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中国物理学会期刊

Z = 118—120超重核α衰变性质的研究

CSTR: 32037.14.aps.74.20240907

Research on α decay properties of superheavy nuclei with Z = 118–120

CSTR: 32037.14.aps.74.20240907
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  • 本文通过考虑原子核的形变效应和引入α粒子预形成因子的解析表达式对统一裂变模型(unified fission model, UFM)进行改进. 通过考虑原子核形变效应得到了改进的UFM (improved UFM-1, IMUFM1), 在IMUFM1基础上引入α粒子预形成因子的解析表达式得到了进一步改进的UFM (improved UFM-2, IMUFM2). 利用UFM, IMUFM1和IMUFM2三个版本分别对 Z \geqslant 92 重核和超重核的α衰变半衰期进行了系统地计算. 通过计算理论值和实验值之间的平均偏差和标准偏差, 发现IMUFM1的精度比UFM的精度仅提高了2.45%, 而IMUFM2的精度却提高了32.09%. 接着, 通过有限力程小液滴模型(finite-range Droplet model-2012, FRDM2012), Weizsäcker-Skyrme-4 (WS4)和Koura-Tachibana-Uno-Yamada (KTUY) 3种质量模型分别提取了Z = 118—120同位素链的α衰变能, 并利用IMUFM1和IMUFM2计算了相应的α衰变半衰期. 通过观察半衰期随同位素链的演化, 发现不同质量模型预言的演化趋势是一致的, 而且在N = 178和N = 184处会出现转折点, 但不同的质量模型预言的α衰变半衰期会出现数量级的差异. 另外, 通过讨论α衰变和自发裂变之间的竞争, 发现N<186质量核区的超重核以α衰变为主. 最后, 结合上述3种核质量模型, 利用IMUFM1和IMUFM2讨论了296Og, 297119和298120 α衰变链的衰变模式, 发现WS4和KTUY两种质量模型的预言结果与实验结果一致. 尽管FRDM2012质量模型预言的288Fl, 285Nh 和 286Fl的衰变模式与实验结果有所差别, 但对于288Fl, IMUFM2的预言结果比IMUFM1更符合实验测量结果, 再次验证了IMUFM2的合理性和可靠性. 上述研究结果可为将来实验鉴别新核素提供理论依据.

     

    An unified fission model (UFM) has been improved by considering the nuclear deformation effect and introducing an analytical expression of preformation factor. The improved version of the UFM by taking into consideration the nuclear deformation effect is named IMUFM1. Based on the IMUFM1, the further improved version is termed IMUFM2, which incorporates an analytical expression of the preformation factor. Within the UFM, the IMUFM1 and the IMUFM2, the α decay half-lives of heavy and superheavy nuclei with Z \geqslant 92 are systematically calculated. The calculated standard deviation between the calculation results and the experimental data shows that the accuracy of the IMUFM1 is improved by 2.45% compared with that of the UFM. The accuracy of the IMUFM2 will be further improved by 32.09% compared with that of the IMUFM1, which implies that the nuclear deformation effect and the preformation factor are both important in prediction. Then, the α decay half-lives of Z = 118–120 isotopes are predicted from the IMUFM1 and the IMUFM2 by inputting the α decay energy values that are extracted from the sinite-range droplet model (FRDM), the Weizsäcker-Skyrme-4 (WS4) model and the Koura-Tachibaba-Uno-Yamads (KTUY) formula, respectively. The observed evolution of the α decay half-lives indicates that the evolution trends obtained from the above-mentioned three mass models are consistent with each other and the shell effects occur at N = 178 and 184, but their orders of magnitude, obtained from different mass models, are different from each other. Meanwhile, the comparison of half-lives between α decay and spontaneous fission shows that the dominant decay modes of the superheavy nuclei with N < 186 are α decay. Finally, the decay modes of 296Og, 297119 and 298120 α decay chains are predicted within the IMUFM1 and the IMUFM2 by using these three mass models, showing that the predictions from the WS4 mass model and KTUY mass model are more consistent with the experimental measurements. Form the FRDM2012 mass model, the predictions of 288Fl, 285Nh and 286Fl within the IMUFM1 mass model are not consistent with the experimental measurements, however, the prediction of 288Fl from the IMUFM2 is good agreement with the experimental measurement, which once again verifies the rationality and reliability of the IMUFM2. This study may be helpful for identifying new nuclide in future experiments.

     

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