高压下富氢高温超导体的研究进展

孙莹; 刘寒雨; 马琰铭

doi:10.7498/aps.70.20202189

摘要

近年来, 高压强极端条件下的富氢化合物成为高温超导体研究的热点目标材料体系. 该领域目前取得了两个标志性重要进展, 先后发现了共价型H₃S富氢超导体(T_c = 200 K)和以LaH₁₀(T_c = 260 K, –13 ℃), YH₆, YH₉等为代表的一类氢笼合物结构的离子型富氢超导体, 先后刷新了超导温度的新纪录. 这些研究工作燃发了人们在高压下富氢化合物中发现室温超导体的希望. 本文重点介绍高压下富氢高温超导体的相关研究进展, 讨论富氢化合物产生高温超导电性的物理机理, 展望未来在富氢化合物中发现室温超导体的可能性并提出多元富氢化合物候选体系.

关键词:

Abstract

In recent years, hydrogen-rich compounds under extremely high pressure have become the hot target materials for high-temperature superconductors. At present, two landmark progresses have been made in this field. Covalent H₃S hydrogen-rich superconductors (T_c = 200 K) and ionic hydrogen-rich superconductors with hydrogen-cage structure, such as LaH₁₀ (T_c = 260 K, –13 ℃), YH₆ and YH₉, have been successively synthesized, setting a new record of superconducting temperature. These studies have given rise to the hope of discovering room-temperature superconductors in hydrogen-rich compounds under high pressure. This paper focuses on the progress of hydrogen-rich superconductors with high critical temperature under high pressure, discusses the physical mechanism of high-temperature superconductivity in hydrogen-rich compounds, provide an outlook on the possibility of discovering room-temperature superconductors in hydrogen-rich compounds in the future, and offer the candidate system for high superconductivity in multiple hydrogen-rich compounds.

Keywords:

作者及机构信息

1.
吉林大学物理学院, 超硬材料国家重点实验室, 长春　130012

2.
吉林大学物理学院, 计算方法与软件国际中心, 长春　130012

3.
吉林大学, 未来科学国际合作联合实验室, 长春　130012

通信作者: 刘寒雨, lhy@calypso.cn ; 马琰铭, mym@jlu.edu.cn

基金项目: 国家自然科学基金重大项目(批准号: 52090024)、中国科学院战略性先导科技专项(批准号: XDB33000000)、国家自然科学基金(批准号: 12074138)和中国博士后科学基金(批准号: 2020M681032)资助的课题

Authors and contacts

1.
State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun 130012, China

2.
International Center for Computational Method and Software, College of Physics, Jilin University, Changchun 130012, China

3.
International Center of Future Science, Jilin University, Changchun 130012, China

Corresponding author: Liu Han-Yu, lhy@calypso.cn ; Ma Yan-Ming, mym@jlu.edu.cn

Funds: Project supported by the Major Program of the National Natural Science Foundation of China (Grant No. 52090024), the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB33000000), the National Natural Science Foundation of China (Grant No. 12074138), and the China Postdoctoral Science Foundation (Grant No. 2020M681032)

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施引文献

图 1 超导体年表. 方形、圆形和菱形色块分别表示BCS超导体、铜氧化物超导体和铁基超导体. 黑色和蓝色标签分别标注常压超导材料和高压超导材料及合成压强

Fig. 1. Timeline of superconductors. The square, circle, and rhombus color blocks respectively represent BCS superconductors, cuprate superconductors, and iron-based superconductors. Black and blue labels represent superconducting materials at atmospheric pressure and high pressure as well as the pressure value required to synthesize these superconductors.

下载: 全尺寸图片幻灯片

[1]	赵忠贤, 陈立泉, 崔长庚, 黄玉珍, 刘锦湘, 陈赓华, 李山林, 郭树权, 何业冶 1987 科学通报 32 177 Google Scholar Zhao Z X, Chen L Q, Cui C G, Huang Y Z, Liu J X, Chen G H, Li S L, Guo S Q, He Y Z 1987 Chin. Sci. Bull. 32 177 Google Scholar
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