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阿秒电离动力学作为超快科学的重要研究方向，其关键实验方法与理论模型的突破对于揭示物质的超快演化过程具有重要的科学意义。强场多光子跃迁干涉方法是该领域的前沿技术之一，利用量子路径干涉原理实现对强场多光子电离动力学过程的阿秒时间分辨探测，已广泛应用于从原子到复杂分子体系中量子态分辨的阿秒级电离延迟测量与表征，为强场物理研究提供了全新的时间分辨视角。本文围绕强场多光子跃迁干涉方法在原子与分子强场多光子电离时间延迟探测中的应用展开，系统阐述该方法的量子干涉机制，总结近年来原子分子阈上电离动力学及共振量子态间阿秒级时间延迟研究方面的最新进展，并展望了该技术在未来可能的应用前景与面临的挑战。
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关键词:
- 强场多光子跃迁干涉方法 /
- 电离时间延迟 /
- 阿秒电子动力学
Attosecond ionization dynamics, as a key research direction in ultrafast science, relies critically on breakthroughs in both experimental techniques and theoretical models to reveal the fundamental processes underlying ultrafast matter evolution. Among the cutting-edge approaches in this field, the strong-field multiphoton transition interferometry (SFMPTI) method stands out for its ability to achieve attosecond time-resolved probing of multiphoton ionization dynamics via quantum path interference. This technique has been widely applied to attosecond-scale measurements and characterizations of ionization time delays with quantum state resolution, ranging from atomic systems to complex molecules, offering a novel time-resolved perspective for strong-field physics.This article focuses on the application of the SFMPTI method in probing strong-field multiphoton ionization time delays in atoms and molecules. We systematically present the quantum interference mechanisms underlying the method, summarize recent progress in attosecond-resolved studies of above-threshold ionization dynamics and resonance-state-mediated delays, and discuss the prospective applications and challenges that lie ahead for this emerging technique.-
Keywords:
- Strong-field multiphoton transition interferometry /
- Ionization time-delay /
- Attosecond electron dynamics
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