggiani G, Zakeri B, Howarth M 2014 Trends Biotechnol. 32 506

    [68]

    Zhang W B, Sun F, Tirrell D A, Arnold F H 2013 J. Am. Chem. Soc. 135 13988

    [69]

    Sun F, Zhang W B, Mahdavi A, Arnold F H, Tirrell D A 2014 Proc. Natl. Acad. Sci. USA 111 11269

    [70]

    Wang X W, Zhang W B 2016 Angew. Chem. Int. Ed. 55 3442

    [71]

    Liu Z, Zhou H, Wang W, Tan W, Fu Y X, Zhu M 2014 Sci. Rep. 4 7266

    [72]

    Schoene C, Fierer J O, Bennett S P, Howarth M 2014 Angew. Chem. Int. Ed. 53

    [73]

    Wang Y, Lin H X, Chen L, Ding S Y, Lei Z C, Liu D Y, Cao X Y, Liang H J, Jiang Y B, Tian Z Q 2014 Chem. Soc. Rev. 43 399

    [74]

    Wang Y, Lin H X, Ding S Y, Liu D Y, Chen L, Lei Z C, Fan F R, Tian Z Q 2012 Sci. Chin. Chem. 42 525

    [75]

    Sun H J, Tu Y, Wang C L, van Horn R M, Tsai C C, Graham M J, Sun B, Lotz B, Zhang W B, Cheng S Z D 2011 J. Mater. Chem. 21 14240

    [76]

    Ren X, Sun B, Tsai C C, Tu Y, Leng S, Li K, Kang Z, van Horn R M, Li X, Zhu M, Wesdemiotis C, Zhang W B, Cheng S Z D 2010 J. Phys. Chem. B 114 4802

    [77]

    Wang C L, Zhang W B, Sun H J, van Horn R M, Kulkarni R R, Tsai C C, Hsu C S, Lotz B, Gong X, Cheng S Z D 2012 Adv. Energy Mater. 2 1375

    [78]

    Dong X H, van Horn R, Chen Z, Ni B, Yu X, Wurm A, Schick C, Lotz B, Zhang W B, Cheng S Z D 2013 J. Phys. Chem. Lett. 4 2356

    [79]

    Cheng S Z D, Zhang A, Chen J, Heberer D P 1991 J. Polym. Sci. Part B: Polym. Phys. 29 287

    [80]

    Cheng S Z D, Zhang A, Barley J S, Chen J, Habenschuss A, Zschack P R 1991 Macromolecules 24 3937

    [81]

    He J, Yue K, Liu Y, Yu X, Ni P, Cavicchi K A, Quirk R P, Chen E Q, Cheng S Z D, Zhang W B 2012 Polym. Chem. 3 2112

    [82]

    Ni B, Dong X H, Chen Z, Lin Z, Li Y, Huang M, Fu Q, Cheng S Z D, Zhang W B 2014 Polym. Chem. 5 3588

    [83]

    Lin Z, Lu P, Hsu C H, Sun J, Zhou Y, Huang M, Yue K, Ni B, Dong X H, Li X, Zhang W B, Yu X, Cheng S Z D 2015 Macromolecules 48 5496

    [84]

    Hsu C H, Dong X H, Lin Z, Ni B, Lu P, Jiang Z, Tian D, Shi A C, Thomas E L, Cheng S Z D 2016 ACS Nano 10 919

    [85]

    Dong X H, Ni B, Huang M, Hsu C H, Chen Z, Lin Z, Zhang W B, Shi A C, Cheng S Z D 2015 Macromolecules 48 7172

    [86]

    Dong X H, Ni B, Huang M, Hsu C H, Bai R, Zhang W B, Shi A C, Cheng S Z D 2016 Angew. Chem. Int. Ed. 55 2459

    [87]

    Yu X, Zhang W B, Yue K, Li X, Liu H, Xin Y, Wang C L, Wesdemiotis C, Cheng S Z D 2012 J. Am. Chem. Soc. 134 7780

    [88]

    Lin Z, Lu P, Hsu C H, Yue K, Dong X H, Liu H, Guo K, Wesdemiotis C, Zhang W B, Yu X, Cheng S Z D 2014 Chem. Eur. J. 20 11630

    [89]

