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中国物理学会期刊

外场驱动下石墨烯正方薄膜中的动力学斯格明子纹理

Dynamical Skyrmion Textures in an Externally Driven Resonant Square Graphene Membrane

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  • 本文针对外场驱动下二维材料振动过程中拓扑结构的形成问题,研究了单层正方形石墨烯薄膜在周期性面外驱动下的共振行为及其三维位移、速度矢量场中的拓扑纹理演化。基于连续张紧膜模型推导了固定边界条件下石墨烯薄膜的本征模态与本征频率关系,并结合Föppl-von Kármán几何非线性讨论了面外振动诱导面内位移的物理机制。基于此,采用分子动力学方法模拟了边长169.74 Å的单层正方形石墨烯在5%等轴拉伸下的高阶共振响应。结果表明,外加周期驱动能够在石墨烯薄膜中激发清晰的高阶驻波振型,理论估算的本征频率与分子动力学模拟中原子振动的快速傅里叶变换提取结果基本一致。进一步分析发现,在特定相位构型下,由完整三维位移矢量场和速度矢量场构造的归一化方向场可形成规则排布的局域拓扑单元,其空间分布与高阶共振模态密切相关。这些局域结构表现出核心-外围反转和径向面内分量等Néel型纹理特征,局域斯格明子数接近±1,并在一个振动周期内随相位发生反转与重复出现。研究结果表明,单层石墨烯薄膜在外场驱动共振过程中不仅表现出清晰的高阶振动模式,而且能够形成具有周期性再现特征的动力学拓扑纹理,为二维材料中振动与拓扑耦合行为的研究提供了新的思路。

     

    Topological textures in externally driven nonequilibrium systems have attracted increasing interest because they provide a route to generating and manipulating nontrivial vector configurations without relying on static magnetic or ferroelectric ordering. Here, we investigate the resonant dynamics of a monolayer square graphene membrane under periodic out-of-plane driving, with particular emphasis on the emergence, spatial organization, and phase-dependent evolution of localized topological textures in the full three-dimensional displacement and velocity fields. A continuum tensioned-membrane model with fixed boundaries is first established to derive the eigenmodes and eigenfrequency relation. The Föppl-von Kármán geometric nonlinearity is then introduced to clarify how finite out-of-plane deformation induces in-plane strain and displacement components, thereby allowing an initially flexural response to develop into a three-dimensional vector field.
    Molecular dynamics simulations are performed for a monolayer square graphene membrane containing 11040 carbon atoms and having a side length of 169.74 Å. The membrane is subjected to a uniform equibiaxial prestrain of 5%, fully relaxed, thermally equilibrated at 300 K, and fixed along finite-width boundary regions. A spatially uniform harmonic force is subsequently applied to the movable atoms in the out-of-plane direction. The effective two-dimensional pretension extracted from the equilibrated in-plane stress is approximately 11.62 N/m. Substituting this value into the continuum model yields a fundamental frequency of approximately 0.163 THz, in close agreement with the value of 0.16 THz obtained from fast Fourier transform analysis of the molecular dynamics trajectories. By tuning the driving frequency to successive resonances, clear standing-wave patterns from low- to high-order modes are obtained. As the resonance order increases, the number of nodal lines grows and the membrane is progressively divided into regularly arranged localized vibration cells.
    To determine whether these localized cells possess nontrivial topology, the complete atomic displacement and velocity vectors are reconstructed from the molecular dynamics trajectories, interpolated onto a two-dimensional grid, normalized, and mapped onto the unit sphere. The corresponding local skyrmion density and skyrmion number are then evaluated from the spatial derivatives of the normalized vector fields. At selected resonance phases, both displacement and velocity fields exhibit a continuous core-to-background reversal of the out-of-plane component together with predominantly radial in-plane components, forming Néel-type skyrmion-like textures. These localized units are spatially locked to the high-order standing-wave pattern rather than being ordinary vibration extrema. For the velocity field under the sixth-order resonance, the average local skyrmion number of several cores reaches approximately Nsk = 0.9923, demonstrating a nearly integer real-space winding.
    Phase-resolved analysis over one oscillation period further reveals that the localized topological units are intrinsically dynamical. Their vector configurations evolve continuously with the driving phase, remain close to Nsk = +1 or -1 over most phase intervals, and pass through noninteger transitional states during polarity reversal. The term “stable” therefore refers to reproducible recurrence under sustained resonant driving rather than to a time-independent or intrinsically protected state. These results establish a direct connection among flexural resonance, geometric nonlinearity, and real-space topology in an atomically thin membrane, and demonstrate that high-order mechanical resonance can generate periodically recurring dynamical topological textures. The proposed mechanism also provides a physical basis for frequencyaddressable topological encoding, topology-assisted mode recognition, and multimodal mechanical sensing in two-dimensional nanoelectromechanical systems.

     

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