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中国物理学会期刊

拓扑材料BaMnSb2的红外光谱学研究

CSTR: 32037.14.aps.71.20220011

Infrared spectroscopic study of topological material BaMnSb2

CSTR: 32037.14.aps.71.20220011
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  • 对于新型拓扑材料BaMnSb2, 研究了从7 K到常温下温度依赖的宽频红外光谱特性. 随着温度的降低, 绝对反射谱中等离子体极小值有着明显的蓝移, 表明载流子浓度存在随温度变化的行为. 在光电导谱的实部中存在两段随着频率线性增加的响应, 它们的线性外延不经过原点, 表明BaMnSb2的费米能级附近有打开能隙的Dirac型色散. 此外, 在低温下还发现了一段不随频率变化的光电导, 且无法用传统的Drude-Lorentz模型拟合. 因此本文引入了一个恒定的光电导分量, 得到了满意的拟合结果. 通过计算和分析, 我们认为恒定光电导分量可能来自于拓扑材料BaMnSb2的表面态响应.

     

    A detailed infrared optical spectrum of the new topological material BaMnSb2 has been measured at temperatures ranging from 7 K to 295 K. As the temperature decreases, the plasma minimum has a clear blue shift in reflectivity spectrum, indicating that the carrier density changes with temperature. In the real part of the optical conductivity \sigma_1(\omega), two linearly-increased components can be identified, but neither of their extrapolation pass through the origin, which proves that BaMnSb2 has a gapped Dirac dispersion near the Fermi level. Comparing with the theoretical calculation by using first-principles methods, the onset of these two linearly-increased components are in good agreement with the band structures. In addition, a range of constant optical conductivity is found in \sigma_1(\omega), which cannot be described well by the Drude-Lorentz model. Therefore, we introduce a frequency-independent component to fit \sigma_1(\omega) successfully. However, different from the Dirac nodal-line semimetal YbMnSb2 which shares same fitting results as well as crystal structure, the constant component in BaMnSb2 has a small proportion of \sigma_1(\omega). Through calculation and analysis, we attribute the constant component to the surface state of BaMnSb2.

     

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