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中国物理学会期刊

基于轻金属Cr垂直磁化多层膜中轨道霍尔磁电阻研究

Investigation of orbital Hall magnetoresistance in perpendicularly magnetized Cr-based multilayers

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  • 轨道霍尔磁电阻效应是研究轨道流输运和轨道角动量-磁矩相互作用的有效手段,近年来引起研究者广泛关注.但轻金属/磁性材料异质结构中受限于轨道流-自旋流转换效率低,磁电阻数值普遍偏小.本文中,我们利用轻金属Cr的轨道霍尔效应提供轨道流,通过重金属Pt提升轨道流-自旋流转换效率,在垂直磁化Cr(t)/Co/Pt3多层膜体系中获得室温下1.6×10-3的轨道霍尔磁电阻,高出以前同类实验报道1个数量级.同时,利用Cr厚度与磁电阻变化关系拟合出Cr中轨道流扩散长度约为0.93 nm,远小于以前的实验报道.进一步,在Cr/Pt/Co/Pt多层膜中,利用重金属Pt插层提高轨道流-自旋流转换效率,通过轨道霍尔效应和自旋霍尔效应共同作用,有效提升体系磁电阻值达到4.5×10-3.这些结果对理解轨道-磁序耦合机制以及发展低功耗自旋轨道电子器件提供重要实验依据.

     

    Orbital Hall magnetoresistance (OHMR) effect provides a powerful platform for investigating orbital current transport and the coupling between orbital angular momentum and magnetization, and has recently emerged as an important topic in spin–orbitronics. In conventional light-metal/ferromagnet heterostructures, however, the OHMR signal is typically weak due to the intrinsically low efficiency of orbital-to-spin current conversion and limited interfacial transparency, all of which hinder effective transfer of angular momentum to the magnetic layer. In this work, Cr(t)/Co/Pt3 multilayers were fabricated by magnetron sputtering, and their OHMR were systematically investigated at room temperature. In this structure, orbital currents are generated via the orbital Hall effect in the light metal Cr layer. The presence of Pt, a heavy metal with strong spin–orbit coupling, plays a dual role: it enhances orbital-to-spin conversion efficiency through spin–orbit interaction, leading to a pronounced modulation of longitudinal resistance via spin-dependent scattering processes. Consequently, a sizable OHMR of 1.6×10−3 is achieved at room temperature, which is approximately one order of magnitude larger than previously reported values in similar systems. By quantitatively analyzing the dependence of OHMR on Cr thickness using the spin-diffusion model, the effective orbital diffusion length in Cr is extracted to be approximately 0.93 nm. This value is significantly shorter than earlier experimental reports, suggesting that orbital transport in Cr is highly localized and likely dominated by rapid orbital relaxation processes. This observation supports a picture in which orbital angular momentum decays over sub-nanometer length scales rather than propagating over long distances. Furthermore, in Cr/Pt/Co/Pt multilayers, the insertion of a Pt spacer layer between Cr and Co enables more efficient conversion of orbital currents into spin currents. At the same time, the spin Hall effect in the top Pt layer generates an additional spin Hall magnetoresistance (SHMR) contribution. The coexistence and synergistic interplay between OHMR and SMR significantly enhance the overall magnetoresistance, yielding a large value of 4.5×10−3, far exceeding that of conventional heavy-metal/ferromagnet bilayers. These results provide important experimental insights into the microscopic mechanisms governing orbital current generation, diffusion, and conversion, and highlight the crucial roles of spin–orbit coupling in optimizing magnetoresistance effects. This work thus offers valuable guidance for the design of high-efficiency, low-power spin–orbitronic devices based on orbital physics.

     

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