    Dong X H, Hsu C H, Li Y, Liu H, Wang J, Huang M, Yue K, Sun H J, Wang C L, Yu X, Zhang W B, Lotz B, Cheng S Z D 2016 Adv. Polym. Sci. DOI: 10.1007/122015343

    [90]

    National Science and Technology Council 2011 Materials Genome Initiative for Global Competitiveness (Washington DC: National Science and Technology Council)

  • [1]

    Ouyang Z C 2000 Soft Matters-Scientific Frontiers at the Crossroad of Physics, Chemistry, and Biology at 21st Century (Changsha: Hunan Education Publishing House) (in Chinese) [欧阳钟灿 2000 软物质21世纪跨物理、化学、生物三大学科的前沿科学 (长沙: 湖南教育出版社)]

    [2]

    Hamley I W 2007 Introduction to Soft Matter: Synthetic and Biological Self-assembling Materials (Rev. Ed.) (Chichester, England: John Wiley Sons)

    [3]

    Degennes P G 1992 Angew. Chem. Int. Ed. 31 842

    [4]

    Doi M 2013 Soft Matter Physics (1st Ed.) (Oxford, UK, Oxford University Press)

    [5]

    Cheng S Z D 2005 J. Polym. Sci. Part B: Polym. Phys. 43 3361

    [6]

    Cheng S Z D 2008 Phase Transitions in Polymers: The Role of Metastable States (1st) (Amsterdam, Boston: Elsevier)

    [7]

    Feynman R P 1960 Eng. Sci. 23 22

    [8]

    Zhang W B, Cheng S Z D 2015 Chin. J. Polym. Sci. 33 797

    [9]

    Zhang W B, Yu X, Wang C L, Sun H J, Hsieh I F, Li Y, Dong X H, Yue K, van Horn R, Cheng S Z D 2014 Macromolecules 47 1221

    [10]

    Kastner M A 1993 Phys. Today 46 24

    [11]

    Tomalia D A, Christensen J B, Boas U 2012 Dendrimers, Dendrons, and Dendritic Polymers: Discovery, Application, and the Future (Cambridge, UK: Cambridge University Press)

    [12]

    Tomalia D A, Jensen A 2007 Periodic Patterns, Relationships and Categories of Well-Defined Nanoscale Building Blocks (National Science Foundation Workshop Report)

    [13]

    Roy X, Lee C H, Crowther A C, Schenck C L, Besara T, Lalancette R A, Siegrist T, Stephens P W, Brus L E, Kim P, Steigerwald M L, Nuckolls C 2013 Science 341 157

    [14]

    Luo Z, Castleman A W 2014 Acc. Chem. Res. 47 2931

    [15]

    Nimmala P R, Knoppe S, Jupally V R, Delcamp J H, Aikens C M, Dass A 2014 J. Phys. Chem. B 118 14157

    [16]

    Wu K, Huang M, Yue K, Liu C, Lin Z, Liu H, Zhang W, Hsu C H, Shi A C, Zhang W B, Cheng S Z D 2014 Macromolecules 47 4622

    [17]

    Yu X, Zhong S, Li X, Tu Y, Yang S, van Horn R M, Ni C, Pochan D J, Quirk R P, Wesdemiotis C, Zhang W B, Cheng S Z D 2010 J. Am. Chem. Soc. 132 16741

    [18]

    Wang Z, Li Y, Dong X H, Yu X, Guo K, Su H, Yue K, Wesdemiotis C, Cheng S Z D, Zhang W B 2013 Chem. Sci. 4 1345

    [19]

    Zhang WB, Tu Y, Ranjan R, van Horn R M, Leng S, Wang J, Polce M, Wesdemiotis C, Quirk R P, Newkome G R, Cheng S Z D 2008 Macromolecules 41 515

    [20]

    Yu X, Li Y, Dong X H, Yue K, Lin Z, Feng X, Huang M, Zhang W B, Cheng S Z D 2014 J. Polym. Sci. Part B: Polym. Phys. 52 1309

    [21]

    Huang M, Hsu C H, Wang J, Mei S, Dong X, Li Y, Li M, Liu H, Zhang W, Aida T, Zhang W B, Yue K, Cheng S Z D 2015 Science 348 424

    [22]

