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中国物理学会期刊

微波场与磁场失配下超冷分子微波屏蔽的稳健性

Robustness of microwave shielding for ultracold molecules under mismatched microwave and magnetic fields

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  • 近年来,微波屏蔽技术在超冷分子领域取得了重大突破.通过施加合适的微波场,超冷分子在碰撞过程中保持稳定,分子间的相互作用也能得到方便有效的调节.为实现良好的微波屏蔽,除了微波场外,通常还需要施加较强的磁场.然而,在当前实验中,微波场与磁场常常处于失配状态.本文通过数值求解失配微波场和磁场下的超冷分子行为,系统论证了这种失配对屏蔽效应的影响极为微弱,这同时也解释了当前常用的无内态结构的刚性转子模型可靠性的物理起源.

     

    Microwave shielding has recently emerged as a powerful technique for suppressing inelastic collisions and enabling evaporative cooling of ultracold polar molecules. With appropriately applied microwave fields, a repulsive shielding barrier emerges at short range, which prevents molecules from reaching reactive collision distances. So far, both fermionic and bosonic molecular gases can be cooled below the degeneracy temperature through microwave shielding. Moreover, it offers a convenient method to tune molecular interaction. In addition to the microwave field, achieving effcient microwave shielding requires a strong bias magnetic field to define a quantization axis and to suppress processes that involve changes in the internal spin degrees of freedom. In current experimental setups, the polarization or spatial orientation of the microwave field is often not perfectly aligned with the magnetic field, which is referred to as mismatched fields, leaving an important gap between idealized theoretical treatments and practical experiments.
    In this work, we theoretically investigate the impact of mismatches between microwave and magnetic fields on the shielding performance. By performing multi-channel scattering calculations together with adiabatic potential analyses for two colliding polar molecules, we systematically vary the mismatch angle and examine the resulting scattering rates. We demonstrate that the shielding effect is highly robust even under significant mismatches: the elastic scattering rate remains essentially unchanged, while the inelastic loss rate stays effciently suppressed to a level comparable to the perfectly aligned case. More importantly, we identify the underlying physical mechanism behind this robustness. We find that in a suffciently strong magnetic field, the projection of the molecular nuclear spin is hardly affected by the mismatch angle. As a result, the molecular state can be accurately approximated as a direct product of a rotational state and a fixed nuclear-spin projection state. This observation reveals that the primary role of the magnetic field is to lock the nuclear-spin projection of the molecule, which does not require precise alignment with the microwave field. Consequently, the microwave shielding effect for ultracold polar molecules is remarkably robust against mismatches between the microwave and magnetic fields.
    Our findings also provide a natural explanation for experimental observations reported in earlier works: even a simple rigid-rotor model that completely ignores hyperfine structure can reproduce experimental results quantitatively, regardless of the mismatch. In typical ultracold molecule experiments, the microwave field often has a large ellipticity, which tends to obscure the subtle effects of field mismatches and hyperfine details. Under such conditions, treating the molecule as a structureless rigid rotor becomes fully adequate.

     

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