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中国物理学会期刊

Fe3GeTe2/Te-doped BP/Fe3GeTe2范德华异质结构中的自旋阀效应

Spin-Valve Effect in Fe3GeTe2/Te-doped BP/Fe3GeTe2 van der Waals Heterostructures

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  • 自旋阀由铁磁层/间隔层/铁磁层构成,作为自旋电子学的核心部件,广泛应用于磁随机存储器、磁传感器和可编程逻辑器件等存储技术领域.基于二维范德华(vdW)异质结构建的自旋阀,为实现自旋电子器件的低功耗与小型化提供了新的可能.在自旋阀中,间隔层材料的选择对器件性能至关重要.碲掺杂的黑磷晶体(Te-doped BP)带隙不仅具有可调性,而且碲掺杂显著提升了黑磷的环境稳定性并有效抑制了氧化降解过程.本文报道了一种全二维范德华异质结,以二维层状半导体Te-doped BP作为间隔层,二维层状Fe3GeTe2作为铁磁层.在磁电阻的测量中,曲线呈台阶状,表明Fe3GeTe2/Te-doped BP/Fe3GeTe2异质结的自旋阀效应.低温10 K时,异质结的磁电阻率达到0.30%.当磁场方向变化时,磁电阻基本保持不变,这可能源于Fe3GeTe2的垂直磁各向异性.这些结果证实了Te-doped BP作为自旋输运通道的可行性,并突显了Fe3GeTe2/Te-doped BP/Fe3GeTe2异质结在具有角度无关磁阻特性的自旋阀中的应用潜力.

     

    A spin valve is a typical multilayer stacked structure composed of two ferromagnetic layers separated by a nonmagnetic spacer layer. As a core component of spintronics, it is widely used in memory technologies such as magnetoresistive random-access memory, magnetic sensors, and programmable logic devices. In recent years, two-dimensional van der Waals (vdW) materials have exhibited unique advantages in atomically flat interfaces, low defect density, and adjustable electronic band structures, providing an effective pathway for the miniaturization and low power consumption of next-generation spin valve devices. In spin valves, the choice of spacer layer material is critical to device performance. Tellurium-doped black phosphorus (Te-doped BP) is a promising two-dimensional semiconductor with a tunable band gap. Te doping can effectively suppress oxidation degradation process of pristine black phosphorus and significantly enhanced environmental stability, which makes it as an ideal candidate for spin transport channels in vdW heterostructures. In this work, we successfully construct an all-two-dimensional Fe3GeTe2/Te-doped BP/Fe3GeTe2 vdW heterostructure, where the ferromagnetic Fe3GeTe2 nanosheets serve as the upper and lower magnetic electrodes, and the semiconductor Te-doped BP nanosheet acts as the intermediate nonmagnetic spacer layer. Systematic magnetotransport measurements are performed to investigate the spin-dependent transport behavior of the fabricated heterostructure. The measured magnetoresistance curves exhibit step-shape, indicating the spin-valve effect in the Fe3GeTe2/Te-doped BP/Fe3GeTe2 heterostructure. At the low temperature of 10 K, the heterostructure achieves a magnetoresistance ratio of 0.30%. Furthermore, the magnetoresistance remains largely unchanged as the direction of the applied magnetic field changes. This angular-insensitive magnetoresistance characteristic originates from strong perpendicular anisotropy of Fe3GeTe2, namely the fixed orientation of the magnetic moments relative to the applied magnetic field. These results not only confirm the feasibility of using Te-doped BP as a spin transport channel for two-dimensional spintronic devices but also clarify the angular-insensitive magnetoresistance property of Fe3GeTe2-based heterosture. This work broadens the potential application of doped black phosphorus in spintronic devices and provides a feasible experimental reference for the design and fabrication of low-dimensional spin valves with stable magnetotransport performance.

     

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