    Li Y, Zhang W B, Hsieh I F, Zhang G, Cao Y, Li X, Wesdemiotis C, Lotz B, Xiong H, Cheng S Z D 2011 J. Am. Chem. Soc. 133 10712

    [23]

    Lin M C, Hsu C H, Sun H J, Wang C L, Zhang W B, Li Y, Chen H L, Cheng S Z D 2014 Polymer 55 4514

    [24]

    Cesareni G 2005 Modular Protein Domains (Weinheim: Wiley-VCH)

    [25]

    Zhang W B 2010 Ph. D. Dissertation (Akron, OH: University of Akron)

    [26]

    Zhang W B, Wang X M, Wang X W, Liu D, Han S Y, Cheng S Z D 2015 Prog. Chem. 27 1333

    [27]

    Corey E J 1967 Pure Appl. Chem. 14 19

    [28]

    Corey E J, Cheng X M 1989 The Logic of Chemical Synthesis (New York: Wiley)

    [29]

    Desiraju G R 1995 Angew. Chem. Int. Ed. 34 2311

    [30]

    Desiraju G R 2003 J. Mol. Struct. 656 5

    [31]

    Arnold F H 1998 Acc. Chem. Res. 31 125

    [32]

    Romero P A, Arnold F H 2009 Nat. Rev. Mol. Cell Biol. 10 866

    [33]

    Ober C K, Cheng S Z D, Hammond P T, Muthukumar M, Reichmains E, Wooley K L, Lodge T P 2009 Macrmolecules 42 465

    [34]

    Feng X, Zhu S, Yue K, Su H, Guo K, Wesdemiotis C, Zhang W B, Cheng S Z D, Li Y 2014 ACS Macro Lett. 3 900

    [35]

    Hirsch A, Brettreich M 2005 Fullerenes: Chemistry and Reactions (Weinheim: Wiley-VCH)

    [36]

    Wang X M, Guo Q Y, Han S Y, Wang J Y, Han D, Fu Q, Zhang W B 2015 Chem. Eur. J. 21 15246

    [37]

    Han S Y, Wang X M, Shao Y, Guo Q Y, Li Y, Zhang W B 2016 Chem. Eur. J. 22 6397

    [38]

    Shao Y, Yin H, Wang X M, Han S Y, Yan X, Xu J, He J, Ni P, Zhang W B 2016 Polym. Chem. 7 2381

    [39]

    Oguri N E Y, Takeda N, Unno M 2016 Angew. Chem. Int. Ed. 55 DOI: 10.1002/anie.201602413

    [40]

    Blazquez-Moraleja A, Eugenia Perez-Ojeda M, Suarez J R, Luisa Jimeno M, Chiara J L 2016 Chem. Commun. 52 5792

    [41]

    Kolb H C, Finn M G, Sharpless K B 2001 Angew. Chem. Int. Ed. 40 2004

    [42]

    Iha R K, Wooley K L, Nystrom A M, Burke D J, Kade M J, Hawker C J 2009 Chem. Rev. 109 5620

    [43]

    Barner-Kowollik C, Du Prez F E, Espeel P, Hawker C J, Junkers T, Schlaad H, van Camp W 2011 Angew. Chem. Int. Ed. 50 60

    [44]

    Li Y, Wang Z, Zheng J, Su H, Lin F, Guo K, Feng X, Wesdemiotis C, Becker M L, Cheng S Z D, Zhang W B 2013 ACS Macro Lett. 2 1026

    [45]

    Xi W, Scott T F, Kloxin C J, Bowman C N 2014 Adv. Funct. Mater. 24 2572

    [46]

    Sletten E M, Bertozzi C R 2009 Angew. Chem. Int. Ed. 48 6974

    [47]

    Hoyle C E, Bowman C N 2010 Angew. Chem. Int. Ed. 49 1540

    [48]

    Li Y, Zhang W B, Janoski J E, Li X, Dong X, Wesdemiotis C, Quirk R P, Cheng S Z D 2011 Macromolecules 44 3328

    [49]

    Li Y, Su H, Feng X, Wang Z, Guo K, Wesdemiotis C, Fu Q, Cheng S Z D, Zhang W B 2014 Polym. Chem. 5 6111

    [50]

