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中国物理学会期刊

基于格子Boltzmann方法的复杂管道中溶质输运特性研究

Transport Characteristics of Solute in Complex Channels Based on Lattice Boltzmann Method

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  • 本文针对复杂管道中的溶质输运问题,构建了一种通过源项重构对流项的高精度格子Boltzmann模型,并将其应用于直管道、平行正弦管道和对称正弦管道中的溶质输运模拟。在固定雷诺数\(Re=10\)条件下,系统研究了佩克莱数\(Pe\)和几何振幅\(\varepsilon\)对溶质云团截面平均浓度分布、质量加权平均速度及有效弥散系数的影响。Taylor-Aris弥散算例表明,本文模型计算得到的有效弥散系数与理论解吻合良好,相对误差小于\(0.1\%\)。结果表明,直管道中溶质云团保持较规则的轴向展布形态,\(Pe\)主要通过改变有效弥散系数\(D_\mathrmeff\)影响云团展宽和峰值浓度,而对质量加权平均速度影响较弱。平行正弦管道中,局部截面高度保持恒定,增大\(\varepsilon\)仅使质量加权平均速度略有降低,对截面平均浓度分布的影响较弱;不同\(Pe\)下速度曲线基本重合,说明\(Pe\)的作用主要体现在弥散展宽过程。对称正弦管道中,局部截面高度沿流向周期变化,收缩-扩张结构使浓度主峰滞后,并降低质量加权平均速度,表现出较平行正弦管道更强的几何调制作用。进一步,基于\(10\le Pe\le120\)、\(0.05\le\varepsilon\le0.3\)范围内的数值结果,建立了平行正弦管道中\(D_\mathrmeff/D\)关于\(Pe\)和\(\varepsilon\)的经验关联式,揭示了等截面中心线弯曲对Taylor-Aris弥散的量化调制机制。

     

    Solute transport in complex channels is widely involved in environmental flows, microfluidic systems, porous media transport, and biochemical mixing processes. Compared with straight channels, curved or periodically varying channels can significantly modify the migration, spreading, and effective dispersion of solute clouds through the coupling between flow structures and wall geometries. To quantitatively investigate these effects, a high-accuracy multiple-relaxation-time lattice Boltzmann method (MRT-LBM) is developed based on the source-term reconstruction of the convection term. In this model, the convection term in the convection-diffusion equation is reformulated as a source term, so that the solute transport equation can be solved in the form of a diffusion equation with a reconstructed source. This treatment avoids the additional deviation that may be introduced by the conventional velocity-dependent equilibrium distribution and is suitable for high-accuracy simulations of solute transport in complex geometries.
    Three typical two-dimensional channels are considered, namely a straight channel, a parallel sinusoidal channel with a constant local height, and a symmetric sinusoidal channel with a periodically varying local height. The Reynolds number is fixed at Re=10, and the Peclet number Pe is adjusted by changing the molecular diffusion coefficient D, while the background flow field remains nearly unchanged under different Pe conditions. The effects of Pe and the geometric amplitude \varepsilon on the cross-sectionally averaged concentration distribution, the mass-weighted average velocity, and the effective dispersion coefficient are systematically analyzed. The accuracy of the present model is first verified by the classical Taylor-Aris dispersion problem in a plane Poiseuille flow. The effective dispersion coefficients calculated by the present model agree well with the theoretical solution, with relative errors less than 0.1\%, demonstrating the high accuracy of the present model in capturing the long-time axial dispersion behavior of solute clouds.
    The numerical results show that the transport mechanisms are strongly dependent on the channel geometry. In the straight channel, the solute cloud maintains a regular axial distribution without obvious geometric distortion. The variation of Pe mainly changes the effective dispersion coefficient D_\mathrmeff, thereby affecting the axial spreading range and the peak concentration of the solute cloud, whereas its influence on the mass-weighted average velocity is weak. In the parallel sinusoidal channel, the upper and lower walls shift synchronously along the streamwise direction, and the local channel height remains constant. As a result, increasing \varepsilon mainly enhances the lateral deflection of the solute cloud along the curved centerline, but has only a weak effect on the axial concentration distribution. The mass-weighted average velocity decreases slightly with increasing \varepsilon, while the velocity curves obtained at different Pe nearly overlap, indicating that Pe mainly affects the dispersion process rather than the overall migration speed.
    In contrast, the symmetric sinusoidal channel exhibits a much stronger geometric modulation effect. Since the local channel height varies periodically along the streamwise direction, alternating contraction and expansion regions are formed. With increasing \varepsilon, the concentration peak shows an obvious axial lag, and the mass-weighted average velocity decreases significantly. This indicates that the periodic contraction-expansion structure can suppress the overall axial migration of the solute cloud and enhance the coupling between geometric modulation and dispersion. At relatively small amplitudes, the concentration distribution still exhibits characteristics similar to Taylor-Aris dispersion. However, when \varepsilon becomes large, the influence of the varying cross-section becomes dominant, and the concentration profiles under different Pe show more complicated differences.
    Furthermore, based on numerical results in the ranges of 10\le Pe\le120 and 0.05\le\varepsilon\le0.3, an empirical correlation for D_\mathrmeff/D in the parallel sinusoidal channel is established. The correlation retains the Taylor-Aris-type Pe^2-dominated structure and introduces a geometric correction factor related to \varepsilon, thereby providing a quantitative description of the effective dispersion coefficient in a channel with a constant cross-section and a periodically curved centerline. These results demonstrate that the present high-accuracy MRT-LBM can effectively describe solute transport in complex channels and provide a useful numerical framework for analyzing geometry-regulated dispersion processes.

     

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