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中国物理学会期刊

射频交变磁场对离子回旋共振分离锂同位素的影响研究

Effect of Radio Frequency Alternating Magnetic Field on Lithium Isotope Separation by Ion Cyclotron Resonance

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  • 基于SIRENA装置实验参数,在HybridCircuit/3DLHDAP仿真软件中构建了四臂螺旋天线离子回旋共振(ion cyclotron resonance, ICR)法分离锂同位素的三维物理模型。在单粒子近似条件下,采用有限元法结合含碰撞效应的冷等离子体介电张量分析了射频天线交变磁场对收集板处锂离子横向能量和分离间距的影响。模拟结果表明:1)射频交变磁场作用下,收集板处6Li+的横向能量及其与7Li+的分离间距峰值均向低频偏移。2)射频交变磁场使磁场梯度漂移效应不可忽略,导致收集板处6Li+的横向能量及其与7Li+的分离间距均随馈入电压和初始横向速度呈非线性变化。同时,馈入电压与初始横向速度均存在最优阈值(分别为6 kV和30 km/s),可使二者达到峰值。3)考虑射频交变磁场效应后,初始轴向速度的最优阈值高于未考虑该效应时的取值。4)在射频频率为774 kHz、馈入电压为6 kV、离子横向速度为30 km/s、轴向速度为40-60 km/s的条件下,射频交变磁场有利于提高收集板处6Li+的横向能量及其与7Li+的分离间距。相关研究结果为ICR法分离同位素实验提供了理论指导。

     

    Ion Cyclotron Resonance (ICR) is a method that uses cyclotron waves at the resonant frequency of target ions to heat the plasma. Owing to its low energy consumption, high separation factor, and ability to effectively circumvent Coulomb repulsion limitations caused by space charge effects in conventional electromagnetic methods, it has become a highly promising isotope separation technology. Magnetic field is a key parameter affecting the performance of isotope separation using the ICR method. Existing theoretical studies on ICR-based isotope separation generally assume a uniform background magnetic field and an ideal circularly polarized electric field (neglecting the RF magnetic field). However, under experimental conditions, plasma collective effects and the actual structure of the antenna can disrupt the ideal circular polarization state of the electric field, in which case the influence of the RF alternating magnetic field on ion motion may no longer be negligible.
    Based on the parameters of the Russian SIRENA device, a three-dimensional physical model for lithium isotope separation by ion cyclotron resonance heating with a four-arm helical antenna was built in the HybridCircuit/3DLHDAP simulation software. Under the single-particle approximation, the finite element method, together with a collision-inclusive cold plasma dielectric tensor, was used to analyze how the RF antenna's alternating magnetic field affects the transverse energy and separation distance of lithium ions at the collector plate.
    The simulation results indicate: 1) Under the influence of the RF alternating magnetic field, which makes the magnetic field gradient drift effect no longer negligible, both the peak transverse energy of the resonant ion 6Li+ and the peak separation distance between 6Li+ and 7Li+ at the collector plate shift toward lower frequencies. Furthermore, both parameters show nonlinear dependences on the feeding voltage and initial transverse velocity, with optimal thresholds of 6 kV and 30 km/s, respectively. 2) When the RF alternating magnetic field effect is taken into account, the optimal threshold of the initial axial velocity becomes higher than that without this effect. 3) Under the conditions of an RF frequency of 774 kHz, a feeding voltage of 6 kV, an ion transverse velocity of 30 km/s, and an axial velocity of 40-60 km/s, the RF alternating magnetic field is beneficial for enhancing the transverse energy of 6Li+ and the separation distance between 6Li+ and 7Li+ at the collector plate.
    This study reveals the dual-action mechanism of the RF alternating magnetic field in ICR lithium isotope separation, corrects the theoretical deviation of the conventional uniform magnetic field model, and provides a more accurate theoretical basis for the experimental design and parameter optimization of ICR isotope separation devices. Future work will further investigate the effects of plasma temperature, antenna structure, and other factors on the isotope separation process.

     

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