    Zhang W B, Li Y, Li X, Dong X, Yu X, Wang C L, Wesdemiotis C, Quirk R P, Cheng S Z D 2011 Macromolecules 44 2589

    [51]

    Li Y, Guo K, Su H, Li X, Feng X, Wang Z, Zhang W, Zhu S, Wesdemiotis C, Cheng S Z D, Zhang W B 2014 Chem. Sci. 5 1046

    [52]

    Yue K, Liu C, Guo K, Yu X, Huang M, Li Y, Wesdemiotis C, Cheng S Z D, Zhang W B 2012 Macromolecules 45 8126

    [53]

    Su H, Li Y, Yue K, Wang Z, Lu P, Feng X, Dong X H, Zhang S, Cheng S Z D, Zhang W B 2014 Polym. Chem. 5 3697

    [54]

    Li Y, Su H, Feng X, Yue K, Wang Z, Lin Z, Zhu X, Fu Q, Zhang Z, Cheng S Z D, Zhang W B 2015 Polym. Chem. 6 827

    [55]

    Lin Z, Lu P, Yu X, Zhang W B, Huang M, Wu K, Guo K, Wesdemiotis C, Zhu X, Zhang Z, Yue K, Cheng S Z D 2014 Macromolecules 47 4160

    [56]

    Li Y, Dong X H, Guo K, Wang Z, Chen Z, Wesdemiotis C, Quirk R P, Zhang W B, Cheng S Z D 2012 ACS Macro Lett. 1 834

    [57]

    Zhang W, Huang M, Su H, Zhang S, Yue K, Dong X H, Li X, Liu H, Zhang S, Wesdemiotis C, Lotz B, Zhang W B, Li Y, Cheng S Z D 2016 ACS Cent. Sci. 2 48

    [58]

    Yue K, Liu C, Guo K, Wu K, Dong X H, Liu H, Huang M, Wesdemiotis C, Cheng S Z D, Zhang W B 2013 Polym. Chem. 4 1056

    [59]

    Yu X, Yue K, Hsieh I F, Li Y, Dong X H, Liu C, Xin Y, Wang H F, Shi A C, Newkome G R, Ho R M, Chen E Q, Zhang W B, Cheng S Z D 2013 Proc. Natl. Acad. Sci. USA 110 10078

    [60]

    Ni B, Huang M, Chen Z, Chen Y, Hsu C H, Li Y, Pochan D, Zhang W B, Cheng S Z D, Dong X H 2015 J. Am. Chem. Soc. 137 1392

    [61]

    Liu H, Hsu C H, Lin Z, Shan W, Wang J, Jiang J, Huang M, Lotz B, Yu X, Zhang W B, Yue K, Cheng S Z D 2014 J. Am. Chem. Soc. 136 10691

    [62]

    Liu H, Luo J, Shan W, Guo D, Wang J, Hsu C H, Huang M, Zhang W, Lotz B, Zhang W B, Liu T, Yue K, Cheng S Z D 2016 ACS Nano DOI: 10.1021/acsnano.6b01336

    [63]

    Fierer J O, Veggiani G, Howarth M 2014 Proc. Natl. Acad. Sci. USA 111 E1176

    [64]

    Veggiani G, Nakamura T, Brenner M D, Gayet R V, Yan J, Robinson C V, Howarth M 2016 Proc. Natl. Acad. Sci. USA 113 1202

    [65]

    Zakeri B, Fierer J O, Celik E, Chittock E C, Schwarz-Linek U, Moy V T, Howarth M 2012 Proc. Natl. Acad. Sci. USA 109 E690

    [66]

    Reddington S C, Howarth M 2015 Curr. Opin. Chem. Biol. 29 94

    [67]

    Veggiani G, Zakeri B, Howarth M 2014 Trends Biotechnol. 32 506

    [68]

    Zhang W B, Sun F, Tirrell D A, Arnold F H 2013 J. Am. Chem. Soc. 135 13988

    [69]

    Sun F, Zhang W B, Mahdavi A, Arnold F H, Tirrell D A 2014 Proc. Natl. Acad. Sci. USA 111 11269

    [70]

    Wang X W, Zhang W B 2016 Angew. Chem. Int. Ed. 55 3442

    [71]

