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中国物理学会期刊

Gd替代YBa2Cu3O7-δ超导体的相结构与局域电子结构的研究

CSTR: 32037.14.aps.54.5382

Phase structures and local electron structures of Gd-doped YBa2Cu3O7-δ systems

CSTR: 32037.14.aps.54.5382
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  • 利用正电子湮没实验,结合x射线衍射(XRD)结构分析,研究了具有混合稀土特征的(Y1 -xGdx)Ba2Cu3O7-δ系列样品. XRD 实验结果表明,半径较大的Gd离子Y位替代使得样品晶胞参数和晶胞体积增大,但所有样品 仍保持与YBa2Cu3O7-δ(YBCO)样品相同的单相正交结 构. 正电子湮没实验表明,正电子各寿命参数表现出很强的Gd替代依赖关系. 从正电子实验 结果出发,计算了Cu-O链区局域电子密度ne的变化. 结果表明,局域电子密度n e随Gd含量x的增加而减小,而超导转变温度Tc随局域电子密度ne的减小而增加,这种局域电子密度ne与超导电性的关联是与铜位替代 完全不同的,且可能是近年来人们关于混合稀土铜氧化物体系具有较高临界电流密度的原因 之一. 该研究结果为铜氧化物超导体的应用和机理研究提供了相应的正电子实验资料.

     

    The Gd substituted Y1-xGdxBa2Cu3O7-δ systems are studied systematically by positron annihilation and x-r ay diffraction. The x-ray results show that the crystal parameters and crystal v olume of the systems increase with the increase of Gd content. However, all the substituted samples maintain the single orthorhombic phase as YBa2Cu3O7-δ (YBCO) sample does. The positron annihilation result s show that positron lifetimes depend on the Gd content strongly. According to t he positron annihilation result, the local electronic density on Cu-O chain is c alculated. The result shows the local electronic density decreases with the incr ease of the Gd content, while the Tc increases with the decrease of t he local electronic density. The relationship between the local electronic densi ty and superconductivity is different from the substitution on Cu site, which ma y be one of the reasons why the mixed rare earth cuprate superconductor has a hi gher critical electric current density than the YBCO. These experimental results give the corresponding positron experiment data for the application of cuprate superconductors and study of the mechanism.

     

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