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中国物理学会期刊

非互易相互作用胶体粒子的定向输运

Directed transport of colloidal particles with non-reciprocal interactions

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  • 本文基于多种类胶体粒子非互易相互作用模型,研究了热噪声强度、外势高度、非对称系数以及非互易相互作用系数对胶体粒子系统定向输运的影响.研究发现,热噪声强度、外势高度和非对称系数在一定条件下都能促进胶体系统的定向运动,且均存在最优的参数能使胶体系统的平均速度达到峰值.特别地,研究发现非互易相互作用是驱动胶体系统定向输运的决定性因素.同时,不同粒子间还存在一对最优的非互易相互作用匹配系数能使胶体粒子的定向输运达到最强.此外,通过功率谱密度分析进一步揭示了非互易相互作用导致多组分胶体系统定向输运增强的物理机制.研究结果可为未来智能胶体自组装、靶向药物输送及动态响应超材料等领域的实验设计与应用提供理论参考.

     

    For complex colloidal suspensions, colloidal particles typically interact with other types of particles in their surrounding environment. Extensive experimental studies have demonstrated that the interactions between various types of particles are usually nonreciprocal. So far, although various directed motion mechanisms for multi-species colloidal particles have been discovered, these works mainly focus on the reciprocal interactions between particles. However, in numerous complex solution environments, nonreciprocal interactions are the key factors that cause directed motion in complex systems, especially in systems with multiple types of colloidal particles. Therefore, this article further explores the directed transport behavior of colloidal particles under the influence of nonreciprocal interactions.
    This work is based on a nonreciprocal interaction model of multiple types of colloidal particles. And the effects of thermal noise intensity, external potential barrier height, asymmetry coefficient, and asymmetric interaction coefficient on the directional transport of colloidal particle systems have been studied. It is found that thermal noise intensity, external potential height, and asymmetry coefficient can all promote the directional motion of colloidal systems under certain conditions. Moreover, there exists an optimal parameter at which the average velocity of the colloidal system possess its largest value. In addition, non reciprocal interactions are the determining factor driving the directional transport of colloidal systems. There exists an optimal pair of non reciprocal interaction matching coefficients between different particles, which can maximize the directional transport of colloidal particles. Through the analysis of power spectral density, the physical mechanism by which non-reciprocal interactions enhance the directional transport in multicomponent colloidal systems has been further elucidated. The research results of this article can provide theoretical references for experimental design and applications in future fields such as intelligent colloidal self-assembly, targeted drug delivery, and dynamically responsive metamaterials.

     

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