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中国物理学会期刊

强场量子相干辐射及应用

Strong-field-induced quantum coherent emission and its applications

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  • 近年来,强场物理与量子光学两个领域交叉产生的物理效应正逐步成为研究热点。融合超快宽谱激发与共振调控,可在亚周期内制备电子-电子、电子-离子多体纠缠与相干,进而产生强场相干性诱导的空气激光、超连续辐射与自由感应衰变等新型相干辐射。本文围绕强场量子光学这一新兴交叉领域,聚焦强场下量子相干辐射及应用,综述其理论基础、物理机制及潜在应用等方面的现状和挑战。期望以此推动开放系统多体强场量子光学的理论与实验研究,以及对多自由度强场量子相干性建立、演化与弛豫规律的探索,拓展强场量子相干辐射与放大机制,为构建时-频-空稳定可控的新型辐射源、发展远程探测新技术、实现空气激光在痕量分子检测与燃烧诊断等方面的应用提供参考。

     

    Intense ultrashort laser fields can prepare quantum coherence and multi-body entanglement in atoms and molecules on a sub-cycle timescale by combining broadband excitation with resonant coupling. Unlike conventional quantum optics, where coherence is built through the resonant interaction of weak narrowband light with atoms, here the coherence is created in an open, nonequilibrium system that undergoes ionization and radiates while the driven process is still under way. This review surveys the emerging field of strong-field quantum optics, covering the creation, diagnosis and application of such coherence. Five elementary processes are analyzed as sources of strong-field coherence: ionization and excitation that leave the ion in a superposition of electronic states, vibrational and rotational wave-packet formation in molecules, nonadiabatic coupling that redistributes coherence among electronic and nuclear degrees of freedom, entanglement between the photoelectron and the parent ion, and multi-electron coherence that initiates charge migration. These processes give rise to novel coherent emissions, including N2+ air lasing, ultraviolet supercontinuum radiation and free induction decay. The gain mechanism of N2+ air lasing remains controversial, and competing scenarios including population inversion, lasing without inversion, superradiance and post-pulse free induction decay are compared. We present an ionization-coupling theoretical framework that treats strong-field ionization and subsequent laser-ion coupling on the same footing, and discuss the challenges of extending it to many-electron, multi-degree-of-freedom open systems and to collective emission. On the experimental side, multidimensional spectroscopy, attosecond transient-absorption spectroscopy and photoelectron momentum spectroscopy are reviewed as state-resolved probes of coherence dynamics. Finally, the unique properties of air lasing and its potential applications in remote sensing, trace-gas detection and combustion diagnostics are discussed. Realizing air lasing as a practical radiation source with controllable temporal, spectral and spatial properties requires improving the output brightness and suppressing the supercontinuum background generated during filamentation.

     

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