    Liu Z, Zhou H, Wang W, Tan W, Fu Y X, Zhu M 2014 Sci. Rep. 4 7266

    [72]

    Schoene C, Fierer J O, Bennett S P, Howarth M 2014 Angew. Chem. Int. Ed. 53

    [73]

    Wang Y, Lin H X, Chen L, Ding S Y, Lei Z C, Liu D Y, Cao X Y, Liang H J, Jiang Y B, Tian Z Q 2014 Chem. Soc. Rev. 43 399

    [74]

    Wang Y, Lin H X, Ding S Y, Liu D Y, Chen L, Lei Z C, Fan F R, Tian Z Q 2012 Sci. Chin. Chem. 42 525

    [75]

    Sun H J, Tu Y, Wang C L, van Horn R M, Tsai C C, Graham M J, Sun B, Lotz B, Zhang W B, Cheng S Z D 2011 J. Mater. Chem. 21 14240

    [76]

    Ren X, Sun B, Tsai C C, Tu Y, Leng S, Li K, Kang Z, van Horn R M, Li X, Zhu M, Wesdemiotis C, Zhang W B, Cheng S Z D 2010 J. Phys. Chem. B 114 4802

    [77]

    Wang C L, Zhang W B, Sun H J, van Horn R M, Kulkarni R R, Tsai C C, Hsu C S, Lotz B, Gong X, Cheng S Z D 2012 Adv. Energy Mater. 2 1375

    [78]

    Dong X H, van Horn R, Chen Z, Ni B, Yu X, Wurm A, Schick C, Lotz B, Zhang W B, Cheng S Z D 2013 J. Phys. Chem. Lett. 4 2356

    [79]

    Cheng S Z D, Zhang A, Chen J, Heberer D P 1991 J. Polym. Sci. Part B: Polym. Phys. 29 287

    [80]

    Cheng S Z D, Zhang A, Barley J S, Chen J, Habenschuss A, Zschack P R 1991 Macromolecules 24 3937

    [81]

    He J, Yue K, Liu Y, Yu X, Ni P, Cavicchi K A, Quirk R P, Chen E Q, Cheng S Z D, Zhang W B 2012 Polym. Chem. 3 2112

    [82]

    Ni B, Dong X H, Chen Z, Lin Z, Li Y, Huang M, Fu Q, Cheng S Z D, Zhang W B 2014 Polym. Chem. 5 3588

    [83]

    Lin Z, Lu P, Hsu C H, Sun J, Zhou Y, Huang M, Yue K, Ni B, Dong X H, Li X, Zhang W B, Yu X, Cheng S Z D 2015 Macromolecules 48 5496

    [84]

    Hsu C H, Dong X H, Lin Z, Ni B, Lu P, Jiang Z, Tian D, Shi A C, Thomas E L, Cheng S Z D 2016 ACS Nano 10 919

    [85]

    Dong X H, Ni B, Huang M, Hsu C H, Chen Z, Lin Z, Zhang W B, Shi A C, Cheng S Z D 2015 Macromolecules 48 7172

    [86]

    Dong X H, Ni B, Huang M, Hsu C H, Bai R, Zhang W B, Shi A C, Cheng S Z D 2016 Angew. Chem. Int. Ed. 55 2459

    [87]

    Yu X, Zhang W B, Yue K, Li X, Liu H, Xin Y, Wang C L, Wesdemiotis C, Cheng S Z D 2012 J. Am. Chem. Soc. 134 7780

    [88]

    Lin Z, Lu P, Hsu C H, Yue K, Dong X H, Liu H, Guo K, Wesdemiotis C, Zhang W B, Yu X, Cheng S Z D 2014 Chem. Eur. J. 20 11630

    [89]

    Dong X H, Hsu C H, Li Y, Liu H, Wang J, Huang M, Yue K, Sun H J, Wang C L, Yu X, Zhang W B, Lotz B, Cheng S Z D 2016 Adv. Polym. Sci. DOI: 10.1007/122015343

    [90]

    National Science and Technology Council 2011 Materials Genome Initiative for Global Competitiveness (Washington DC: National Science and Technology Council)

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  • 收稿日期:  2016-08-02
  • 修回日期:  2016-08-22
  • 刊出日期:  2016-09-05

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