Strontium atoms are widely used in quantum information and precision measurement, with their excited states 5s4d
3D
1,2,3 and 5s6s
3S
1 playing key roles in related experiments. However, existing key atomic parameters such as hyperfine structure constants and Landé-
g factors are inconsistent, limiting further research. In this work, we employed the Multi-configuration Dirac-Hartree-Fock (MCDHF) method to systematically optimize the energy levels of the 5s5p
3P
0,1,2, 5s4d
3D
1,2,3,
1D
2 and 5s6s
3S
1,
1S
0 states for strontium, and focused on calculating the hyperfine structure constants (
A and
B) and Landé-
g factors of the 5s4d
3D
1,2,3,
1D
2, and 5s6s
3S
1 states. We comprehensively considered electronic correlation effects through an active space approach and multi-reference single and double excitations (MR-SD) method. The Breit interaction and quantum electrodynamics (QED) corrections were also included to improve calculation accuracy. Moreover, a rigorous uncertainty assessment was conducted in this work. Our results show that the magnetic dipole hyperfine structure constant
A of the 5s4d
3D
1,2,3 triplet has a deviation of less than 3% from experimental values, while that of the 5s6s
3S
1 state is only 0.4%, significantly reducing the prior theory-experiment discrepancy, as shown in figure. Notably, we first reported the theoretical values of the electric quadrupole hyperfine structure constant
B for the 5s4d
3D
1,2,3 states, which are in good agreement with experimental data, filling the theoretical gap. The Landé-
g factor of the 5s4d
3D
1 state deviates by no more than 10
–4 from the experimental value, achieving higher precision than previous studies. Additionally, the calculated lifetimes of these states are consistent with most theoretical and experimental results. This work provides high-precision theoretical parameters for experiments related to strontium optical lattice clocks and quantum information, and verifies the reliability of the MCDHF method in studying highly excited atomic states, laying a foundation for further research on atomic structure and properties.